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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 18, Iss. 6 — Mar. 15, 2010
  • pp: 6340–6346

Anti-bunching and luminescence blinking suppression from plasmon-interacted single CdSe/ZnS quantum dot

Xiao-Wei Wu, Ming Gong, Chun-Hua Dong, Jin-Ming Cui, Yong Yang, Fang-Wen Sun, Guang-Can Guo, and Zheng-Fu Han  »View Author Affiliations


Optics Express, Vol. 18, Issue 6, pp. 6340-6346 (2010)
http://dx.doi.org/10.1364/OE.18.006340


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Abstract

CdSe/ZnS colloidal quantum dots generally exist as blinking phenomena during the luminescence process that remarkably influences its applications. In this work, we used the surface plasmonic effect to effectively modulate single quantum dots. Obvious contrasts have been observed by comparing single quantum dots on silica and gold films. The surface plasmon is shown to obviously suppress the blinking of single quantum dots. With further demonstrated second- order correlation measurements, an anti-bunching effect was observed. The anti-bunching dip gives the smallest value of g(2)(0) = 0.15, and the lifetime of the exciton has been reduced. This method presents the application’s potential towards tunable high-emitting-speed single photon sources at room temperature.

© 2010 Optical Society of America

OCIS Codes
(030.5260) Coherence and statistical optics : Photon counting
(240.6680) Optics at surfaces : Surface plasmons
(270.5290) Quantum optics : Photon statistics

ToC Category:
Quantum Optics

History
Original Manuscript: January 14, 2010
Revised Manuscript: February 18, 2010
Manuscript Accepted: March 5, 2010
Published: March 12, 2010

Citation
Xiao-Wei Wu, Ming Gong, Chun-Hua Dong, Jin-Ming Cui, Yong Yang, Fang-Wen Sun, Zheng-Fu Han, and Guang-Can Guo, "Anti-bunching and luminescence blinking suppression from plasmon-interacted single CdSe/ZnS quantum dot," Opt. Express 18, 6340-6346 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-6-6340


