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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 17, Iss. 24 — Nov. 23, 2009
  • pp: 22171–22178

Strong exciton-photon coupling in inorganic-organic multiple quantum wells embedded low-Q microcavity

K. Pradeesh, J. J. Baumberg, and G. Vijaya Prakash  »View Author Affiliations


Optics Express, Vol. 17, Issue 24, pp. 22171-22178 (2009)
http://dx.doi.org/10.1364/OE.17.022171


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Abstract

Optoelectronic-compatible heterostructures are fabricated from layered inorganic-organic multiple quantum wells (IO-MQW) of Cyclohexenyl ethyl ammonium lead iodide, (C6H9C2H4NH3)2PbI4 (CHPI). These hybrids possess strongly-resonant optical features, are thermally stable and compatible with hybrid photonics assembly. Room-temperature strong-coupling is observed when these hybrids are straightforwardly embedded in metal-air (M-A) and metal-metal (M-M) low-Q microcavities, due to the large oscillator strength of these IO-MQWs. The strength of the Rabi splitting is 130meV for M-A and 160meV for M-M cavities. These values are significantly higher than for J-aggregates in all-metal microcavities of similar length. These experimental results are in good agreement with transfer matrix simulations based on resonant excitons. Incorporating exciton-switching hybrids allows active control of the strong-coupling parameters by temperature, suggesting new device applications.

© 2009 OSA

OCIS Codes
(160.4670) Materials : Optical materials
(250.5230) Optoelectronics : Photoluminescence
(310.3840) Thin films : Materials and process characterization
(140.3948) Lasers and laser optics : Microcavity devices
(250.4745) Optoelectronics : Optical processing devices

ToC Category:
Optoelectronics

History
Original Manuscript: August 19, 2009
Revised Manuscript: September 23, 2009
Manuscript Accepted: September 27, 2009
Published: November 19, 2009

Citation
K. Pradeesh, J. J. Baumberg, and G. Vijaya Prakash, "Strong exciton-photon coupling in inorganic-organic multiple quantum wells embedded low-Q microcavity," Opt. Express 17, 22171-22178 (2009)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-17-24-22171


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