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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 18, Iss. 7 — Mar. 29, 2010
  • pp: 6577–6582

Near-infrared single-photons from aligned molecules in ultrathin crystalline films at room temperature

C. Toninelli, K. Early, J. Bremi, A. Renn, S. Götzinger, and V. Sandoghdar  »View Author Affiliations


Optics Express, Vol. 18, Issue 7, pp. 6577-6582 (2010)
http://dx.doi.org/10.1364/OE.18.006577


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Abstract

We investigate the optical properties of Dibenzoterrylene (DBT) molecules in a spin-coated crystalline film of anthracence. By performing single molecule studies, we show that the dipole moments of the DBT molecules are oriented parallel to the plane of the film. Despite a film thickness of only 20 nm, we observe an exceptional photostability at room temperature and photon count rates around 106 per second from a single molecule. These properties together with an emission wavelength around 800 nm make this system attractive for applications in nanophotonics and quantum optics.

© 2010 Optical Society of America

OCIS Codes
(030.5290) Coherence and statistical optics : Photon statistics
(270.0270) Quantum optics : Quantum optics
(300.0300) Spectroscopy : Spectroscopy

ToC Category:
Quantum Optics

History
Original Manuscript: January 26, 2010
Revised Manuscript: March 3, 2010
Manuscript Accepted: March 3, 2010
Published: March 15, 2010

Citation
C. Toninelli, K. Early, J. Bremi, A. Renn, S. Götzinger, and V. Sandoghdar, "Near-infrared single-photons from aligned molecules in ultrathin crystalline films at room temperature," Opt. Express 18, 6577-6582 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-7-6577


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