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Investigation of the electronic and physical properties of defect structures responsible for laser-induced damage in DKDP crystals
Stavros G. Demos, Paul DeMange, Raluca A. Negres, and Michael D. Feit »View Author Affiliations
Stavros G. Demos,*
Paul DeMange,
Raluca A. Negres,
and Michael D. Feit
Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, CA 94550, USA
*Corresponding author: demos1@llnl.gov
Optics Express, Vol. 18, Issue 13, pp. 13788-13804 (2010)
http://dx.doi.org/10.1364/OE.18.013788
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Abstract
Laser-induced damage at near operational laser excitation conditions can limit the performance of potassium dihydrogen phosphate (KH2PO4, or KDP) and its deuterated analog (DKDP) which are currently the only nonlinear optical materials suitable for use in large-aperture laser systems. This process has been attributed to pre-existing damage precursors that were incorporated or formed during growth that have not yet been identified. In this work, we present a novel experimental approach to probe the electronic structure of the damage precursors. The results are modeled assuming a multi-level electronic structure that includes a bottleneck for 532 nm excitation. This model reproduces our experimental observations as well as other well-documented behaviors of laser damage in KDP crystals. Comparison of the electronic structure of known defects in KDP with this model allows for identification of a specific class that we postulate may be the constituent defects in the damage precursors. The experimental results also provide evidence regarding the physical parameters affecting the ability of individual damage precursors to initiate damage, such as their size and defect density; these parameters were found to vary significantly between KDP materials that exhibit different damage performance characteristics.
© 2010 OSA
OCIS Codes
(140.3330) Lasers and laser optics : Laser damage
(160.4330) Materials : Nonlinear optical materials
ToC Category:
Lasers and Laser Optics
History
Original Manuscript: April 7, 2010
Revised Manuscript: May 11, 2010
Manuscript Accepted: May 13, 2010
Published: June 11, 2010
Citation
Stavros G. Demos, Paul DeMange, Raluca A. Negres, and Michael D. Feit, "Investigation of the electronic and physical properties of defect structures responsible for laser-induced damage in DKDP crystals," Opt. Express 18, 13788-13804 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-13-13788
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Fusion Sci. Technol.
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Int. Mater. Rev.
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J. Opt. Soc. Am. B
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Nature
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Nucl. Fusion
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Opt. Eng.
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Opt. Express
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Opt. Lett.
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Phys. Rev. B
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Phys. Rev. Lett.
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Proc. SPIE
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Rev. Sci. Instrum.
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2010, Reyné, Appl. Phys. Lett.
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- J. J. Adams, T. L. Weiland, J. R. Stanley, W. D. Sell, R. L. Luthi, J. L. Vickers, C. W. Carr, M. D. Feit, A. M. Rubenchik, M. L. Spaeth, and R. P. Hackel, “Pulse length dependence of laser conditioning and bulk damage in KH2PO4,” Proc. SPIE 5647, 265–278 (2005). [CrossRef]
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- P. DeMange, C. W. Carr, H. B. Radousky, and S. G. Demos, “System for evaluation of laser-induced damage performance of optical materials for large aperture lasers,” Rev. Sci. Instrum. 75(10), 3298–3301 (2004). [CrossRef]
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- M. D. Feit, A. M. Rubenchik, and M. Runkel, “Analysis of Bulk DKDP Damage Distribution, Obscuration and Pulselength Dependence,” Proc. SPIE 4347, 383–388 (2001). [CrossRef]
- S. I. Kudryashov and V. I. Emelyanov, “Band Gap Collapse and Ultrafast Cold Melting of Silicon during Femtosecond Laser Pulse,” JETP Lett. 73(5), 228–231 (2001). [CrossRef]
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- S. G. Demos, M. Yan, M. Staggs, J. J. De Yoreo, and H. B. Radousky, “Raman Scattering Investigation of KDP Subsequent to High Fluence Laser Irradiation,” Appl. Phys. Lett. 72(19), 2367–2369 (1998). [CrossRef]
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