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Lasing from InGaP quantum dots in a spin-coated flexible microcavity
V. M. Menon, M. Luberto, N. V. Valappil, and S. Chatterjee »View Author Affiliations
1Laboratory for Nano and Micro Photonics, Department of Physics, Queens College of the City University of New York (CUNY), Flushing, NY 11367
2Graduate Center of the City University of New York, New York, NY 10016
*Corresponding author: vmenon@qc.cuny.edu
Optics Express, Vol. 16, Issue 24, pp. 19535-19540 (2008)
http://dx.doi.org/10.1364/OE.16.019535
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Abstract
We report the realization of a mechanically flexible microcavity laser emitting at 657 nm using spin coating. These optically pumped vertical cavity surface emitting lasers use InGaP colloidal quantum dots as the active medium and alternating polymer layers of different refractive indices as the Bragg mirrors. Results of photoluminescence measurements indicating enhancement in spontaneous emission are presented. We also demonstrate the possibility of peeling the device off the substrate yielding a flexible structure that can conform to any shape and whose emission spectra can be mechanically tuned. This new class of hybrid lasers combines advantages of organic and inorganic materials.
© 2008 Optical Society of America
OCIS Codes
(140.3948) Lasers and laser optics : Microcavity devices
(140.7270) Lasers and laser optics : Vertical emitting lasers
(250.5590) Optoelectronics : Quantum-well, -wire and -dot devices
ToC Category:
Lasers and Laser Optics
History
Original Manuscript: September 15, 2008
Revised Manuscript: November 7, 2008
Manuscript Accepted: November 7, 2008
Published: November 11, 2008
Citation
V. M. Menon, M. Luberto, N. V. Valappil, and S. Chatterjee, "Lasing from InGaP quantum dots in a
spin-coated flexible microcavity," Opt. Express 16, 19535-19540 (2008)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-16-24-19535
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References
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- M. Kahl, T. Thomay, V. Kohnle, K. Beha, J. Merlein, M. Hagner, A. Halm, J. Ziegler, T. Nann, Y. Fedutik, U. Woggon, M. Artemyev, F. P-Willard, A. Leitenstorfer, and R. Bratschitsch, "Colloidal quantum dots in all-dielectric high-Q pillar microcavities," Nano. Lett. 7, 2897-2900 (2007). [CrossRef] [PubMed]
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- L. Persano, P. D. Carro, E. Mele, R. Cingolani, D. Pisignano, M. Z-Rossi, S. Longhi, G. Lanzani, "Monolithic polymer microcavity lasers with on-top evaporated dielectric mirrors," Appl. Phys. Lett. 88, 121110 (2006). [CrossRef]
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- R. Bose, X. Yang, R. Chatterjee, J. Gao, and C. Wong, "Weak coupling interactions of colloidal lead sulphide nanocrystals with silicon photonic crystal nanocavities near 1.55 µm at room temperature," Appl. Phys. Lett. 90, 111117 (2007). [CrossRef]
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- L. Persano, P. D. Carro, E. Mele, R. Cingolani, D. Pisignano, M. Z-Rossi, S. Longhi, G. Lanzani, "Monolithic polymer microcavity lasers with on-top evaporated dielectric mirrors," Appl. Phys. Lett. 88, 121110 (2006). [CrossRef]
- N. V. Valappil, M. Luberto, V. M. Menon, I. Zeylikovich, T. K. Gayen, J. Franco, B. B. Das, and R. R. Alfano, "Solution processed microcavity structures with embedded quantum dots," Photon. Nanostruct. 5, 184-188 (2007). [CrossRef]
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- V. C. Sundar, H.-J. Eisler, T. Deng, Y. Chan, E. L. Thomas, and M. G. Bawendi, "Soft-lithographically embossed, multilayered distributed-feedback nanocrystal lasers," Adv. Mater. 16, 2137-2141 (2004). [CrossRef]
