Ultrafast Optical Excitation of a Combined Coherent-Squeezed Phonon field in SrTiO3
Optics Express, Vol. 1, Issue 12, pp. 385-389 (1997)
http://dx.doi.org/10.1364/OE.1.000385
Enhanced HTML
Acrobat PDF (123 KB)
Abstract
We have simultaneously excited a coherent and a squeezed phonon field in SrTiO3 using femtosecond laser pulses and stimulated Raman scattering. The frequency of the coherent state (~ 1.3 THz) is that of the A1g-component of the soft mode responsible for the cubic-tetragonal phase transformation at ≈ 110 K. The squeezed field involves a continuum of transverse acoustic phonons dominated by a narrow peak in the density of states at ~ 6.9 THz.
© Optical Society of America
[Optical Society of America ]
OCIS Codes
(270.1670) Quantum optics : Coherent optical effects
(290.5910) Scattering : Scattering, stimulated Raman
(320.7130) Ultrafast optics : Ultrafast processes in condensed matter, including semiconductors
ToC Category:
Focus Issue: Coherent Phenomena in Solids
History
Original Manuscript: September 30, 1997
Published: December 8, 1997
Citation
Gregory Garrett, John Whitaker, Ajay Sood, and Roberto Merlin, "Ultrafast Optical Excitation of a Combined Coherent-Squeezed Phonon field in SrTiO3," Opt. Express 1, 385-389 (1997)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-1-12-385
Sort: Journal | Reset
References
- R. Merlin, Generating coherent THz phonons with light pulses, Solid State Commun. 102, 207-220 (1997). [CrossRef]
- G. A. Garrett, A. G. Rojo, A. K. Sood, J. F. Whitaker and R. Merlin, Vacuum squeezing of solids: macroscopic quantum states driven by light pulses, Science 275, 1638-1640 (1997). [CrossRef] [PubMed]
- See, e. g., D. F. Walls and G. J. Wilburn, Quantum Optics (Springer, Berlin, 1994), chap. 2.
- P. A. Fleury, J. F. Scott and J. M. Worlock, Soft phonon modes and the 110 0 K phase transition in SrTiO3, Phys. Rev. Lett. 21, 16-19 (1968). [CrossRef]
- K. A. Mller and H. Burkard, SrTiO3: an intrinsic quantum paraelectric below 4 K, Phys. Rev. B 19, 3593-3602 (1979). [CrossRef]
- See: W. Zhong and D. Vanderbilt, Effect of quantum fluctuations on structural phase transitions in SrTiO3 and BaTiO3, Phys. Rev. B 53, 5047-5050 (1996), and references therein. [CrossRef]
- P. A. Fleury and J. M. Worlock, Electric-Field-Induced Raman scattering in SrTiO3 and BaTiO3, Phys. Rev. 174, 613-623 (1968) [CrossRef]
- D. E. Grupp and A. M. Goldman, Giant piezoelectric effect in strontium titanate at cryogenic temperatures, Science 276, 392-394 (1997). [CrossRef] [PubMed]
- H. Uwe and T. Sakudo, Stress-induced ferroelectricity and soft modes in SrTiO3, Phys. Rev. B 13, 271-286 (1976). [CrossRef]
- W. G. Nielsen and J. G. Skinner, Raman spectrum of strontium titanate, J. Chem. Phys. 48, 2240-2248 (1968). [CrossRef]
- W. G. Stirling, Neutron inelastic scattering study of the lattice dynamics of strontium titanate: harmonic models, J. Phys. C 5, 2711-2730 (1972). [CrossRef]
Cited By |
OSA is able to provide readers links to articles that cite this paper by participating in CrossRef's Cited-By Linking service. CrossRef includes content from more than 3000 publishers and societies. In addition to listing OSA journal articles that cite this paper, citing articles from other participating publishers will also be listed.
Multimedia
| Multimedia Files | Recommended Software |
| » Media 1: MOV (55 KB) | QuickTime |
| » Media 2: MOV (56 KB) | QuickTime |
| » Media 3: MOV (162 KB) | QuickTime |





OSA is a member of 