Internuclear-distance dependence of electron correlation in nonsequential double ionization of H2
Optics Express, Vol. 18, Issue 9, pp. 9064-9070 (2010)
http://dx.doi.org/10.1364/OE.18.009064
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Abstract
Using three-dimensional classical ensembles, we have investigated the internuclear distance dependence of nonsequential double ionization (NSDI) of H2 molecules by an 800 nm, 1×1014 W/cm2 laser pulse. For the internuclear distance R ranging from 2 to 12 a.u., the NSDI of H2 provides rich correlation patterns in the two-electron momentum distributions. These correlation patterns essentially reveal different microscopic dynamics in NSDI process. Moreover, our calculations show that R ≈ 4 a.u. is the critical distance for double ionization yield of H2. These results are qualitatively explained based on the classical barrier expression model and back analysis.
© 2010 Optical Society of America
OCIS Codes
(020.4180) Atomic and molecular physics : Multiphoton processes
(260.3230) Physical optics : Ionization
(270.6620) Quantum optics : Strong-field processes
ToC Category:
Atomic and Molecular Physics
History
Original Manuscript: February 25, 2010
Revised Manuscript: March 28, 2010
Manuscript Accepted: April 14, 2010
Published: April 15, 2010
Citation
Aihong Tong, Qing Liao, Yueming Zhou, and Peixiang Lu, "Internuclear-distance dependence of electron correlation in nonsequential double ionization of H2," Opt. Express 18, 9064-9070 (2010)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-18-9-9064
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References
- D. N. Fittinghoff, P. R. Bolton, B. Chang, and K. C. Kulander, "Observation of nonsequential double ionization of helium with optical tunneling," Phys. Rev. Lett. 69,2642-2645 (1992). [CrossRef] [PubMed]
- P. B. Corkum, "Plasma perspective on strong field multiphoton ionization," Phys. Rev. Lett. 71,1994-1997 (1993). [CrossRef] [PubMed]
- M. Lein, E. K. U. Gross, and V. Engel, "Intense-Field Double Ionization of Helium: identifying the Mechanism," Phys. Rev. Lett. 85, 4707-4710 (2000). [CrossRef] [PubMed]
- A. S. Alnaser, T. Osipov, E. P. Benis, A. Wech, B. Shan, C. L. Cocke, X. M. Tong, and C. D. Lin, "Rescattering double ionization of D2 and H2 by intense laser pulses," Phys. Rev. Lett. 91,163002 (2003). [CrossRef] [PubMed]
- S. Saugout and C. Cornaggia, "Temporal separation of H2 double-ionization channels using intense ultrashort 10-fs laser pulses," Phys. Rev. A. 73,041406(R) (2006). [CrossRef]
- Q. Liao, P. Lu, Q. Zhang, Z. Yang, and X. Wang, "Double ionization of HeH+ molecules in intense laser fields," Opt. Express 16,17070-17075 (2008). [CrossRef] [PubMed]
- T. Zuo and A. D. Bandrauk, "Charge-resonance-enhanced ionization of diatomic molecular ions by intense lasers," Phys. Rev. A. 52, R2511-R2514 (1996). [CrossRef]
- S. Saugout, "H2 double ionization with few-cycle laser pulses," Phys. Rev. A. 77, 023404 (2008). [CrossRef]
- G. N. Gibson, M. Li, C. Guo, and J. Neira, "Strong-field dissociation and ionization of H+ 2 using ultrashort laser pulses," Phys. Rev. Lett. 79, 2022-2025 (1997). [CrossRef]
- C. Trump, H. Rottke, M. Wittmann, G. Korn, W. Sandner, M. Lein, and V. Engel, "Pulse-width and isotope effects in femtosecond-pulse strong-field dissociation of H+ 2 and D+2, " Phys. Rev. A. 62, 063402 (2000). [CrossRef]
