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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 17, Iss. 9 — Apr. 27, 2009
  • pp: 6975–6981

Controllable transport mean free path of light in xerogel matrixes embedded with polystyrene spheres

Boris P. J. Bret, Nuno J. G. Couto, Mariana Amaro, Eduardo J. Nunes-Pereira, and Michael Belsley  »View Author Affiliations


Optics Express, Vol. 17, Issue 9, pp. 6975-6981 (2009)
http://dx.doi.org/10.1364/OE.17.006975


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Abstract

Xerogel matrices, made by sol-gel techniques, are embedded with polystyrene spheres to promote multiple scattering of light. Varying the concentration of the spheres inside the matrix allows one to adjust the transport mean free path of light inside the material. Coherent backscattering measurements show that a range of transport mean free paths from 90 to 600 nm is easily achieved. The determination of the matrix refractive index permits a direct comparison to multiple scattering and Mie theory. Such tunable diffusive sol-gel derived samples can be further optimized as random laser materials.

© 2009 Optical Society of America

OCIS Codes
(030.1670) Coherence and statistical optics : Coherent optical effects
(160.2710) Materials : Inhomogeneous optical media

ToC Category:
Coherence and Statistical Optics

History
Original Manuscript: January 14, 2009
Revised Manuscript: January 28, 2009
Manuscript Accepted: January 29, 2009
Published: April 13, 2009

Citation
Boris P. Bret, Nuno J. Couto, Mariana Amaro, Eduardo J. Nunes-Pereira, and Michael Belsley, "Controllable transport mean free path of light in xerogel matrixes embedded with polystyrene spheres," Opt. Express 17, 6975-6981 (2009)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-17-9-6975


