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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 16, Iss. 11 — May. 26, 2008
  • pp: 7832–7841

Fabrication of spatial modulated second order nonlinear structures and quasi-phase matched second harmonic generation in a poled azo-copolymer planar waveguide

Jian Hung Lin, Ngoc Diep Lai, Chau Han Chiu, Chi-Yuan Lin, Georg W. Rieger, Jeff F. Young, Forest Shih-Sen Chien, and Chia Chen Hsu  »View Author Affiliations


Optics Express, Vol. 16, Issue 11, pp. 7832-7841 (2008)
http://dx.doi.org/10.1364/OE.16.007832


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Abstract

This work demonstrates that arbitrary types of spatially modulated second-order susceptibility (χ(2)) structures such as 1D and 2D, periodic and quasi-periodic structures can be obtained by using the combination of corona poling and direct laser writing (DLW) techniques. The fabrication technique is based on the photodepoling of azo-dye molecules caused by one-photon or two-photon absorption during the DLW process. Polarization and second harmonic generation (SHG) images of the fabricated structures were measured by electrostatic force microscope and SHG mapping techniques, respectively. Furthermore, quasi-phase-matched (QPM) enhanced SHG from a 1D periodically poled azo-copolymer planar waveguide is demonstrated using an optical parametric oscillator laser by scanning wavelength from 1500 to 1600 nm. The resonant wavelength of the QPM enhanced SHG is peaked at 1537 nm with FWHM≅2.5nm.

© 2008 Optical Society of America

OCIS Codes
(190.2620) Nonlinear optics : Harmonic generation and mixing
(190.4710) Nonlinear optics : Optical nonlinearities in organic materials
(230.4320) Optical devices : Nonlinear optical devices

ToC Category:
Nonlinear Optics

History
Original Manuscript: March 25, 2008
Revised Manuscript: May 5, 2008
Manuscript Accepted: May 6, 2008
Published: May 15, 2008

Citation
Jian Hung Lin, Ngoc Diep Lai, Chau Han Chiu, Chi-Yuan Lin, Georg W. Rieger, Jeff F. Young, Forest Shih-Sen Chien, and Chia Chen Hsu, "Fabrication of spatial modulated second order nonlinear structures and quasi-phase matched second harmonic generation in a poled azo-copolymer planar waveguide," Opt. Express 16, 7832-7841 (2008)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-16-11-7832


