High pressure effect on the ultrafast energy relaxation rate of LDS698 (C19H23N2O4Cl) in a solution

doi:10.1364/OE.18.006863

High pressure effect on the ultrafast energy relaxation rate of LDS698 (C₁₉H₂₃N₂O₄Cl) in a solution

Bingguo Liu, Chunyuan He, Mingxing Jin, Qiaoqiao Wang, Sheng Hsien Lin, and Dajun Ding »View Author Affiliations

Optics Express, Vol. 18, Issue 7, pp. 6863-6870 (2010)
http://dx.doi.org/10.1364/OE.18.006863

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Abstract

Effects of high pressure in a range of up to 1.7 GPa on ultrafast energy relaxation of LDS698 (C₁₉H₂₃N₂O₄Cl) molecules in solution have experimentally been illustrated by a method of femtosecond time-resolved absorption spectroscopy. The rates of the intramolecular and intermolecular energy relaxations show quite different pressure dependences. The observed results are in good agreement with the theoretical interpretation based on the pressure influences on the molecular energy gaps, the intermolecular H-bond interaction, and the solution viscosity.

OCIS Codes
(300.6500) Spectroscopy : Spectroscopy, time-resolved
(320.7130) Ultrafast optics : Ultrafast processes in condensed matter, including semiconductors

ToC Category:
Spectroscopy

History
Original Manuscript: December 16, 2009
Revised Manuscript: February 10, 2010
Manuscript Accepted: March 10, 2010
Published: March 18, 2010

Citation
Bingguo Liu, Chunyuan He, Mingxing Jin, Qiaoqiao Wang, Sheng Hsien Lin, and Dajun Ding, "High pressure effect on the ultrafast energy relaxation rate of LDS698 (C₁₉H₂₃N₂O₄Cl) in a solution," Opt. Express 18, 6863-6870 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-7-6863