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References

  1. B. Lounis and M. Orrit, "Single-photon sources," Rep. Prog. Phys. 68,1129-1179 (2005). [CrossRef]
  2. D. Loss and D. P. DiVincenzo, "Quantum computation with quantum dots," Phys. Rev. A 57,120-126 (1998). [CrossRef]
  3. T. Yoshie, A. Scherer, J. Hendrickson, G. Khitrova, H. M. Gibbs, G. Rupper, C. Ell, O. B. Shchekin, and D. G. Deppe, "Vacuum Rabi splitting with a single quantum dot in a photonic crystal nanocavity," Nature 432,200-203 (2004). [CrossRef] [PubMed]
  4. H. Mattoussi, J. M. Mauro, E. R. Goldman, G. P. Anderson, V. C. Sundar, F. V. Mikulec, and M. G. Bawendi, "Self-assembly of CdSe/ZnS quantum dot bioconjugates using an engineered recombinant protein," J. Am. Chem. Soc. 122,12142-12150 (2000). [CrossRef]
  5. J. P. Reithmaier, G. Sek, A. L¨offler, C. Hofmann, S. Kuhn, S. Reitzenstein, L. V. Keldysh, V. D. Kulakovskii, T. L. Reinecke, and A. Forchel, "Strong coupling in a single quantum dot-semiconductor microcavity system," Nature 432,197-200 (2004). [CrossRef] [PubMed]
  6. Y. Fedutik, V. V. Temnov, O. Sch¨ops, U. Woggon, and M. V. Artemyev, "Exciton-plasmon-photon conversion in plasmonic nanostructures," Phys. Rev. Lett. 99,136802 (2007). [CrossRef] [PubMed]
  7. P. Michler, A. Imamo˘glu, M. D. Mason, P. J. Carson, G. F. Strouse, and S. K. Buratto, "Quantum correlation among photons from a single quantum dot at room temperature," Nature 406,968-970 (2000). [CrossRef] [PubMed]
  8. C. Yang, Z. Zhong, and C. M. Lieber, "Encoding electronic properties by synthesis of axial modulation-doped silicon nanowires," Science 310,1304-1307 (2005). [CrossRef] [PubMed]
  9. Y. Ito, K. Matsuda, and Y. Kanemitsu, "Mechanism of photoluminescence enhancement in single semiconductor nanocrystals on metal surfaces," Phys. Rev. B 75,033309 (2007). [CrossRef]
  10. C. T. Yuan, P. Yu, and J. Tang, "Blinking suppression of colloidal CdSe/ZnS quantum dots by coupling to silver nanoprisms," Appl. Phys. Lett. 94,243108 (2009). [CrossRef]
  11. H. J. Kimble, M. Dagenais, and L. Mandel, "Photon antibunching in resonance fluorescence," Phys. Rev. Lett. 39,691-695 (1977). [CrossRef]
  12. Q1. F. Koberling, A. Mews, and T. Basch’e, "Oxygen-induced blinking of single CdSe nanocrystals," Adv. Mater. 13,672-676 (2000). [CrossRef]
  13. V. I. Klimov, A. A. Mikhailovsky, D. W. McBranch, C. A. Leatherdale, and M. G. Bawendi, "Quantization of multiparticle Auger rates in semiconductor quantum dots," Science 287,1011-1013 (2000). [CrossRef] [PubMed]
  14. M. Kuno, D. P. Fromm, H. F. Hamann, A. Gallagher, and D. J. Nesbitt, "Nonexponential ’blinking’ kinetics of single CdSe quantum dots: a universal power law behavior," J. Chem. Phys. 112,3117-3120 (2000). [CrossRef]
  15. K. T. Shimizu, R. G. Neuhauser, C. A. Leatherdale, S. A. Empedocles,W. K. Woo, and M. G. Bawendi, "Blinking statistics in single semiconductor nanocrystal quantum dots," Phys. Rev. B 63,205316 (2001). [CrossRef]
  16. S. Schietinger, M. Barth, T. Aichele, and O. Benson, "Plasmon-enhanced single photon emission from a nanoassembled metal-diamond hybrid structure at room temperature," Nano Lett. 9,1694-1698 (2009). [CrossRef] [PubMed]
  17. S. K¨uhn, U. H°akanson, L. Rogobete, and V. Sandoghdar, "Enhancement of single-molecule fluorescence using a gold nanoparticle as an optical nanoantenna," Phys. Rev. Lett. 97,017402 (2006). [CrossRef] [PubMed]
  18. P. Bharadwaj and L. Novotny, "Spectral dependence of single molecule fluorescence enhancement," Opt. Express 15,14266-14274 (2007). [CrossRef] [PubMed]
  19. B. Lounis, H. A. Bechtel, D. Gerion, A. P. Alivisatos, and W. E. Moerner, "Photon antibunching in single CdSe/ZnS quantum dot fluorescence," Chem. Phys. Lett. 329,399-404 (2000). [CrossRef]
  20. M. Moskovits, "Surface-enhanced spectroscopy," Rev. Mod. Phys. 57,783-826 (1985). [CrossRef]
  21. K. T. Shimizu, W. K. Woo, B. R. Fisher, H. J. Eisler, and M. G. Bawendi, "Surface-enhanced emission from single semiconductor nanocrystals," Phys. Rev. Lett. 89,117404 (2002). [CrossRef]
  22. A. O. Govorov, G. W. Bryant, W. Zhang, T. Skeini, J. Lee, N. A. Kotov, J. M. Slocik, and R. R. Naik, "Excitonplasmon interaction and hybrid excitons in semiconductor-metal nanoparticle assemblies," Nano Lett. 6,984-994 (2006). [CrossRef]
  23. M. T. Cheng, S. D. Liu, and Q. Q. Wang, "Modulating emission polarization of semiconductor quantum dots through surface plasmon of metal nanorod," Appl. Phys. Lett. 92,162107 (2008). [CrossRef]
  24. C. Becker, A. Kiraz, P. Michler, A. Imamoglu, W. V. Schoenfeld, P. M. Petroff, L. D. Zhang, and E. Hu, "Nonclassical radiation from a single self-assembled InAs quantum dot," Phys. Rev. B 63,121312 (2001). [CrossRef]
  25. K. Sebald, P. Michler, T. Passow, D. Hommel, G. Bacher, and A. Forchel, "Single-photon emission of CdSe quantum dots at temperatures up to 200 K," Appl. Phys. Lett. 81,2920-2922 (2002). [CrossRef]
  26. M. Califano, A. Franceschetti, and A. Zunger, "Lifetime and polarization of the radiative decay of excitons, biexcitons, and trions in CdSe nanocrystal quantum dots," Phys. Rev. B 75,115401 (2007). [CrossRef]
  27. E. Waks, C. Santori, and Y. Yamamoto, "Security aspects of quantum key distribution with sub-Poisson light," Phys. Rev. A 66,042315 (2002). [CrossRef]
  28. X. Wang, X. Ren, K. Kahen, M. A. Hahn, M. Rajeswaran, S. Maccagnano-Zacher, J. Silcox, G. E. Cragg, A. L. Efros, and T. D. Krauss, "Non-blinking semiconductor nanocrystals," Nature 459,686-689 (2009). [CrossRef] [PubMed]
  29. C. Kurtsiefer, S. Mayer, P. Zarda, and H. Weinfurter, "Stable solid-state source of single photons," Phys. Rev. Lett. 85,290-293 (2000). [CrossRef] [PubMed]

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