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Optics Express

Optics Express

  • Editor: Michael Duncan
  • Vol. 11, Iss. 19 — Sep. 22, 2003
  • pp: 2440–2445

Frequency conversion of subnanojoule femtosecond laser pulses in a microstructure fiber for photochromism initiation

Stas O. Konorov and Aleksei M. Zheltikov  »View Author Affiliations


Optics Express, Vol. 11, Issue 19, pp. 2440-2445 (2003)
http://dx.doi.org/10.1364/OE.11.002440


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Abstract

Microstructure fibers with multiple submicron cores are used to frequency-convert unamplified 0.3-nJ, 80-fs pulses of 800-nm Ti: sapphire laser radiation to the spectral range of 400–500 nm. This frequency-upconverted radiation is then employed to induce reversible changes in the absorption spectrum of spiropyran molecules through photochromic transformations in a solid-phase spiropyran/PMMA sample. Microstructure fibers are thus shown to enhance the capabilities of low-power femtosecond lasers, making unamplified ultrashort pulses suitable for photochemical and micromachining applications.

© 2003 Optical Society of America

OCIS Codes
(120.4610) Instrumentation, measurement, and metrology : Optical fabrication
(190.4370) Nonlinear optics : Nonlinear optics, fibers

ToC Category:
Research Papers

History
Original Manuscript: August 6, 2003
Revised Manuscript: September 12, 2003
Published: September 22, 2003

Citation
Stas Konorov and Aleksei Zheltikov, "Frequency conversion of subnanojoule femtosecond laser pulses in a microstructure fiber for photochromism initiation," Opt. Express 11, 2440-2445 (2003)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-11-19-2440