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References

S. Woutersen and H. J. Bakker, “Resonant intermolecular transfer of vibrational energy in liquid water,” Nature 402(6761), 507–509 (1999). [CrossRef]
C. Chudoba, E. T. J. Nibbering, and T. Elsaesser, “Site-specific excited-state solute-solvent interactions probed by femtosecond vibrational spectroscopy,” Phys. Rev. Lett. 81(14), 3010–3013 (1998). [CrossRef]
J. Assmann, R. V. Benten, A. Charvat, and B. Abel, “Vibrational energy relaxation of selectively excited aromatic molecules in solution: The effect of a methyl rotor and its chemical substitution,” J. Phys. Chem. A 107(12), 1904–1913 (2003). [CrossRef]
S. H. Lin, “Rate of interconversion of electronic and vibrational energy,” J. Chem. Phys. 44(10), 3759–3767 (1966). [CrossRef]
T. Kobayashi, M. Shiga, A. Murakami, and S. J. Nakamura, “Ab initio study of ultrafast photochemical reaction dynamics of phenol blue,” J. Am. Chem. Soc. 129(20), 6405–6424 (2007). [CrossRef] [PubMed]
R. M. Stratt and M. Maroncelli, “Nonreactive dynamics in solution: the emerging molecular view of solvation dynamics and vibrational relaxation,” J. Phys. Chem. 100(31), 12981–12996 (1996). [CrossRef]
J. Y. Liu, W. H. Fan, K. L. Han, D. L. Xu, and N. Q. Lou, “Ultrafast dynamics of dye molecules in solution as a function of temperature,” J. Phys. Chem. A 107(12), 1914–1917 (2003). [CrossRef]
J. Y. Liu, W. H. Fan, K. L. Han, W. Q. Deng, D. L. Xu, and N. Q. Lou, “Ultrafast vibrational and thermal relaxation of dye molecules in solutions,” J. Phys. Chem. A 107(50), 10857–10861 (2003). [CrossRef]
K. Niss, B. Begen, B. Frick, J. Ollivier, A. Beraud, A. Sokolov, V. N. Novikov, and C. Alba-Simionesco, “Influence of pressure on the boson peak: stronger than elastic medium transformation,” Phys. Rev. Lett. 99(5), 055502 (2007). [CrossRef] [PubMed]
D. J. Mitchell, G. B. Schuster, and H. G. Drickamer, “Effect of pressure on the fluorescence of 9-carbonyl substituted anthracenes,” J. Am. Chem. Soc. 99(4), 1145–1148 (1977). [CrossRef]
H. Li, B. Zhong, L. M. He, G. Q. Yang, Y. Li, S. Wu, and J. Liu, “High pressure effects on the luminescent properties and structure of coumarin 153,” Appl. Phys. Lett. 80(13), 2299–2301 (2002). [CrossRef]
B. C. Hess, G. S. Kanner, Z. V. Vardeny, and G. L. Baker, “High-pressure effects on ultrafast-relaxation kinetics of excitons in polydiacetylene 4BCMU,” Phys. Rev. Lett. 66(18), 2364–2367 (1991). [CrossRef] [PubMed]
N. Baden, O. Kajimoto, and K. Hara, “High-pressure studies on aggregation number of surfactant micelles using the fluorescence quenching method,” J. Phys. Chem. B 106(34), 8621–8624 (2002). [CrossRef]
S. Bai and C. R. Yonker, “Pressure and temperature effects on the hydrogen-bond structures of liquid and supercritical fluid methanol,” J. Phys. Chem. A 102(45), 8641–8647 (1998). [CrossRef]
J. P. Schmidtke, J. S. Kim, J. Gierschner, C. Silva, and R. H. Friend, “Optical spectroscopy of a polyfluorene copolymer at high pressure: intra- and intermolecular interactions,” Phys. Rev. Lett. 99(16), 167401 (2007). [CrossRef] [PubMed]
Y. Umebayashi, J. C. Jiang, Y. L. Shan, K. H. Lin, K. Fujii, S. Seki, S. I. Ishiguro, S. H. Lin, and H. C. Chang, “Structural change of ionic association in ionic liquid/water mixtures: a high-pressure infrared spectroscopic study,” J. Chem. Phys. 130(12), 124503 (2009). [CrossRef] [PubMed]
D. Ducoulombier, H. Zhou, C. Boned, J. Peyrelasse, H. Saint-Guirons, and P. Xans, “Pressure (1-1000bar) and temperature (20-100oC) dependence of the viscosity of liquid hydrocarbons,” J. Phys. Chem. 90(8), 1692–1700 (1986). [CrossRef]
S. H. Lin, “Effect of high pressure on molecular electronic spectra and electronic relaxation,” J. Chem. Phys. 59(8), 4458–4467 (1973). [CrossRef]
R. J. Hemley, P. M. Bell, and H. K. Mao, “Laser Techniques in High-Pressure Geophysics,” Science 237(4815), 605–612 (1987). [CrossRef] [PubMed]
B. G. Liu, M. X. Jin, H. Liu, C. Y. He, D. W. Jiang, and D. Ding, “Femtosecond time-resolved measurement of LDS698 molecular processes under high pressure,” Appl. Phys. Lett. 92(24), 241916 (2008). [CrossRef]
H. G. Drickamer, and C. W. Frank, “Electronic transitions and the high pressure chemistry and physics of solids” (Chapman-Hall, London, 1973).
M. Dantus, M. J. Rosker, and A. H. Zewail, “Real-time femtosecond probing of transition-states in chemical-reactions,” J. Chem. Phys. 87(4), 2395–2397 (1987). [CrossRef]
S. H. Lin, C. H. Chang, K. K. Liang, R. Chang, Y. J. Shiu, J. M. Zhang, T. S. Yang, M. Hayashi, and F. C. Hsu, “Ultrafast dynamics and spectroscopy of bacterial photosynthetic reaction centers,” Adv. Chem. Phys. 121, 1–88 (2002). [CrossRef]
T. Förster, “Transfer mechanisms of electronic excitation,” Discuss. Faraday Soc. 27, 7–17 (1959).
J. M. Brown, L. J. Slutsky, K. A. Nelson, and L. T. Cheng, “Velocity of sound and equations of state for methanol and ethanol in a diamond-anvil cell,” Science 241(4861), 65–67 (1988). [CrossRef] [PubMed]

