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Optics Express

Optics Express

  • Editor: Michael Duncan
  • Vol. 13, Iss. 10 — May. 16, 2005
  • pp: 3619–3624

Photoresponsive polymers for topographic simulation of the optical near-field of a nanometer sized gold tip in a highly focused laser beam

Yann Gilbert, Renaud Bachelot, Alexandre Vial, Gilles Lerondel, Pascal Royer, Alexandre Bouhelier, and Gary P. Wiederrecht  »View Author Affiliations


Optics Express, Vol. 13, Issue 10, pp. 3619-3624 (2005)
http://dx.doi.org/10.1364/OPEX.13.003619


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Abstract

The local perturbation of a diffraction-limited spot by a nanometer sized gold tip in a popular apertureless scanning near-field optical microscopy (ASNOM) configuration is reproduced through topography changes in a photoresponsive polymer. Our method relies on the observation of the photochemical migration of azobenzene molecules grafted to a polymer placed beneath the tip. A local molecular displacement has been shown to be activated by a gold tip as a consequence of the lateral surface charge density present at the edges of the tip’s end, resulting from a strong near-field depolarization predicted by theory.

© 2005 Optical Society of America

OCIS Codes
(180.5810) Microscopy : Scanning microscopy
(260.2110) Physical optics : Electromagnetic optics
(310.6860) Thin films : Thin films, optical properties

ToC Category:
Research Papers

History
Original Manuscript: March 21, 2005
Revised Manuscript: April 29, 2005
Published: May 16, 2005

Citation
Yann Gilbert, Renaud Bachelot, Alexandre Vial, Gilles Lerondel, Pascal Royer, Alexandre Bouhelier, and Gary Wiederrecht, "Photoresponsive polymers for topographic simulation of the optical near-field of a nanometer sized gold tip in a highly focused laser beam," Opt. Express 13, 3619-3624 (2005)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-13-10-3619


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