- N. Tessler, G. J. Denton, and R. H. Friend, "Lasing from conjugated polymer microcavities," Nature 382, 695-697 (1996). [CrossRef]
- A. C. Edrington, A. M. Urbas, P. DeRege, C. X. Chen, T. M. Swager, N. Hadjichristidis, M. Xenidou, L. J. Fetters, J. D. Jounnopoulos, Y. Fink, and E. L. Thomas, "Polymer based photonic crystals," Adv. Mater. 13, 421-425 (2001). [CrossRef]
- M. Reufer, S. Reichel, J. M. Lupton, J. Feldmann, U. Lemmer, D. Schneider, T. Benstem, T. Dobbertin, W. Kowalsky, A. Gombert, K. Forberich, V. Wittwer, and U. Scherf, "Low threshold distributed feedback lasers with metallic contacts," Appl. Phys. Lett. 84, 3262-3264 (2004). [CrossRef]
- M. Meier, A. Mekis, A. Dodabalapur, A. Timko, R. E. Slusher, J. D. Joannopoulos, and O. Nalamasu, "Laser action from two-dimensional distributed feedback in photonic crystals," Appl. Phys. Lett. 74, 7-9 (1999) [CrossRef]
- M. Kuwata-Gonokami, R. H. Jordan, A. Dodabalapur, H. E. Katz, M. L. Schilling, R. E. Slusher, and S. Ozawa, "Polymer microdisk and microring lasers," Opt. Lett. 20, 2093-2095 (1995). [CrossRef] [PubMed]
- C. Poitras, M. Lipson, H. Du, M. Hahn, and T. Krauss, "Photoluminescence enhancement of colloidal quantum dots embedded in a monolithic microcavity," Appl. Phys. Lett. 82, 4032-4034 (2003). [CrossRef]
- A. C. Edrington, A. M. Urbas, P. DeRege, C. X. Chen, T. M. Swager, N. Hadjichristidis, M. Xenidou, L. J. Fetters, J. D. Jounnopoulos, Y. Fink, and E. L. Thomas, "Polymer based photonic crystals," Adv. Mater. 13, 421-425 (2001). [CrossRef]
- H. Eisler, V. C. Sundar, M. G. Bawendi, M. Walsh, H. I. Smith, and V. Klimov, "Color selective semiconductor nanocrystal laser," Appl. Phys. Lett. 80, 4614-4616 (2002). [CrossRef]
- V. C. Sundar, H.-J. Eisler, T. Deng, Y. Chan, E. L. Thomas, and M. G. Bawendi, "Soft-lithographically embossed, multilayered distributed-feedback nanocrystal lasers," Adv. Mater. 16, 2137-2141 (2004). [CrossRef]
- I. Fushman, D. Englund, and J. Vučković, "Coupling of PbS quantum dots to photonic crystal cavities at room temperature," Appl. Phys. Lett. 87, 241102 (2005). [CrossRef]
- M. Kahl, T. Thomay, V. Kohnle, K. Beha, J. Merlein, M. Hagner, A. Halm, J. Ziegler, T. Nann, Y. Fedutik, U. Woggon, M. Artemyev, F. P-Willard, A. Leitenstorfer, and R. Bratschitsch, "Colloidal quantum dots in all-dielectric high-Q pillar microcavities," Nano. Lett. 7, 2897-2900 (2007). [CrossRef] [PubMed]
- M. Reufer, S. Reichel, J. M. Lupton, J. Feldmann, U. Lemmer, D. Schneider, T. Benstem, T. Dobbertin, W. Kowalsky, A. Gombert, K. Forberich, V. Wittwer, and U. Scherf, "Low threshold distributed feedback lasers with metallic contacts," Appl. Phys. Lett. 84, 3262-3264 (2004). [CrossRef]
- S. Riechel, C. Kallinger, U. Lemmer, J. Feldmann, A. Gombert, V. Wittwer, and U. Scherf, "A nearly diffraction limited surface emitting conjugated polymer laser utilizing a two-dimensional photonic band structure," Appl. Phys. Lett. 77, 2310-2312 (2000). [CrossRef]
- A. C. Edrington, A. M. Urbas, P. DeRege, C. X. Chen, T. M. Swager, N. Hadjichristidis, M. Xenidou, L. J. Fetters, J. D. Jounnopoulos, Y. Fink, and E. L. Thomas, "Polymer based photonic crystals," Adv. Mater. 13, 421-425 (2001). [CrossRef]
- A. C. Edrington, A. M. Urbas, P. DeRege, C. X. Chen, T. M. Swager, N. Hadjichristidis, M. Xenidou, L. J. Fetters, J. D. Jounnopoulos, Y. Fink, and E. L. Thomas, "Polymer based photonic crystals," Adv. Mater. 13, 421-425 (2001). [CrossRef]
- C. Finlayson, D. Ginger, and N. Greenham, "Optical microcavities using highly luminescent films of semiconductor nanocrystals," Appl. Phys. Lett. 77, 2500-2502 (2000). [CrossRef]
