Highly efficient organic light-emitting devices beyond theoretical prediction under high current density
Optics Express, Vol. 17, Issue 24, pp. 21370-21375 (2009)
http://dx.doi.org/10.1364/OE.17.021370
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Abstract
We develop a simple method to improve external quantum efficiencies (EQEs) of OLEDs under a wide range of current density. An insulating inorganic ultrathin layer (LiF) was sandwiched between exciton formation layer and electron transporting layer. A maximal EQE of 5.9% in a DCM based fluorescent OLED, which far exceeds the theoretical upper limit of 3.7%, was obtained under the current density of 487 mA/cm2 with a brightness maximum of 76740 cd/m2. The similar electroluminescence properties were also obtained in a C545T based green OLED using this method. The overall enhancement of EQE, and the nonlinear enhancement of EQE at high current density in these devices are attributed to the effect of electrical field on excitons.
© 2009 OSA
OCIS Codes
(160.4890) Materials : Organic materials
(230.3670) Optical devices : Light-emitting diodes
ToC Category:
Optical Devices
History
Original Manuscript: August 31, 2009
Revised Manuscript: October 16, 2009
Manuscript Accepted: October 28, 2009
Published: November 9, 2009
Citation
Miaomiao Tian, Jinsong Luo, and Xingyuan Liu, "Highly efficient organic light-emitting devices beyond theoretical prediction under high current density," Opt. Express 17, 21370-21375 (2009)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-17-24-21370
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References
- C. W. Tang and S. A. Vanslyke, “Organic electroluminescent diodes,” Appl. Phys. Lett. 51(12), 913–915 (1987). [CrossRef]
- J. H. Burroughes, D. D. C. Bradley, A. R. Brown, R. N. Marks, K. Mackay, R. H. Friend, P. L. Burns, and A. B. Holmes, “Light-emitting diodes based on conjugated polymers,” Nature 347(6293), 539–541 (1990). [CrossRef]
- R. H. Friend, R. W. Gymer, A. B. Holmes, J. H. Burroughes, R. N. Marks, C. Taliani, D. D. C. Bradley, D. A. Dos Santos, J. L. Brédas, M. L?gdlund, and W. R. Salaneck, “Electroluminescence in conjugated polymers,” Nature 397(6715), 121–128 (1999). [CrossRef]
- C. C. Tong and K. C. Hwang, “Enhancement of OLED Efficiencies and High-Voltage Stabilities of Light-Emitting Materials by Deuteration,” J. Phys. Chem. C 111(8), 3490–3494 (2007). [CrossRef]
- K. Okumoto, H. Kanno, Y. Hamaa, H. Takahashi, and K. Shibata, “Green fluorescent organic light-emitting device with external quantum efficiency of nearly 10%,” Appl. Phys. Lett. 89(6), 063504 (2006). [CrossRef]
- Q. Huang, S. Reineke, K. Walzer, M. Pfeiffer, and K. Leo, “Quantum efficiency enhancement in top-emitting organic light-emitting diodes as a result of enhanced intrinsic quantum yield,” Appl. Phys. Lett. 89(26), 263512 (2006). [CrossRef]
- X. Liu, H. Li, C. Song, Y. Liao, and M. Tian, “Microcavity organic laser device under electrical pumping,” Opt. Lett. 34(4), 503–505 (2009). [CrossRef] [PubMed]
- N. Tessler, “Lasers Based on Semiconducting Organic Materials,” Adv. Mater. 11(5), 363–370 (1999). [CrossRef]
- M. Koschorreck, R. Gehlhaar, V. G. Lyssenko, M. Swoboda, M. Hoffmann, and K. Leo, “Dynamics of a high-Q vertical-cavity organic laser,” Appl. Phys. Lett. 87(18), 181108 (2005). [CrossRef]
- I. D. W. Samuel and G. A. Turnbull, “Organic Semiconductor Lasers,” Chem. Rev. 107(4), 1272–1295 (2007). [CrossRef] [PubMed]
- M. A. Baldo, R. J. Holmes, and S. R. Forrest, “Prospects for electrically pumped organic lasers,” Phys. Rev. B 66(3), 035321 (2002). [CrossRef]
- T. Matsushima and C. Adachi, “Extremely low voltage organic light-emitting diodes with p-doped alpha-sexithiophene hole transport and n-doped phenyldipyrenylphosphine oxide electron transport layers,” Appl. Phys. Lett. 89(25), 253506 (2006). [CrossRef]
- H. Zhang, Y. Dai, D. Ma, and H. Zhang, “High efficiency tandem organic light-emitting devices with Al/WO3/Au interconnecting layer,” Appl. Phys. Lett. 91(12), 123504 (2007). [CrossRef]
- Y. Kawamura, H. Sasabe, and C. Adachi, “Simple Accurate System for Measuring Absolute Photoluminescence Quantum Efficiency in Organic Solid-State Thin Films,” Jpn. J. Appl. Phys. 43(No. 11A), 7729–7730 (2004). [CrossRef]
- M. Segal, M. Singh, K. Rivoire, S. Difley, T. Van Voorhis, and M. A. Baldo, “Extrafluorescent electroluminescence in organic light-emitting devices,” Nat. Mater. 6(5), 374–378 (2007). [CrossRef] [PubMed]
- A. J. Heeger, Y. Cao, I. D. Parker, G. Yu, and C. Zhang, “Improved quantum efficiency for electroluminescence in semiconducting polymers,” Nature 397(6718), 414–417 (1999). [CrossRef]
- H. You, Y. Dai, Z. Zhang, and D. Ma, “Improved performances of organic light-emitting diodes with metal oxide as anode buffer,” J. Appl. Phys. 101(2), 026105 (2007). [CrossRef]
- S. R. Forrest, D. D. C. Bradley, and M. E. Thompson, “Measuring the efficiency of organic light-emitting devices,” Adv. Mater. 15(13), 1043–1048 (2003). [CrossRef]
- S. Qu, X. Chen, X. Shao, F. Li, H. Zhang, H. Wang, P. Zhang, Z. Yu, K. Wu, Y. Wang, and M. Li, “Self-assembly of highly luminescent bi-1,3,4-oxadiazole derivatives through electron donor–acceptor interactions in three-dimensional crystals, two-dimensional layers and mesophases,” J. Mater. Chem. 18(33), 3954–3964 (2008). [CrossRef]
- H. Nakanotani, H. Sasabe, and C. Adachi, “Singlet-singlet and singlet-heat annihilations in fluorescence-based organic light-emitting diodes under steady-state high current density,” Appl. Phys. Lett. 86(21), 213506 (2005). [CrossRef]
- S. Yin, L. Chen, P. Xuan, K.-Q. Chen, and Z. Shuai, “Field Effect on the Singlet and Triplet Exciton Formation in Organic/Polymeric Light-Emitting Diodes,” J. Phys. Chem. B 108(28), 9608–9613 (2004). [CrossRef]
- J. Yang and J. Shen, “Doping effects in organic electroluminescent devices,” J. Appl. Phys. 84(4), 2105–2111 (1998). [CrossRef]
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