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References

  1. Z. Sekkat and W. Knoll, Photoreactive Organic Thin Films (Academic Press, USA, 2002).
  2. P. Prasad and D. J. Williams, Introduction to Nonlinear Optical Effects in Molecules and Polymers (John Wiley & Sons, USA, 1991).
  3. D. S. Chemla and J. Zyss, Nonlinear Optical Properties of Organic Molecules and Crystals (Academic Press, USA, 1987).
  4. J. Zyss, Molecular Nonlinear Optics Materials, Physics, and Devices (Academic Press, USA, 1994).
  5. J. A. Armstrong, N. Bloembergen, J. Ducuing, and P. S. Pershan, "Interactions between light waves in a nonlinear dielectric," Phys. Rev. 127, 1918-1939 (1962). [CrossRef]
  6. G. Kanarian, R. A. Norwood, D. Haas, B. Feuer, and D. Karim, "Phase-matched second-harmonic generation in a polymer waveguides," Appl. Phys. Lett. 57, 977-979 (1990). [CrossRef]
  7. Y. Shuto, T. Watanabe, S. Tomaru, I. Yokohama, M. Hikita, and M. Amano, "Quasi-phase-matched second-harmonic generation in diazo-dye-substituted polymer channel waveguides," IEEE J. Quantum Electron. 33, 349-357 (1997). [CrossRef]
  8. M. Jager, G. I. Stegeman, W. Brinker, S. Yilmaz, S. Bauer, W. H. G. Horsthuis, and G. R. Mohlmann, "Comparison of quasi-phase-matching geometries for second-harmonic generation in poled polymer channel waveguides at 1.5 μm," Appl. Phys. Lett. 68, 1183-1185 (1996). [CrossRef]
  9. S. Tomaru, T. Watanabe, M. Hikita, M. Amano, Y. Shuto, I. Yokohoma, T. Kaino, and M. Asobe, "Quasi-phase-mateched second harmonic generation in a polymer waveguide with a periodic poled structure," Appl. Phys. Lett. 68, 1760-1762 (1996). [CrossRef]
  10. G. Martin, S. Ducci, R. Hierle, D. Josse, and J. Zyss, "Quasiphase matched second-harmonic generation from periodic optical randomization of poled polymer channel waveguides," Appl. Phys. Lett. 83, 1086-1088 (2003). [CrossRef]
  11. J. J. Ju, J. Kim, J. Y. Do, M.-S. Kim, S. K. Park, S. Park, and M.-H. Lee, "Second-harmonic generation in periodically poled nonlinear polymer waveguides," Opt. Lett. 29, 89-91 (2004). [CrossRef] [PubMed]
  12. G. L. J. A. Rikken, C. J. E. Seppen, S. Nijhuis, and E. W. Meijer, "Poled polymers for frequency doubling of diode lasers," Appl. Phys. Lett. 58, 435-437 (1991). [CrossRef]
  13. O. Sugihara, Y. Che, N. Okamoto, H. Fujimura, C. Egami, and S. Umegaki, "High-resolution periodically poled structure in diazo-dye-substituted polymer film based on direct electron-beam writing technique," Appl. Phys. Lett. 73, 3028-3030 (1998). [CrossRef]
  14. O. Sugihara, M. Nakanishi, Y. Che, C. Egami, Y. Kawata, and N. Okamoto, "Single-pulse ultraviolet laser recording of periodically poled structures in polymer thin films," Appl. Opt. 39, 5632-5637 (2000). [CrossRef]
  15. X. Ni, M. Nakanishi, O. Sugihara, and N. Okamato, "Fabrication of ?(2) grating in poled polymer waveguide based on direct laser beam writing," Opt. Rev. 5, 9-11 (1998). [CrossRef]
  16. H. Ishitobi, Z. Sekkat, and S. Kawata, "Photo-orientation by multiphoton photonselection," J. Opt. Soc. Am. B 23, 868-872 (2006). [CrossRef]
  17. H. Ishitobi, Z. Sekkat, and S. Kawata, "Ordering of azobenzens by two-photon isomerization," J. Chem. Phys. 125, 164718-164718-4 (2006). [CrossRef] [PubMed]
  18. D. Gindre, A. Boeglin, A. Fort, L. Marger, and K. D. Dorkenoo, "Rewritable optical data storage in azobenzene copolymers," Opt. Express 14, 9896-9901 (2006). [CrossRef] [PubMed]
  19. M. Maeda, H. Ishitobi, Z. Sekkat, and S. Kawata, "Polarization storage by nonlinear orientational hole burning in azo dye-containing polymer films," Appl. Phys. Lett. 85, 351-353 (2004). [CrossRef]
  20. X. Li, J. W. M. Chon, R. A. Evans, and M. Gu, "Two photon energy transfer enhanced three-dimensional optical memory in quantum-dot and azo-dye doped polymers," Appl. Phys. Lett. 92, 063309-063309-3 (2008). [CrossRef]
  21. Z. Sekkat, J. Wood, E. F. Aust, W. Knoll, W. Volksen, and R. D. Miller, "Light induced orientation in a high glass transition temperature polyimide with polar azo dyes in the side chain," J. Opt. Soc. Am. B 13, 1713-1724 (1996). [CrossRef]
  22. R. Loucif-Saibi, K. Nakatani, J. A. Delaire, M. Dumont, and Z. Sekkat, "Photoisomerization and second harmonic generation in disperse one-doped and functionalized poly(methyl methacrylate) films," Chem. Mater. 5, 229-236 (1993). [CrossRef]
  23. V. M. Churikov and C. C. Hsu, "Optical control of third-harmonic generation in azo-doped polymethylmethacrylate thin films," Appl. Phys. Lett. 77, 2095-2097 (2000). [CrossRef]
  24. S. Bian, L. Li, J. Kumar, D. Y. Kim, J. Williams, and S. K. Tripathy, "Single laser beam-induced surface deformation on azobenzene polymer films," Appl. Phys. Lett. 73, 1817-1819 (1998). [CrossRef]
  25. M. J. Ventura, M. Straub, and M. Gu, "Void channel microstructures in resin solids as an efficient way to infrared photonic crystals," Appl. Phys. Lett. 82, 1649 (2003). [CrossRef]
  26. M. M. Fejer, G. A. Magel, D. H. Jundt, and R. L. Byer, "Quasi-phase-matched second harmonic generation: Tuning and Tolerances," IEEE J. Quantum Electron. 28, 2631-2654 (1992). [CrossRef]
  27. N. D. Lai, J. H. Lin, W. P. Liang, and C. C. Hsu, "Precisely introducing defects into periodic structures by using a double-step laser scanning technique," Appl. Opt. 45, 5777-5782 (2006). [CrossRef] [PubMed]
  28. R. Dianoux, F. Martins, F. Marchi, C. Alandi, F. Comin, and J. Chevrier, "Detection of electrostatic forces with an atomic force microscope: Analytical and experimental dynamic force curves in the nonlinear regime," Phys. Rev. B 68, 045403 (2003). [CrossRef]
  29. H. Ishitobi, M. Tanabe, Z. Sekkat, and S. Kawata, "The anisotropic nanomovement of azo-polymers," Opt. Express 15, 652-659 (2007). [CrossRef] [PubMed]
  30. V. Berger, "Nonlinear photonic crystals," Phys. Rev. Lett. 81, 4136-4139 (1998). [CrossRef]
  31. N.G. R. Broderick, G. W. Ross, H. L. Offerhaus, D. J. Richardson, and D. C. Hanna, "Hexagonal poled lithium niobate: a two dimensional nonlinear photonic crystal," Phys. Rev. Lett. 84, 4345-4347 (2000). [CrossRef] [PubMed]
  32. S. Saltiel and Y. Kivshar, "Phase matching in nonlinear ?(2) photonic crystals," Opt. Lett. 25, 1204-1206 (2000). [CrossRef]
  33. R. Lifshitz, A. Arie, and A. Bahabad, "Photonic quasicrystals for nonlinear optical frequency conversion," Phys. Rev. Lett. 95, 133901-133901-4 (2005). [CrossRef] [PubMed]
  34. R. J. Bratfalean, A. C. Peacock, N. G. R. Broderick, K. G.allon, and R. Lewen, "Harmonic generation in a two-dimensional nonlinear quasi-crystal," Opt. Lett. 30, 424-426 (2005). [CrossRef] [PubMed]
  35. E. Kim, Y.-K. Choi, and M.-H. Lee, "Photoinduced refractive index change of a photochromic diarylethene polymer," Macromolecules,  32, 4855-4860 (1999). [CrossRef]
  36. M. W. McCutcheon, G. W. Rieger, I. W. Cheung, J. F. Young, D. Dalacu, S. Frederick, P. J. Poole, G. C. Aers, and R. L. Williams, "Resonant scattering and second-harmonic spectroscopy of planar photonic crystal microcavities," Appl. Phys. Lett. 87, 221110(1-3) (2005). [CrossRef]

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