- P. Lodahl, A. Floris van Driel, I. S. Nikolaev, A. Irman, K. Overgaag, D. Vanmaekelbergh, and W. L. Vos, "Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals," Nature 430, 654-657 (2004) [CrossRef] [PubMed]
- M. Reufer, S. Reichel, J. M. Lupton, J. Feldmann, U. Lemmer, D. Schneider, T. Benstem, T. Dobbertin, W. Kowalsky, A. Gombert, K. Forberich, V. Wittwer, and U. Scherf, "Low threshold distributed feedback lasers with metallic contacts," Appl. Phys. Lett. 84, 3262-3264 (2004). [CrossRef]
- J. Lawrence, Y. Ying, P. Jiang, and S. Foulger, "Dynamic tuning of organic lasers with colloidal crystals," Adv. Mater. 18, 300-303 (2006). [CrossRef]
- N. V. Valappil, M. Luberto, V. M. Menon, I. Zeylikovich, T. K. Gayen, J. Franco, B. B. Das, and R. R. Alfano, "Solution processed microcavity structures with embedded quantum dots," Photon. Nanostruct. 5, 184-188 (2007). [CrossRef]
- N. Tessler, G. J. Denton, and R. H. Friend, "Lasing from conjugated polymer microcavities," Nature 382, 695-697 (1996). [CrossRef]
- S. Furumi, H. Fudouzi, H. Miyazaki, and Y. Sakka, "Flexible polymer colloidal -crystal lasers with a light-emitting planar defect," Adv. Mater. 19, 2067-2072 (2007). [CrossRef]
- S. Furumi, H. Fudouzi, H. Miyazaki, and Y. Sakka, "Flexible polymer colloidal -crystal lasers with a light-emitting planar defect," Adv. Mater. 19, 2067-2072 (2007). [CrossRef]
- I. Fushman, D. Englund, and J. Vučković, "Coupling of PbS quantum dots to photonic crystal cavities at room temperature," Appl. Phys. Lett. 87, 241102 (2005). [CrossRef]
- R. Bose, X. Yang, R. Chatterjee, J. Gao, and C. Wong, "Weak coupling interactions of colloidal lead sulphide nanocrystals with silicon photonic crystal nanocavities near 1.55 µm at room temperature," Appl. Phys. Lett. 90, 111117 (2007). [CrossRef]
- N. V. Valappil, M. Luberto, V. M. Menon, I. Zeylikovich, T. K. Gayen, J. Franco, B. B. Das, and R. R. Alfano, "Solution processed microcavity structures with embedded quantum dots," Photon. Nanostruct. 5, 184-188 (2007). [CrossRef]
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- N. V. Valappil, M. Luberto, V. M. Menon, I. Zeylikovich, T. K. Gayen, J. Franco, B. B. Das, and R. R. Alfano, "Solution processed microcavity structures with embedded quantum dots," Photon. Nanostruct. 5, 184-188 (2007). [CrossRef]
- P. Lodahl, A. Floris van Driel, I. S. Nikolaev, A. Irman, K. Overgaag, D. Vanmaekelbergh, and W. L. Vos, "Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals," Nature 430, 654-657 (2004) [CrossRef] [PubMed]
- P. Lodahl, A. Floris van Driel, I. S. Nikolaev, A. Irman, K. Overgaag, D. Vanmaekelbergh, and W. L. Vos, "Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals," Nature 430, 654-657 (2004) [CrossRef] [PubMed]
- I. Fushman, D. Englund, and J. Vučković, "Coupling of PbS quantum dots to photonic crystal cavities at room temperature," Appl. Phys. Lett. 87, 241102 (2005). [CrossRef]
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- M. Sandrok, M. Wiggins, J. S. Shirk, H. Tai, A. Ranade, E. Baer, and A. Hiltner, "A widely tunable refractive index in a nanolayered photonic material," Appl. Phys. Lett. 84, 3621-3623 (2004). [CrossRef]
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- Z. Wu, Z. Mi, P. Bhattacharya, T. Zhu, and J. Xu, "Enhanced spontaneous emission at 1.55 µm from colloidal PbSe quantum dots in a Si photonic crystal microcavity," Appl. Phys. Lett. 90, 171105 (2007). [CrossRef]
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- G. Heliotis, R. Xia, D. D. C. Bradley, G. A. Turnbull, I. D. W. Samuel, P. Andrew, and W. L. Barnes, "Blue surface emitting distributed feedback polyfluorene lasers," Appl. Phys. Lett. 83, 2118-2120 (2003). [CrossRef]
