Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode

doi:10.1364/OPEX.13.003697

Optics Express

Editor: Michael Duncan
Vol. 13, Iss. 10 — May. 16, 2005
pp: 3697–3706

Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode

Wolfgang Wagner, Chunqiang Li, John Semmlow, and Warren Warren »View Author Affiliations

Optics Express, Vol. 13, Issue 10, pp. 3697-3706 (2005)
http://dx.doi.org/10.1364/OPEX.13.003697

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Abstract
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Abstract

Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented.

OCIS Codes
(320.5540) Ultrafast optics : Pulse shaping
(320.7150) Ultrafast optics : Ultrafast spectroscopy

ToC Category:
Research Papers

History
Original Manuscript: January 4, 2005
Revised Manuscript: April 15, 2005
Published: May 16, 2005

Citation
Wolfgang Wagner, Chunqiang Li, John Semmlow, and Warren Warren, "Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode," Opt. Express 13, 3697-3706 (2005)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-13-10-3697

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References

E.L. Hahn, �??Nuclear induction due to free Larmor precession,�?? Phys. Rev. 77, 297-300 (1950). [CrossRef]
W.P. Aue, E. Bartholdi, and R.R. Ernst, �??Two-dimensional spectroscopy. Applications to nuclear magnetic resonance,�?? J. Opt. Soc. Am. B 64, 2229 (1976).
David M. Jonas, �??Two-Dimensional Femtosecond Spectroscopy,�?? Ann. Rev. Phys. Chem. 54, 425-463 (2003). [CrossRef]
M.C. Asplund, M.T. Zanni, and R.M. Hochstrasser �??Two-Dimensional Femtosecond Spectroscopy,�?? Proc. Natl. Acad. Sci. U.S.A. 97, 8219-8224 (2000). [CrossRef] [PubMed]
O. Golonzka, M. Khalil, N. Demirdoven, and A. Tokmakoff, �??Vibrational Anharmonicities Revealed by Coherent Two-Dimensional Infrared Spectroscopy,�?? Phys. Rev. Lett. 86 No. 10, 2154-2157 (2001). [CrossRef] [PubMed]
T. Elsaesser, J.G. Fujimoto, D.A. Wiersma, and W. Zinth, Ultrafast Phenomena XI Springer Verlab, 1998. [CrossRef]
P. Tian, D. Keusters, S. Yoshifumi, and W.S. Warren, �??Femtosecond Phase-Coherent Two-Dimensional Spectroscopy,�?? Science 300, 1553-1555 (2003). [CrossRef] [PubMed]
D. Keusters, H. Tan, and W.S. Warren, �??Role of Pulse Phase and Direction in Two-Dimensional Optical Spectroscopy,�?? J. Phys. Chem. A 103, 10369-10380 (1999). [CrossRef]
W.Yang, D.Keusters, D.Goswami, and W.S.Warren, �??Rapid ultrafine-tunable optical delay line at the 1.55-µm wavelength,�?? Optics Letters 23, 1843-1845 (1998). [CrossRef]
A.M. Weiner, J.P. Heritage, and E.M. Kirschner, �??High-resolution femtosecond pulse shaping,�?? J. Opt. Soc. Am. B 5, 1563-1572 (1988). [CrossRef]
S. Mukamel, �??Multidimensional Femtosecond Correlation Spectroscopies of Electronic and Vibrational Excitations,�?? Ann. Rev. Phys. Chem. 51, 691-729 (2000). [CrossRef]
J.D. Hybl, A.W. Albrecht, S.M. Gallagher-Faeder, and D.M. Jonas,�??Two-dimensional electronic spectroscopy,�?? Chem. Phys. Lett. 297, 307-313 (1998). [CrossRef]
S. Woutersen and P. Hamm,�??Nonlinear two-dimensional vibrational spectroscopy of peptides,�?? J. Phys. Cond. Matt. 14, R1035-1062 (2002). [CrossRef]
L. Cowan , J. P. Ogilvie and R. J. D. Miller,�??Two-dimensional spectroscopy using diffractive optics based phased-locked photon echoes,�?? Chem. Phys. Lett. 386, 184-189 (2004). [CrossRef]
L, Allen and J.H. Eberly, Optical Resonance and Two Level Atoms Dover Publications, 1987.
S. Mukamel, Principles of Nonlinear Optical Spectroscopy Oxford Series in Optical and Imaging Sciences, 1995.
R.W. Boyd, Nonlinear Optics Academic Press, 1992.
H.S. Tan, Generation, Measurement and Applications of Amplified Visitble, Near Infrared, And Mid Infrared Shaped Ultrashort Pulses, PhD Thesis, Princeton University, 2003. [PubMed]

Ann. Rev. Phys. Chem.