Abel, B.
Alba-Simionesco, C.
Assmann, J.
Baden, N.
Bai, S.
Baker, G. L.
Bakker, H. J.
Begen, B.
Bell, P. M.
Benten, R. V.
Beraud, A.
Boned, C.
Brown, J. M.
Chang, C. H.
Chang, H. C.
Chang, R.
Charvat, A.
Cheng, L. T.
Chudoba, C.
Dantus, M.
Deng, W. Q.
Ding, D.
Drickamer, H. G.
Ducoulombier, D.
Elsaesser, T.
Fan, W. H.
Förster, T.
Frick, B.
Friend, R. H.
Fujii, K.
Gierschner, J.
Han, K. L.
Hara, K.
Hayashi, M.
He, C. Y.
He, L. M.
Hemley, R. J.
Hess, B. C.
Hsu, F. C.
Ishiguro, S. I.
Jiang, D. W.
Jiang, J. C.
Jin, M. X.
Kajimoto, O.
Kanner, G. S.
Kim, J. S.
Kobayashi, T.
Li, H.
Li, Y.
Liang, K. K.
Lin, K. H.
Lin, S. H.
Liu, B. G.
Liu, H.
Liu, J.
Liu, J. Y.
Lou, N. Q.
Mao, H. K.
Maroncelli, M.
Mitchell, D. J.
Murakami, A.
Nakamura, S. J.
Nelson, K. A.
Nibbering, E. T. J.
Niss, K.
Novikov, V. N.
Ollivier, J.
Peyrelasse, J.
Rosker, M. J.
Saint-Guirons, H.
Schmidtke, J. P.
Schuster, G. B.
Seki, S.
Shan, Y. L.
Shiga, M.
Shiu, Y. J.
Silva, C.
Slutsky, L. J.
Sokolov, A.
Stratt, R. M.
Umebayashi, Y.
Vardeny, Z. V.
Woutersen, S.
Wu, S.
Xans, P.
Xu, D. L.
Yang, G. Q.
Yang, T. S.
Yonker, C. R.
Zewail, A. H.
Zhang, J. M.
Zhong, B.
Zhou, H.

Adv. Chem. Phys.

S. H. Lin, C. H. Chang, K. K. Liang, R. Chang, Y. J. Shiu, J. M. Zhang, T. S. Yang, M. Hayashi, and F. C. Hsu, “Ultrafast dynamics and spectroscopy of bacterial photosynthetic reaction centers,” Adv. Chem. Phys. 121, 1–88 (2002). [CrossRef]

Appl. Phys. Lett.

B. G. Liu, M. X. Jin, H. Liu, C. Y. He, D. W. Jiang, and D. Ding, “Femtosecond time-resolved measurement of LDS698 molecular processes under high pressure,” Appl. Phys. Lett. 92(24), 241916 (2008). [CrossRef]
H. Li, B. Zhong, L. M. He, G. Q. Yang, Y. Li, S. Wu, and J. Liu, “High pressure effects on the luminescent properties and structure of coumarin 153,” Appl. Phys. Lett. 80(13), 2299–2301 (2002). [CrossRef]

Discuss. Faraday Soc.

T. Förster, “Transfer mechanisms of electronic excitation,” Discuss. Faraday Soc. 27, 7–17 (1959).

J. Am. Chem. Soc.

D. J. Mitchell, G. B. Schuster, and H. G. Drickamer, “Effect of pressure on the fluorescence of 9-carbonyl substituted anthracenes,” J. Am. Chem. Soc. 99(4), 1145–1148 (1977). [CrossRef]
T. Kobayashi, M. Shiga, A. Murakami, and S. J. Nakamura, “Ab initio study of ultrafast photochemical reaction dynamics of phenol blue,” J. Am. Chem. Soc. 129(20), 6405–6424 (2007). [CrossRef] [PubMed]