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- R. Katouf, T. Komikado, M. Itoh, T. Yatagai, and S. Umegaki, "Ultra-fast optical switches using 1D polymeric photonic crystals," Photon. Nanostruct. 3, 116-119 (2005). [CrossRef]
- J. Lawrence, Y. Ying, P. Jiang, and S. Foulger, "Dynamic tuning of organic lasers with colloidal crystals," Adv. Mater. 18, 300-303 (2006). [CrossRef]
- T. Komikado, S. Yoshida, and S. Umegaki, "Surface-emitting distributed-feedback dye laser of a polymeric multilayer fabricated by spin coating," Appl. Phys. Lett. 89, 061123 (2006). [CrossRef]
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Adv. Mater.
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- S. Furumi, H. Fudouzi, H. Miyazaki, and Y. Sakka, "Flexible polymer colloidal -crystal lasers with a light-emitting planar defect," Adv. Mater. 19, 2067-2072 (2007). [CrossRef]
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Appl. Phys. Lett.
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- T. Komikado, S. Yoshida, and S. Umegaki, "Surface-emitting distributed-feedback dye laser of a polymeric multilayer fabricated by spin coating," Appl. Phys. Lett. 89, 061123 (2006). [CrossRef]
- M. Meier, A. Mekis, A. Dodabalapur, A. Timko, R. E. Slusher, J. D. Joannopoulos, and O. Nalamasu, "Laser action from two-dimensional distributed feedback in photonic crystals," Appl. Phys. Lett. 74, 7-9 (1999) [CrossRef]
- P. Andrew, G. A. Turnbull, I. D. W. Samuel, and W. L. Barnes, "Photonic band structure and emission characteristics of a metal-backed polymeric distributed feedback laser," Appl. Phys. Lett. 81, 954-956 (2002). [CrossRef]
- G. Heliotis, R. Xia, D. D. C. Bradley, G. A. Turnbull, I. D. W. Samuel, P. Andrew, and W. L. Barnes, "Blue surface emitting distributed feedback polyfluorene lasers," Appl. Phys. Lett. 83, 2118-2120 (2003). [CrossRef]
- M. Reufer, S. Reichel, J. M. Lupton, J. Feldmann, U. Lemmer, D. Schneider, T. Benstem, T. Dobbertin, W. Kowalsky, A. Gombert, K. Forberich, V. Wittwer, and U. Scherf, "Low threshold distributed feedback lasers with metallic contacts," Appl. Phys. Lett. 84, 3262-3264 (2004). [CrossRef]
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- L. Persano, P. D. Carro, E. Mele, R. Cingolani, D. Pisignano, M. Z-Rossi, S. Longhi, G. Lanzani, "Monolithic polymer microcavity lasers with on-top evaporated dielectric mirrors," Appl. Phys. Lett. 88, 121110 (2006). [CrossRef]
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- A. V. Malko, A. A. Mikhailovsky, M. A. Petruska, J. A. Hollingsworth, H. Htoon, M. G. Bawendi, and V. I. Klimov, "From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids," Appl. Phys. Lett. 81, 1303-1305 (2002). [CrossRef]
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- I. Fushman, D. Englund, and J. Vučković, "Coupling of PbS quantum dots to photonic crystal cavities at room temperature," Appl. Phys. Lett. 87, 241102 (2005). [CrossRef]
- R. Bose, X. Yang, R. Chatterjee, J. Gao, and C. Wong, "Weak coupling interactions of colloidal lead sulphide nanocrystals with silicon photonic crystal nanocavities near 1.55 µm at room temperature," Appl. Phys. Lett. 90, 111117 (2007). [CrossRef]
- Z. Wu, Z. Mi, P. Bhattacharya, T. Zhu, and J. Xu, "Enhanced spontaneous emission at 1.55 µm from colloidal PbSe quantum dots in a Si photonic crystal microcavity," Appl. Phys. Lett. 90, 171105 (2007). [CrossRef]
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- C. Finlayson, D. Ginger, and N. Greenham, "Optical microcavities using highly luminescent films of semiconductor nanocrystals," Appl. Phys. Lett. 77, 2500-2502 (2000). [CrossRef]
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J. Appl. Phys.
