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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 16, Iss. 22 — Oct. 27, 2008
  • pp: 17654–17666

Fluorescence relaxation in the near-field of a mesoscopic metallic particle: distance dependence and role of plasmon modes

G. Colas des Francs, A. Bouhelier, E. Finot, J. C. Weeber, A. Dereux, C. Girard, and E. Dujardin  »View Author Affiliations


Optics Express, Vol. 16, Issue 22, pp. 17654-17666 (2008)
http://dx.doi.org/10.1364/OE.16.017654


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Abstract

We analytically and numerically analyze the fluorescence decay rate of a quantum emitter placed in the vicinity of a spherical metallic particle of mesoscopic size (i.e with dimensions comparable to the emission wavelength). We discuss the efficiency of the radiative decay rate and non-radiative coupling to the particle as well as their distance dependence. The electromagnetic coupling mechanisms between the emitter and the particle are investigated by analyzing the role of the plasmon modes and their nature (dipole, multipole or interface mode). We demonstrate that near-field coupling can be expressed in a simple form verifying the optical theorem for each particle modes.

© 2008 Optical Society of America

OCIS Codes
(240.6680) Optics at surfaces : Surface plasmons
(260.2160) Physical optics : Energy transfer
(260.2510) Physical optics : Fluorescence

ToC Category:
Physical Optics

History
Original Manuscript: July 1, 2008
Revised Manuscript: August 22, 2008
Manuscript Accepted: August 24, 2008
Published: October 17, 2008

Citation
G. Colas des Francs, A. Bouhelier, E. Finot, J. C. Weeber, A. Dereux, C. Girard, and E. Dujardin, "Fluorescence relaxation in the near–field of a mesoscopic metallic particle: distance dependence and role of plasmon modes," Opt. Express 16, 17654-17666 (2008)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-16-22-17654


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