J. Chem. Phys.

S. H. Lin, “Rate of interconversion of electronic and vibrational energy,” J. Chem. Phys. 44(10), 3759–3767 (1966). [CrossRef]
Y. Umebayashi, J. C. Jiang, Y. L. Shan, K. H. Lin, K. Fujii, S. Seki, S. I. Ishiguro, S. H. Lin, and H. C. Chang, “Structural change of ionic association in ionic liquid/water mixtures: a high-pressure infrared spectroscopic study,” J. Chem. Phys. 130(12), 124503 (2009). [CrossRef] [PubMed]
M. Dantus, M. J. Rosker, and A. H. Zewail, “Real-time femtosecond probing of transition-states in chemical-reactions,” J. Chem. Phys. 87(4), 2395–2397 (1987). [CrossRef]
S. H. Lin, “Effect of high pressure on molecular electronic spectra and electronic relaxation,” J. Chem. Phys. 59(8), 4458–4467 (1973). [CrossRef]

J. Phys. Chem.

D. Ducoulombier, H. Zhou, C. Boned, J. Peyrelasse, H. Saint-Guirons, and P. Xans, “Pressure (1-1000bar) and temperature (20-100oC) dependence of the viscosity of liquid hydrocarbons,” J. Phys. Chem. 90(8), 1692–1700 (1986). [CrossRef]
R. M. Stratt and M. Maroncelli, “Nonreactive dynamics in solution: the emerging molecular view of solvation dynamics and vibrational relaxation,” J. Phys. Chem. 100(31), 12981–12996 (1996). [CrossRef]

J. Phys. Chem. A

J. Y. Liu, W. H. Fan, K. L. Han, D. L. Xu, and N. Q. Lou, “Ultrafast dynamics of dye molecules in solution as a function of temperature,” J. Phys. Chem. A 107(12), 1914–1917 (2003). [CrossRef]
J. Y. Liu, W. H. Fan, K. L. Han, W. Q. Deng, D. L. Xu, and N. Q. Lou, “Ultrafast vibrational and thermal relaxation of dye molecules in solutions,” J. Phys. Chem. A 107(50), 10857–10861 (2003). [CrossRef]
J. Assmann, R. V. Benten, A. Charvat, and B. Abel, “Vibrational energy relaxation of selectively excited aromatic molecules in solution: The effect of a methyl rotor and its chemical substitution,” J. Phys. Chem. A 107(12), 1904–1913 (2003). [CrossRef]
S. Bai and C. R. Yonker, “Pressure and temperature effects on the hydrogen-bond structures of liquid and supercritical fluid methanol,” J. Phys. Chem. A 102(45), 8641–8647 (1998). [CrossRef]

J. Phys. Chem. B

N. Baden, O. Kajimoto, and K. Hara, “High-pressure studies on aggregation number of surfactant micelles using the fluorescence quenching method,” J. Phys. Chem. B 106(34), 8621–8624 (2002). [CrossRef]

Nature

S. Woutersen and H. J. Bakker, “Resonant intermolecular transfer of vibrational energy in liquid water,” Nature 402(6761), 507–509 (1999). [CrossRef]

Phys. Rev. Lett.

C. Chudoba, E. T. J. Nibbering, and T. Elsaesser, “Site-specific excited-state solute-solvent interactions probed by femtosecond vibrational spectroscopy,” Phys. Rev. Lett. 81(14), 3010–3013 (1998). [CrossRef]
K. Niss, B. Begen, B. Frick, J. Ollivier, A. Beraud, A. Sokolov, V. N. Novikov, and C. Alba-Simionesco, “Influence of pressure on the boson peak: stronger than elastic medium transformation,” Phys. Rev. Lett. 99(5), 055502 (2007). [CrossRef] [PubMed]
B. C. Hess, G. S. Kanner, Z. V. Vardeny, and G. L. Baker, “High-pressure effects on ultrafast-relaxation kinetics of excitons in polydiacetylene 4BCMU,” Phys. Rev. Lett. 66(18), 2364–2367 (1991). [CrossRef] [PubMed]
J. P. Schmidtke, J. S. Kim, J. Gierschner, C. Silva, and R. H. Friend, “Optical spectroscopy of a polyfluorene copolymer at high pressure: intra- and intermolecular interactions,” Phys. Rev. Lett. 99(16), 167401 (2007). [CrossRef] [PubMed]

Science

R. J. Hemley, P. M. Bell, and H. K. Mao, “Laser Techniques in High-Pressure Geophysics,” Science 237(4815), 605–612 (1987). [CrossRef] [PubMed]
J. M. Brown, L. J. Slutsky, K. A. Nelson, and L. T. Cheng, “Velocity of sound and equations of state for methanol and ethanol in a diamond-anvil cell,” Science 241(4861), 65–67 (1988). [CrossRef] [PubMed]

Other

H. G. Drickamer, and C. W. Frank, “Electronic transitions and the high pressure chemistry and physics of solids” (Chapman-Hall, London, 1973).