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Jpn. J. Appl. Phys.
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- T. Matsui, M. Ozaki, K. Yoshino, and F. Kajzar, "Fabrication of flexible distributed feedback laser using photoinduced surface relief grating on azo-polymer films as a template," Jpn. J. Appl. Phys. 41, L1386-L1388 (2002). [CrossRef]
Nano. Lett.
- M. Kahl, T. Thomay, V. Kohnle, K. Beha, J. Merlein, M. Hagner, A. Halm, J. Ziegler, T. Nann, Y. Fedutik, U. Woggon, M. Artemyev, F. P-Willard, A. Leitenstorfer, and R. Bratschitsch, "Colloidal quantum dots in all-dielectric high-Q pillar microcavities," Nano. Lett. 7, 2897-2900 (2007). [CrossRef] [PubMed]
Nature
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Opt. Express
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2007, Bose, Appl. Phys. Lett.
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- Z. Wu, Z. Mi, P. Bhattacharya, T. Zhu, and J. Xu, "Enhanced spontaneous emission at 1.55 µm from colloidal PbSe quantum dots in a Si photonic crystal microcavity," Appl. Phys. Lett. 90, 171105 (2007). [CrossRef]
- M. Kahl, T. Thomay, V. Kohnle, K. Beha, J. Merlein, M. Hagner, A. Halm, J. Ziegler, T. Nann, Y. Fedutik, U. Woggon, M. Artemyev, F. P-Willard, A. Leitenstorfer, and R. Bratschitsch, "Colloidal quantum dots in all-dielectric high-Q pillar microcavities," Nano. Lett. 7, 2897-2900 (2007). [CrossRef] [PubMed]
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- J. Lawrence, Y. Ying, P. Jiang, and S. Foulger, "Dynamic tuning of organic lasers with colloidal crystals," Adv. Mater. 18, 300-303 (2006). [CrossRef]
- L. Persano, P. D. Carro, E. Mele, R. Cingolani, D. Pisignano, M. Z-Rossi, S. Longhi, G. Lanzani, "Monolithic polymer microcavity lasers with on-top evaporated dielectric mirrors," Appl. Phys. Lett. 88, 121110 (2006). [CrossRef]
- T. Komikado, S. Yoshida, and S. Umegaki, "Surface-emitting distributed-feedback dye laser of a polymeric multilayer fabricated by spin coating," Appl. Phys. Lett. 89, 061123 (2006). [CrossRef]
- L. Martidadonna, L. Carbone, M. De Giorgi, L. Manna, G. Gigli, R. Cingolani, and M. De Vittorio, "High Q factor colloidal nanocrystal based vertical microcavity by hot embossing," Appl. Phys. Lett. 88, 181108 (2006). [CrossRef]
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- I. Fushman, D. Englund, and J. Vučković, "Coupling of PbS quantum dots to photonic crystal cavities at room temperature," Appl. Phys. Lett. 87, 241102 (2005). [CrossRef]
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- M. Sandrok, M. Wiggins, J. S. Shirk, H. Tai, A. Ranade, E. Baer, and A. Hiltner, "A widely tunable refractive index in a nanolayered photonic material," Appl. Phys. Lett. 84, 3621-3623 (2004). [CrossRef]
- V. C. Sundar, H.-J. Eisler, T. Deng, Y. Chan, E. L. Thomas, and M. G. Bawendi, "Soft-lithographically embossed, multilayered distributed-feedback nanocrystal lasers," Adv. Mater. 16, 2137-2141 (2004). [CrossRef]