- H. Yu, T. Zuo, and A. D. Bandrauk, "Molecules in intense laser fields: enhanced ionization in a one-dimensional model of H2," Phys. Rev. A. 54, 3290-3298 (1996). [CrossRef] [PubMed]
- A. Saenz, "Enhanced ionization of molecular hydrogen in very strong fields," Phys. Rev. A. 61, 051402 (2000). [CrossRef]
- X. M. Tong, Z. X. Zhao, and C. D. Lin, "Probing molecular dynamics at attosecond resolution with femtosecond laser pulses," Phys. Rev. Lett. 91, 233203 (2003). [CrossRef] [PubMed]
- A. S. Alnaser, X. M. Tong, T. Osipov, S. Voss, C. M. Maharjan, P. Ranitovic, B. Ulrich, B. Shan, Z. Chang, C. D. Lin, and C. L. Cocke, "Routes to control of H2 coulomb explosion in few-cycle laser pulses," Phys. Rev. Lett. 93, 183202 (2004). [CrossRef] [PubMed]
- K. Codling, L. J. Frasinski, and P. A. Hatherly, "On the field ionisation of diatomic molecules by intense laser fields," J.Phys.B 22, L321-L327 (1989). [CrossRef]
- S. L. Haan, L. Breen, A. Karim, and J. H. Eberly, "Variable time lag and backward ejection in full-dimensional analysis of strong-field double ionization," Phys. Rev. Lett. 97, 103008 (2006). [CrossRef] [PubMed]
- S. L. Haan, L. Breen, A. Karim, and J. H. Eberly, "Recollision dynamics and time delay in strong-field double ionization," Opt. Express 15, 767-778 (2007). [CrossRef] [PubMed]
- S. L. Haan, J. S. Van Dyke, and Z. S. Smith, "Recollision excitation, electron correlation, and the production of high-momentum electrons in double ionization," Phys. Rev. Lett. 101, 113001 (2008). [CrossRef] [PubMed]
- S. L. Haan, Z.S. Smith, K. N. Shomsky, and P. W. Plantinga, "Electron drift directions in strong-field double ionization of atoms," J. Phys. B 42, 134009 (2009). [CrossRef]
- Q. Liao and P. Lu, "Manipulating nonsequential double ionization via alignment of asymmetric molecules," Opt. Express 17,15550-15557 (2009). [CrossRef] [PubMed]
- Y. Zhou, Q. Liao, and P. Lu, "Mechanism for high-energy electrons in nonsequential double ionization below the recollision-excitation threshold, " Phys. Rev. A. 80, 023412 (2009). [CrossRef]
- T.-T. Nguyen-Dang, F. Chateauneuf, and S. Manoli, "Tunnel ionization of H2 in a low-frequency laser field: a wave-packet approach," Phys. Rev. A. 56, 2142-2167 (1997). [CrossRef]
- R. Panfili and J. H. Eberly, "Comparing classical and quantum dynamics of strong-field double ionization," Opt. Express 8,431-435 (2001). [CrossRef] [PubMed]
- J. Chen and C. H. Nam, "Ion momentum distributions for He single and double ionization in strong laser fields," Phys. Rev. A. 66, 053415 (2002). [CrossRef]
- A. Staudte, C. Ruiz, M. Schoffler, S. Schossler, D. Zeidler, Th. Weber, M. Meckel, D. M. Villeneuve, P. B. Corkum, A. Becker, and R. Dorner, "Binary and recoil collisions in strong field double ionization of Helium," Phys. Rev. Lett. 99, 263002 (2007). [CrossRef]
- Th. Weber, H. Giessen, M. Weckenbrock, G. Urbasch, A. Staudte, L. Spielberger, O. Jagutzki, V. Mergel, M. Vollmer, and R. Dorner, "Correlated electron emission in multiphoton double ionization," Nature 405, 658-661 (2000). [CrossRef] [PubMed]
- B. Feuerstein, R. Moshammer, D. Fischer, A. Dorn, C. D. Schroter, J. Deipenwisch, J. R. Crespo Lopez-Urrutia, C. Hohr, P. Neumayer, J. Ullrich, H. Rottke, C. Trump, M. Wittmann, G. Korn, and W. Sandner, "Separation of recollision mechanisms in nonsequential strong field double ionization of Ar: the role of excitation tunneling," Phys. Rev. Lett. 87, 043003 (2001). [CrossRef] [PubMed]
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