2009, Umebayashi, J. Chem. Phys.
2008, Liu, Appl. Phys. Lett.
2007, Schmidtke, Phys. Rev. Lett.
2007, Niss, Phys. Rev. Lett.
2007, Kobayashi, J. Am. Chem. Soc.
2003, Liu, J. Phys. Chem. A
2003, Liu, J. Phys. Chem. A
2003, Assmann, J. Phys. Chem. A
2002, Li, Appl. Phys. Lett.
2002, Baden, J. Phys. Chem. B
2002, Lin, Adv. Chem. Phys.
1999, Woutersen, Nature
1998, Chudoba, Phys. Rev. Lett.
1998, Bai, J. Phys. Chem. A
1996, Stratt, J. Phys. Chem.
1991, Hess, Phys. Rev. Lett.
1988, Brown, Science
1987, Hemley, Science
1987, Dantus, J. Chem. Phys.
1986, Ducoulombier, J. Phys. Chem.
1977, Mitchell, J. Am. Chem. Soc.
1973, Lin, J. Chem. Phys.
1966, Lin, J. Chem. Phys.
1959, Förster, Discuss. Faraday Soc.

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[1] S. Woutersen and H. J. Bakker, “Resonant intermolecular transfer of vibrational energy in liquid water,” Nature 402(6761), 507–509 (1999). [CrossRef]

[2] C. Chudoba, E. T. J. Nibbering, and T. Elsaesser, “Site-specific excited-state solute-solvent interactions probed by femtosecond vibrational spectroscopy,” Phys. Rev. Lett. 81(14), 3010–3013 (1998). [CrossRef]

[3] J. Assmann, R. V. Benten, A. Charvat, and B. Abel, “Vibrational energy relaxation of selectively excited aromatic molecules in solution: The effect of a methyl rotor and its chemical substitution,” J. Phys. Chem. A 107(12), 1904–1913 (2003). [CrossRef]

[4] S. H. Lin, “Rate of interconversion of electronic and vibrational energy,” J. Chem. Phys. 44(10), 3759–3767 (1966). [CrossRef]

[5] T. Kobayashi, M. Shiga, A. Murakami, and S. J. Nakamura, “Ab initio study of ultrafast photochemical reaction dynamics of phenol blue,” J. Am. Chem. Soc. 129(20), 6405–6424 (2007). [CrossRef] [PubMed]

[6] R. M. Stratt and M. Maroncelli, “Nonreactive dynamics in solution: the emerging molecular view of solvation dynamics and vibrational relaxation,” J. Phys. Chem. 100(31), 12981–12996 (1996). [CrossRef]

[7] J. Y. Liu, W. H. Fan, K. L. Han, D. L. Xu, and N. Q. Lou, “Ultrafast dynamics of dye molecules in solution as a function of temperature,” J. Phys. Chem. A 107(12), 1914–1917 (2003). [CrossRef]

[8] J. Y. Liu, W. H. Fan, K. L. Han, W. Q. Deng, D. L. Xu, and N. Q. Lou, “Ultrafast vibrational and thermal relaxation of dye molecules in solutions,” J. Phys. Chem. A 107(50), 10857–10861 (2003). [CrossRef]

[9] K. Niss, B. Begen, B. Frick, J. Ollivier, A. Beraud, A. Sokolov, V. N. Novikov, and C. Alba-Simionesco, “Influence of pressure on the boson peak: stronger than elastic medium transformation,” Phys. Rev. Lett. 99(5), 055502 (2007). [CrossRef] [PubMed]