- Y. Chan, J. M. Caruge, P. T. Snee, and M. G. Bawendi, "Multiexcitonic two-state lasing in a CdSe nanocrystal laser," Appl. Phys. Lett. 85, 2460-2462 (2004). [CrossRef]
- P. Lodahl, A. Floris van Driel, I. S. Nikolaev, A. Irman, K. Overgaag, D. Vanmaekelbergh, and W. L. Vos, "Controlling the dynamics of spontaneous emission from quantum dots by photonic crystals," Nature 430, 654-657 (2004) [CrossRef] [PubMed]
- C. Poitras, M. Lipson, H. Du, M. Hahn, and T. Krauss, "Photoluminescence enhancement of colloidal quantum dots embedded in a monolithic microcavity," Appl. Phys. Lett. 82, 4032-4034 (2003). [CrossRef]
- G. Heliotis, R. Xia, D. D. C. Bradley, G. A. Turnbull, I. D. W. Samuel, P. Andrew, and W. L. Barnes, "Blue surface emitting distributed feedback polyfluorene lasers," Appl. Phys. Lett. 83, 2118-2120 (2003). [CrossRef]
- P. Andrew, G. A. Turnbull, I. D. W. Samuel, and W. L. Barnes, "Photonic band structure and emission characteristics of a metal-backed polymeric distributed feedback laser," Appl. Phys. Lett. 81, 954-956 (2002). [CrossRef]
- A. V. Malko, A. A. Mikhailovsky, M. A. Petruska, J. A. Hollingsworth, H. Htoon, M. G. Bawendi, and V. I. Klimov, "From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids," Appl. Phys. Lett. 81, 1303-1305 (2002). [CrossRef]
- H. Eisler, V. C. Sundar, M. G. Bawendi, M. Walsh, H. I. Smith, and V. Klimov, "Color selective semiconductor nanocrystal laser," Appl. Phys. Lett. 80, 4614-4616 (2002). [CrossRef]
- T. Matsui, M. Ozaki, K. Yoshino, and F. Kajzar, "Fabrication of flexible distributed feedback laser using photoinduced surface relief grating on azo-polymer films as a template," Jpn. J. Appl. Phys. 41, L1386-L1388 (2002). [CrossRef]
- A. C. Edrington, A. M. Urbas, P. DeRege, C. X. Chen, T. M. Swager, N. Hadjichristidis, M. Xenidou, L. J. Fetters, J. D. Jounnopoulos, Y. Fink, and E. L. Thomas, "Polymer based photonic crystals," Adv. Mater. 13, 421-425 (2001). [CrossRef]
- C. Finlayson, D. Ginger, and N. Greenham, "Optical microcavities using highly luminescent films of semiconductor nanocrystals," Appl. Phys. Lett. 77, 2500-2502 (2000). [CrossRef]
- S. Riechel, C. Kallinger, U. Lemmer, J. Feldmann, A. Gombert, V. Wittwer, and U. Scherf, "A nearly diffraction limited surface emitting conjugated polymer laser utilizing a two-dimensional photonic band structure," Appl. Phys. Lett. 77, 2310-2312 (2000). [CrossRef]
- M. Meier, A. Mekis, A. Dodabalapur, A. Timko, R. E. Slusher, J. D. Joannopoulos, and O. Nalamasu, "Laser action from two-dimensional distributed feedback in photonic crystals," Appl. Phys. Lett. 74, 7-9 (1999) [CrossRef]
- N. Tessler, G. J. Denton, and R. H. Friend, "Lasing from conjugated polymer microcavities," Nature 382, 695-697 (1996). [CrossRef]
- H. Soda, K. Iga, C. Kitahara, and Y. Suematsu, "GaInAsP/InP surface emitting injection lasers," Jpn. J. Appl. Phys. 18, 2329-2330 (1979). [CrossRef]
- M. Kimura, K. Okahara, and T. Miyamoto, "Tunable multilayer-film distributed Bragg reflector filter," J. Appl. Phys. 50, 1222- 1225 (1979). [CrossRef]
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