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Optics Express

Optics Express

  • Editor: Michael Duncan
  • Vol. 13, Iss. 10 — May. 16, 2005
  • pp: 3697–3706

Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode

Wolfgang Wagner, Chunqiang Li, John Semmlow, and Warren S. Warren  »View Author Affiliations


Optics Express, Vol. 13, Issue 10, pp. 3697-3706 (2005)
http://dx.doi.org/10.1364/OPEX.13.003697


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Abstract

Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented.

© 2004 Optical Society of America

OCIS Codes
(320.5540) Ultrafast optics : Pulse shaping
(320.7150) Ultrafast optics : Ultrafast spectroscopy

ToC Category:
Research Papers

History
Original Manuscript: January 4, 2005
Revised Manuscript: April 15, 2005
Published: May 16, 2005

Citation
Wolfgang Wagner, Chunqiang Li, John Semmlow, and Warren Warren, "Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode," Opt. Express 13, 3697-3706 (2005)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-13-10-3697


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