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References

  1. P. Sheng, Introduction to Wave Scattering, Localization, and Mesoscopic Phenomena (Academic, New York, 1995)
  2. M. P. van Albada and A. Lagendijk, "Observation of weak localization of light in a random medium," Phys. Rev. Lett. 55, 2692-2695 (1985) [CrossRef] [PubMed]
  3. P. E. Wolf and G. Maret, "Weak localization and coherent backscattering of photons in disordered media," Phys. Rev. Lett. 55, 2696-2699 (1985) [CrossRef] [PubMed]
  4. J. L. Thomas, P. Roux, and M. Fink, "Inverse scattering analysis with an acoustic time-reversal mirror," Phys. Rev. Lett. 72, 637-640 (1994) [CrossRef] [PubMed]
  5. A. Derode, P. Roux, and M. Fink, "Robust acoustic time-reversal with high-order multiple-scattering," Phys. Rev. Lett. 75, 4206-4209 (1995) [CrossRef] [PubMed]
  6. R. Pappu, B. Recht, J. Taylor, and N. Gershenfeld, "Physical one-way functions," Science 297, 2026-2030 (2002) [CrossRef] [PubMed]
  7. A. L. Moustakas, H. U. Baranger, L. Balents, A. M. Sengupta, and S. H. Simon, "Communication through a diffusive medium: Coherence and capacity," Science 287, 287-290 (2000) [CrossRef] [PubMed]
  8. I. M. Vellekoop and A. P. Mosk, "Focusing coherent light through opaque strongly scattering media," Opt. Lett. 32, 2309-2311 (2007) [CrossRef] [PubMed]
  9. I. M. Vellekoop and A. P. Mosk, "Universal optimal transmission of light through disordered materials,"Phys. Rev. Lett. 101, 120601 (2008) [CrossRef] [PubMed]
  10. V. S. Letokhov, "Generation of light by a scattering medium with negative resonance absorption," Zh. Eksp. Teor. Fiz. 53, 1442 (1968), [Sov. Phys. JETP 26, 835]
  11. C. Gouedard, D. Husson, C. Sauteret, F. Auzel, and A. Migus, "Generation of spatially incoherent short pulses in laser-pumped neodymium stoichiometric crystals and powders," J. Opt. Soc. Am. B 10, 2358-2363 (1993) [CrossRef]
  12. H. Cao, J. Y. Xu, E.W. Seelig, and R. P. H. Chang, "Microlaser made of disordered media," Appl. Phys. Lett. 76, 2997-2999 (2000) [CrossRef]
  13. L. L. Hench and J. K. West, "The sol-gel process," Chem. Rev. 90, 33-72 (1990) [CrossRef]
  14. C. J. Brinker and G. W. Scherer, Sol-Gel Science: The Physics and Chemistry of Sol-Gel Processing (Academic Press, 1990)
  15. G. Hungerford, K. Suhling, and J. A. Ferreira, "Comparison of the fluorescence behaviour of rhodamine 6G in bulk and thin film tetraethylorthosilicate derived sol-gel matrices," J. Photochem. Photobiol A 129, 71-80 (1999) [CrossRef]
  16. Y. Takahashi, T. Kitamura, M. Nogami, K. Uchida, and T. Yamanaka, "Luminescence of rhodamine dyes doped in amorphous silica glasses," J.Lumin. 60/61, 451-453 (1994) [CrossRef]
  17. H. Nakazumi, T. Tarao, S.-I. Taniguchi, and H. Nanto, "Fluorescent thin gel films using organic dyes and pigments," in Sol-gel optics IV, B. S. Dunn, J. D. Mackenzie, E. J. A. Pope, H. K. Schmidt, and M. Yamane, eds., Proc. SPIE 3136, 159-167 (1997) [CrossRef]
  18. M. Casalboni, F. De Matteis, V. Ferone, P. Prosposito, R. Senesi, R. Pizzoferrato, A. Bianco, and A. De Mico, "DODCI molecules incorporated in sol-gel glasses: the interaction with the silica matrix," Chem. Phys. Lett. 291, 167-172 (1998) [CrossRef]
  19. L. L. Hu, and Z. H. Jiang, "Laser performance in dye molecules doped xerogels," in Sol-gel optics IV, B. S. Dunn, J. D. Mackenzie, E. J. A. Pope, H. K. Schmidt, and M. Yamane, eds., Proc. SPIE 3136, 94-101 (1997) [CrossRef]
  20. E. T. Knobbe, B. Dunn, P. D. Fuqua, and F. Nishida, "Laser behavior and photostability of organic-dye doped silicate gel materials," Appl. Opt. 29, 2729-2733 (1990) [CrossRef] [PubMed]
  21. M. D. Rahn and T. A. King, "Comparison of laser performance of dye molecules in sol-gel, polycom, ormosil, and poly(methyl methacrylate) host media," Appl. Opt. 34, 8260-8271 (1995) [CrossRef] [PubMed]
  22. T. H. Nhung, M. Canva, T. T. A. Dao, F. Chaput, A. Brun, N. D. Hung, and J.-P. Boilot, "Stable doped hybrid sol-gel materials for solid-state dye laser," Appl. Opt. 42, 2213-2218 (2003) [CrossRef] [PubMed]
  23. P. Boutin, J. Mugnier, and B. Valeur, "A fast-responding optical pH sensor based on the fluorescence of eosin trapped in a TiO2 solgel thin film," J. Fluorescence 7, 215S-218S (1997)
  24. K. Dou, X. Sun, X. Wang, and E. K. Knobbe,"Nonlinear absorption and emission of excited states in metalloporphyrin-doped sol gels" in Sol-gel optics IV, B. S. Dunn, J. D. Mackenzie, E. J. A. Pope, H. K. Schmidt, and M. Yamane, eds., Proc. SPIE 3136, 48-56 (1997) [CrossRef]
  25. N. Hayashida, A. Kosuda, and J. Yoshinari,"A new class of photopolymer for holographic data storage media based on organometallic matrix," Jpn. J. Appl. Phys. 47, 5895-5899 (2008) [CrossRef]
  26. G. Hungerford, A. Rei, and M. I. C. Ferreira, "Use of fluorescence to monitor the incorporation of horseradish peroxidase into a sol-gel derived medium," Biophys. Chem. 120, 81-86 (2006) [CrossRef]
  27. D. Richter and D. Lipka, "Measurement of the refractive index of silica aerogel in vacuum," Nucl. Instr. and Methods in Phys. Res. A 513, 635-638 (2003) [CrossRef]
  28. L. C. Klein, Sol-gel technology for thin films, fibers, preforms, electronics, and speciality shapes (Noyes publications, 1998)
  29. D. Stroud, "Generalized effective-medium approach to conductivity of an inhomogeneous material,"Phys. Rev. B 12, 3368-3373 (1975) [CrossRef]
  30. M. M. Braun and L. Pilon, "Effective optical properties of non-absorbing nanoporous thin films," Thin Sol. Films 496, 505-514 (2006) [CrossRef]
  31. D. S. Wiersma, M. P. van Albada, B. A. van Tiggelen and A. Lagendijk, "Experimental evidence for recurrent multiple-scattering events of light in disordered media," Phys. Rev. Lett. 74, 4193-4196 (1995) [CrossRef] [PubMed]
  32. M. B. van der Mark, M. P. van Albada, and A. Lagendijk, "Light-scattering in strongly scattering media -Multiple-scattering and weak localization," Phys. Rev. B 37, 3575-3592 (1988) [CrossRef]
  33. D. S. Wiersma, P. Bartolini, A. Lagendijk, and R. Righini, "Localization of light in a disordered medium," Nature 390, 671-673 (1997) [CrossRef]
  34. F. J. P. Schuurmans, D. Vanmaekelbergh, J. van de Lagemaat, and A. Lagendijk, "Strongly photonic macroporous gallium phosphide networks," Science 284, 141-143 (1999) [CrossRef] [PubMed]
  35. J. Gómez Rivas, R. W. Tjerkstra, D. Vanmaekelbergh, J. J. Kelly, and A. Lagendijk, "Tunable photonic strength in porous GaP," Appl. Phys. Lett. 80, 4498-4500 (2002) [CrossRef]
  36. M. Störzer, P. Gross, C. M. Aegerter, and G. Maret, "Observation of the critical regime near Anderson localization of light," Phys. Rev. Lett. 96, 063904 (2006) [CrossRef] [PubMed]
  37. S. Gottardo, R. Sapienza, P. D. Garca, A. Blanco, D. S. Wiersma and C. López, "Resonance-driven random lasing," Nature Photonics 2, 429-432 (2008) [CrossRef]
  38. G. Mie, "Articles on the optical characteristics of turbid tubes, especially colloidal metal solutions," Ann. Phys. (Leipzig) 25, 377-445 (1908)
  39. C. F. Bohren and D. R. Huffman, Absorption and scattering of light by small particles (JohnWiley & Sons, New York, 1983)

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