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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 19, Iss. 23 — Nov. 7, 2011
  • pp: 22486–22495

Off-resonance and non-resonant dispersion of Kerr nonlinearity for symmetric molecules [Invited]

George Stegeman, Mark G. Kuzyk, Dimitris G. Papazoglou, and Stelios Tzortzakis  »View Author Affiliations


Optics Express, Vol. 19, Issue 23, pp. 22486-22495 (2011)
http://dx.doi.org/10.1364/OE.19.022486


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Abstract

The exact formula is derived from the “sum over states” (SOS) quantum mechanical model for the frequency dispersion of the nonlinear refractive index coefficient n2 for centrosymmetric molecules in the off-resonance and non-resonant regimes. This expression is characterized by interference between terms from two-photon transitions from the ground state to the even-symmetry excited states and one-photon transitions between the ground state and odd-symmetry excited states. When contributions from the two-photon terms exceed those from the one-photon terms, the non-resonant intensity-dependent refractive index n2>0, and vice versa. Examples of the frequency dispersion for the three-level SOS model are given. Comparison is made with other existing theories.

© 2011 OSA

OCIS Codes
(190.0190) Nonlinear optics : Nonlinear optics
(190.3270) Nonlinear optics : Kerr effect
(190.5940) Nonlinear optics : Self-action effects

ToC Category:
Nonlinear Absorption and Dispersion

History
Original Manuscript: August 30, 2011
Revised Manuscript: September 27, 2011
Manuscript Accepted: October 5, 2011
Published: October 25, 2011

Virtual Issues
Nonlinear Optics (2011) Optical Materials Express

Citation
George Stegeman, Mark G. Kuzyk, Dimitris G. Papazoglou, and Stelios Tzortzakis, "Off-resonance and non-resonant dispersion of Kerr nonlinearity for symmetric molecules [Invited]," Opt. Express 19, 22486-22495 (2011)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-19-23-22486


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