[10] D. J. Mitchell, G. B. Schuster, and H. G. Drickamer, “Effect of pressure on the fluorescence of 9-carbonyl substituted anthracenes,” J. Am. Chem. Soc. 99(4), 1145–1148 (1977). [CrossRef]

[11] H. Li, B. Zhong, L. M. He, G. Q. Yang, Y. Li, S. Wu, and J. Liu, “High pressure effects on the luminescent properties and structure of coumarin 153,” Appl. Phys. Lett. 80(13), 2299–2301 (2002). [CrossRef]

[12] B. C. Hess, G. S. Kanner, Z. V. Vardeny, and G. L. Baker, “High-pressure effects on ultrafast-relaxation kinetics of excitons in polydiacetylene 4BCMU,” Phys. Rev. Lett. 66(18), 2364–2367 (1991). [CrossRef] [PubMed]

[13] N. Baden, O. Kajimoto, and K. Hara, “High-pressure studies on aggregation number of surfactant micelles using the fluorescence quenching method,” J. Phys. Chem. B 106(34), 8621–8624 (2002). [CrossRef]

[14] S. Bai and C. R. Yonker, “Pressure and temperature effects on the hydrogen-bond structures of liquid and supercritical fluid methanol,” J. Phys. Chem. A 102(45), 8641–8647 (1998). [CrossRef]

[15] J. P. Schmidtke, J. S. Kim, J. Gierschner, C. Silva, and R. H. Friend, “Optical spectroscopy of a polyfluorene copolymer at high pressure: intra- and intermolecular interactions,” Phys. Rev. Lett. 99(16), 167401 (2007). [CrossRef] [PubMed]

[16] Y. Umebayashi, J. C. Jiang, Y. L. Shan, K. H. Lin, K. Fujii, S. Seki, S. I. Ishiguro, S. H. Lin, and H. C. Chang, “Structural change of ionic association in ionic liquid/water mixtures: a high-pressure infrared spectroscopic study,” J. Chem. Phys. 130(12), 124503 (2009). [CrossRef] [PubMed]

[17] D. Ducoulombier, H. Zhou, C. Boned, J. Peyrelasse, H. Saint-Guirons, and P. Xans, “Pressure (1-1000bar) and temperature (20-100oC) dependence of the viscosity of liquid hydrocarbons,” J. Phys. Chem. 90(8), 1692–1700 (1986). [CrossRef]

[18] S. H. Lin, “Effect of high pressure on molecular electronic spectra and electronic relaxation,” J. Chem. Phys. 59(8), 4458–4467 (1973). [CrossRef]

[19] R. J. Hemley, P. M. Bell, and H. K. Mao, “Laser Techniques in High-Pressure Geophysics,” Science 237(4815), 605–612 (1987). [CrossRef] [PubMed]

[20] B. G. Liu, M. X. Jin, H. Liu, C. Y. He, D. W. Jiang, and D. Ding, “Femtosecond time-resolved measurement of LDS698 molecular processes under high pressure,” Appl. Phys. Lett. 92(24), 241916 (2008). [CrossRef]

[21] H. G. Drickamer, and C. W. Frank, “Electronic transitions and the high pressure chemistry and physics of solids” (Chapman-Hall, London, 1973).

[22] M. Dantus, M. J. Rosker, and A. H. Zewail, “Real-time femtosecond probing of transition-states in chemical-reactions,” J. Chem. Phys. 87(4), 2395–2397 (1987). [CrossRef]

[23] S. H. Lin, C. H. Chang, K. K. Liang, R. Chang, Y. J. Shiu, J. M. Zhang, T. S. Yang, M. Hayashi, and F. C. Hsu, “Ultrafast dynamics and spectroscopy of bacterial photosynthetic reaction centers,” Adv. Chem. Phys. 121, 1–88 (2002). [CrossRef]

[24] T. Förster, “Transfer mechanisms of electronic excitation,” Discuss. Faraday Soc. 27, 7–17 (1959).

[25] J. M. Brown, L. J. Slutsky, K. A. Nelson, and L. T. Cheng, “Velocity of sound and equations of state for methanol and ethanol in a diamond-anvil cell,” Science 241(4861), 65–67 (1988). [CrossRef] [PubMed]

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