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References

  1. J.C. Knight, T.A. Birks, P.St.J. Russell, and D.M. Atkin, �??All-silica single-mode optical fiber with photonic crystal cladding,�?? Opt. Lett. 21, 1547-1549 (1996). [CrossRef] [PubMed]
  2. J.C. Knight, J. Broeng, T.A. Birks, and P.St.J. Russell, �??Photonic bandgap guidance in optical fibers,�?? Science 282, 1476-1478 (1998). [CrossRef] [PubMed]
  3. W.H. Reeves, J.C. Knight, P.St.J. Russell, and P.J. Roberts, �??Demonstration of ultraflattened dispersion in photonic crystal fibers,�?? Opt. Express 10, 609-613 (2002), <a href= �??http://www.opticsexpress.org/abstract.cfm?URI=OPEX-10-14-609">http://www.opticsexpress.org/abstract.cfm?URI=OPEX-10-14-609</a>. [CrossRef] [PubMed]
  4. N.G.R. Broderick, T.M. Monro, P.J. Bennett, and D.J. Richardson, �??Nonlinearity in holey optical fibers: measurement and future opportunities,�?? Opt. Lett. 24, 1395-1397 (1999). [CrossRef]
  5. A.B. Fedotov, A.M. Zheltikov, A.P. Tarasevitch, and D. von der Linde, �??Enhanced spectral broadening of short laser pulses in high-numerical-aperture holey fibers,�?? Appl. Phys. B 73, 181-184 (2001). [CrossRef]
  6. Nonlinear optics of photonic crystals, Feature issue of J. Opt. Soc. Am. B 19, no. 9 (2002).
  7. B. J. Eggleton, C. Kerbage, P. S. Westbrook, R. S. Windeler, and A. Hale, �??Microstructured optical fiber devices,�?? Opt. Express 9, 698-713 (2001), <a href= �??http://www.opticsexpress.org/abstract.cfm?URI=OPEX-9-13-698.">http://www.opticsexpress.org/abstract.cfm?URI=OPEX-9-13-698</a>. [CrossRef] [PubMed]
  8. J.K. Ranka, R.S. Windeler, and A.J. Stentz, �??Visible continuum generation in air-silica microstructure optical fibers with anomalous dispersion at 800 nm,�?? Opt. Lett. 25, 25-27 (2000). [CrossRef]
  9. W.J. Wadsworth, A. Ortigosa-Blanch, J.C. Knight, T.A. Birks, T.P.M. Mann, and P.St.J. Russell, �??Supercontinuum generation in photonic crystal fibers and optical fiber tapers: a novel light source,�?? J. Opt. Soc. Am. B 19, 2148-2155 (2002). [CrossRef]
  10. D.J. Jones, S.A. Diddams, J.K. Ranka, A. Stentz, R.S. Windeler, J.L. Hall, and S.T. Cundiff, �??Carrier-envelope phase control of femtosecond mode-locked lasers and direct optical frequency synthesis,�?? Science, 288, 635-639 (2000). [CrossRef] [PubMed]
  11. R. Holzwarth, T. Udem, T.W. Hänsch, J.C. Knight, W.J. Wadsworth, and P.St.J. Russell, �??Optical frequency synthesizer for precision spectroscopy,�?? Phys. Rev. Lett. 85, 2264-2267 (2000). [CrossRef] [PubMed]
  12. A. Baltuska, T. Fuji, and T. Kobayashi, �??Self-referencing of the carrier-envelope slip in a 6-fs visible parametric amplifier,�?? Opt. Lett. 27, 1241-1243 (2002). [CrossRef]
  13. A.B. Fedotov, Ping Zhou, A.P. Tarasevitch, K.V. Dukel�??skii, Yu.N. Kondrat�??ev, V.S. Shevandin, V.B. Smirnov, D. von der Linde, and A.M. Zheltikov, J. Raman Spectrosc. �??Microstructure-Fiber Sources of Mode-Separable Supercontinuum Emission for Wave-Mixing Spectroscopy,�?? 33, 888-896 (2002). [CrossRef]
  14. I. Hartl, X. D. Li, C. Chudoba, R.K. Rhanta, T.H. Ko, J.G. Fujimoto, J.K. Ranka, and R.S. Windeler, �??Ultrahigh-resolution optical coherence tomography using continuum generation in an air-silica microstructure optical fiber,�?? Opt. Lett. 26, 608-610 (2001). [CrossRef]
  15. A.N. Naumov, A.B. Fedotov, A.M. Zheltikov, V.V. Yakovlev, L.A. Mel'nikov, V.I. Beloglazov, N.B. Skibina, and A.V. Shcherbakov, �??Enhanced �?(3) interactions of unamplified femtosecond Cr: forsterite laser pulses in photonic-crystal fibers,�?? J. Opt. Soc. Am. B 19, 2183-2191 (2002). [CrossRef]
  16. S. Coen, A. Hing Lun Chau, R. Leonhardt, J.D. Harvey, J.C. Knight, W.J. Wadsworth, and P.St.J. Russell, �??Supercontinuum generation by stimulated Raman scattering and parametric four-wave mixing in photonic crystal fibers,�?? J. Opt. Soc. Am. B 19, 753-764 (2002). [CrossRef]
  17. A. Efimov, A.J. Taylor, F.G. Omenetto, J.C. Knight, W.J. Wadsworth, and P.St.J. Russell, �??Nonlinear generation of very high-order UV modes in microstructured fibers,�?? Opt. Express 11, 910-918 (2003), <a href= �??http://www.opticsexpress.org/abstract.cfm?URI=OPEX-11-8-910.">http://www.opticsexpress.org/abstract.cfm?URI=OPEX-11-8-910</a>. [CrossRef] [PubMed]
  18. A.B. Fedotov, I. Bugar, D.A. Sidorov-Biryukov, E.E. Serebryannikov, D. Chorvat Jr., M. Scalora, D. Chorvat, and A.M. Zheltikov, �??Pump-depleting four-wave mixing in supercontinuum-generating microstructure fibers,�?? Appl. Phys. B 77, no. 1/2 (2003). [CrossRef]
  19. H. Dürr and H. Bouas-Laurent (Eds.), Photochromism: Molecules and Systems (Elsevier, Amsterdam, 1990).
  20. D.A. Parthenopoulos and P.M. Rentzepis, �??Three-dimensional optical storage memory,�?? Science 245, 843-845 (1989). [CrossRef] [PubMed]
  21. D.A. Akimov, N.I. Koroteev, S.A. Magnitskii, A.N. Naumov, D.A. Sidorov-Biryukov, A.B. Fedotov, and A.M. Zheltikov, �??Optimizing two-photon three-dimensional data storage in photochromic materials using the principles of nonlinear optics,�?? Jpn. J. Appl. Phys. 36, 426-428 (1997). [CrossRef]
  22. S. Lecomte, U. Gubler, M. Jäger, Ch. Bosshard, G. Montemezzani, P. Günter, L. Gobbi, and F. Diederich, �??Reversible optical structuring of polymer waveguides doped with photochromic molecules,�?? Appl. Phys. Lett. 77, 921-923 (2000). [CrossRef]
  23. S.O. Konorov, A.B. Fedotov, and A.M. Zheltikov, �??Three-dimensional reversible laser micromachining with subnanojoule femtosecond pulses based on two-photon photochromism,�?? Appl. Phys. B 76, 707-710 (2003). [CrossRef]
  24. I. Willner, �??Photoswitchable biomaterials: en route to optobioelectronic systems,�?? Acc. Chem. Res. 30, 347-356 (1997). [CrossRef]

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