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Optics Express

Optics Express

  • Vol. 16, Iss. 16 — Aug. 4, 2008
  • pp: 12139–12147

Broadband coherent light generation in diamond driven by femtosecond pulses

Miaochan Zhi, Xi Wang, and Alexei V. Sokolov  »View Author Affiliations


Optics Express, Vol. 16, Issue 16, pp. 12139-12147 (2008)
http://dx.doi.org/10.1364/OE.16.012139


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Abstract

We demonstrate broadband light generation in diamond pumped by two-color femtosecond laser pulses. We find that phase matching plays a critical role in the output angle and frequency of the generated sidebands. When a third femtosecond probe pulse is applied to the crystal in the boxed Coherent anti-Stokes Raman Scattering geometry, a two-dimensional array of multi-color beams is generated through the Raman, four-wave mixing, and six-wave-mixing processes. We test the mutual coherence between the generated sidebands. Such coherence, maintained over the broad spectrum, opens possibilities for synthesis of subfemtosecond light waveforms.

© 2008 Optical Society of America

OCIS Codes
(190.4720) Nonlinear optics : Optical nonlinearities of condensed matter
(190.5650) Nonlinear optics : Raman effect
(190.5890) Nonlinear optics : Scattering, stimulated
(320.2250) Ultrafast optics : Femtosecond phenomena

ToC Category:
Nonlinear Optics

History
Original Manuscript: May 29, 2008
Revised Manuscript: July 17, 2008
Manuscript Accepted: July 23, 2008
Published: July 29, 2008

Citation
Miaochan Zhi, Xi Wang, and Alexei V. Sokolov, "Broadband coherent light generation in diamond driven by femtosecond pulses," Opt. Express 16, 12139-12147 (2008)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-16-16-12139


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References

  1. A. V. Sokolov and S. E. Harris, "Ultrashort pulse generation by molecular modulation," J. Opt. B. 5, R1 (2003). [CrossRef]
  2. A. V. Sokolov, M. Y. Shverdin, D. R. Walker, D. D. Yavuz, A. M. Burzo, G. Y. Yin, and S. E. Harris, "Generation and control of femtosecond pulses by molecular modulation," J. Mod. Opt. 52, 285 (2005). [CrossRef]
  3. M. Zhi and A. V. Sokolov, "Broadband coherent light generation in a Raman-active crystal driven by two-color femtosecond laser pulses," Opt. Lett. 32, 2251-2253 (2007). [CrossRef] [PubMed]
  4. M. Zhi and A. V. Sokolov, "Broadband generation in a Raman crystal driven by a pair of time-delayed linearly chirped pulses," New J. Phys. 10, 025032 (2008). [CrossRef]
  5. J. Takahashi, "Generatoin of a broadband spectral comb with multiwave mixing by exchange of an impulsively stimulated phonon, " Opt. Express 12, 1185 (2004). [CrossRef] [PubMed]
  6. E. Matsubabra, K. Inoue, and E. Hanamura, "Dynamical symmetry breaking induced by ultrashort laser pulses in KTaO3," J. Phys. Soc. Jpn. 75, 024712 (2006). [CrossRef]
  7. H. Matsuki, K. Inoue, and E. Hanamura, "Multiple coherent anti-Stokes Raman scattering due to phonon grating in KNbO3 induced by crossed beams of two-color femtosecond pulses," Phys. Rev. B 75, 024102 (2007). [CrossRef]
  8. E. Matsubara, T. Sekikawa, and M. Yamashita, "Generation of ultrashort optical pulses using multiple coherent anti-Stokes Raman scattering in a crystal at room temperature," Appl. Phys. Lett. 92, 071104 (2008). [CrossRef]
  9. T. T. Basiev, A. A. Sobol, P. G. Zverev, V. V. Osiko, and R. C. Powell, "Comparative spontaneous Raman spectroscopy of crystals for Raman lasers," Appl. Opt. 38, 594-598 (1999). [CrossRef]
  10. H. O. Piersonf, Handbook of Carbon Graphite, Diamond and Fullerenes: Properties, Processing, and Applications (Noyes Publications, 1993).
  11. G. Eckhardt, D. P. Bortfeld, and M. Geller, "Stimulated Emission of Stokes AND Anti-Stokes Raman Lines from Diamond, Calcite, and Alpha-sulfur Single Crystals," Appl. Phys. Lett. 3, 137-138 (1963). [CrossRef]
  12. A. A. Kaminskii, V. G. Ralchenko, V. I. Konov, and H. J. Eichler, "High-order Stokes and anti-Stokes Raman generation in CVD diamond, " Phys. Status Solidi (B) 242, R4 (2005). [CrossRef]
  13. A. A. Kaminskii, V. G. Ralchenko, and V. I. Konov, "CVD-diamond - a novel |3-nonlinear active crystalline material for SRS generation in very wide spectral range," Laser Phys. Lett. 3, 171 (2006). [CrossRef]
  14. D. Y. Smith, M. Inokuti, and W. Karstens, "A generalized Cauchy dispersion formula and the refractivity of elemental semiconductors," J. Phys. : Condens. Matter 13, 3883 (2001). [CrossRef]
  15. D. F. Edwards and E. Ochoa, "Infrared refractive index of diamond," J. Opt. Soc. Am. 71, 607-608 (1981). [CrossRef]

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