David M. Jonas, �??Two-Dimensional Femtosecond Spectroscopy,�?? Ann. Rev. Phys. Chem. 54, 425-463 (2003). [CrossRef]
S. Mukamel, �??Multidimensional Femtosecond Correlation Spectroscopies of Electronic and Vibrational Excitations,�?? Ann. Rev. Phys. Chem. 51, 691-729 (2000). [CrossRef]

Chem. Phys. Lett.

J.D. Hybl, A.W. Albrecht, S.M. Gallagher-Faeder, and D.M. Jonas,�??Two-dimensional electronic spectroscopy,�?? Chem. Phys. Lett. 297, 307-313 (1998). [CrossRef]
L. Cowan , J. P. Ogilvie and R. J. D. Miller,�??Two-dimensional spectroscopy using diffractive optics based phased-locked photon echoes,�?? Chem. Phys. Lett. 386, 184-189 (2004). [CrossRef]

J. Opt. Soc. Am. B

A.M. Weiner, J.P. Heritage, and E.M. Kirschner, �??High-resolution femtosecond pulse shaping,�?? J. Opt. Soc. Am. B 5, 1563-1572 (1988). [CrossRef]
W.P. Aue, E. Bartholdi, and R.R. Ernst, �??Two-dimensional spectroscopy. Applications to nuclear magnetic resonance,�?? J. Opt. Soc. Am. B 64, 2229 (1976).

J. Phys. Chem. A

D. Keusters, H. Tan, and W.S. Warren, �??Role of Pulse Phase and Direction in Two-Dimensional Optical Spectroscopy,�?? J. Phys. Chem. A 103, 10369-10380 (1999). [CrossRef]

J. Phys. Cond. Matt.

S. Woutersen and P. Hamm,�??Nonlinear two-dimensional vibrational spectroscopy of peptides,�?? J. Phys. Cond. Matt. 14, R1035-1062 (2002). [CrossRef]

Optics Letters

W.Yang, D.Keusters, D.Goswami, and W.S.Warren, �??Rapid ultrafine-tunable optical delay line at the 1.55-µm wavelength,�?? Optics Letters 23, 1843-1845 (1998). [CrossRef]

Phys. Rev.

E.L. Hahn, �??Nuclear induction due to free Larmor precession,�?? Phys. Rev. 77, 297-300 (1950). [CrossRef]

Phys. Rev. Lett.

O. Golonzka, M. Khalil, N. Demirdoven, and A. Tokmakoff, �??Vibrational Anharmonicities Revealed by Coherent Two-Dimensional Infrared Spectroscopy,�?? Phys. Rev. Lett. 86 No. 10, 2154-2157 (2001). [CrossRef] [PubMed]

Proc. Natl. Acad. Sci. U.S.A.

M.C. Asplund, M.T. Zanni, and R.M. Hochstrasser �??Two-Dimensional Femtosecond Spectroscopy,�?? Proc. Natl. Acad. Sci. U.S.A. 97, 8219-8224 (2000). [CrossRef] [PubMed]

Science

P. Tian, D. Keusters, S. Yoshifumi, and W.S. Warren, �??Femtosecond Phase-Coherent Two-Dimensional Spectroscopy,�?? Science 300, 1553-1555 (2003). [CrossRef] [PubMed]

Other

L, Allen and J.H. Eberly, Optical Resonance and Two Level Atoms Dover Publications, 1987.
S. Mukamel, Principles of Nonlinear Optical Spectroscopy Oxford Series in Optical and Imaging Sciences, 1995.
R.W. Boyd, Nonlinear Optics Academic Press, 1992.
H.S. Tan, Generation, Measurement and Applications of Amplified Visitble, Near Infrared, And Mid Infrared Shaped Ultrashort Pulses, PhD Thesis, Princeton University, 2003. [PubMed]
T. Elsaesser, J.G. Fujimoto, D.A. Wiersma, and W. Zinth, Ultrafast Phenomena XI Springer Verlab, 1998. [CrossRef]

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