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Beating spatio-temporal coupling: implications for pulse shaping and coherent control experimentsDaan Brinks, Richard Hildner, Fernando D. Stefani, and Niek F. van Hulst »View Author Affiliations
Daan Brinks,1
Richard Hildner,1,2
Fernando D. Stefani,1,3
and Niek F. van Hulst1,4
1ICFO—Institut de Ciencies Fotoniques, Mediterranean Technology Park, 08860 Castelldefels (Barcelona), Spain 2Currently with Experimentalphysik IV, Universität Bayreuth, 95440 Bayreuth, Germany 3Currently with Departamento de Física & Instituto de Física de Buenos Aires (IFIBA, CONICET), Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, 1438 Buenos Aires, Argentina 4ICREA—Institució Catalana de Recerca i Estudis Avançats, 08015 Barcelona, Spain *Corresponding author: daan.brinks@icfo.es |
Optics Express, Vol. 19, Issue 27, pp. 26486-26499 (2011)
http://dx.doi.org/10.1364/OE.19.026486
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Abstract
Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.
© 2011 OSA
OCIS Codes
(020.1670) Atomic and molecular physics : Coherent optical effects
(120.4820) Instrumentation, measurement, and metrology : Optical systems
(320.2250) Ultrafast optics : Femtosecond phenomena
(320.5540) Ultrafast optics : Pulse shaping
(320.7100) Ultrafast optics : Ultrafast measurements
(320.7160) Ultrafast optics : Ultrafast technology
ToC Category:
Ultrafast Optics
History
Original Manuscript: October 21, 2011
Revised Manuscript: November 28, 2011
Manuscript Accepted: November 28, 2011
Published: December 13, 2011
Citation
Daan Brinks, Richard Hildner, Fernando D. Stefani, and Niek F. van Hulst, "Beating spatio-temporal coupling: implications for pulse shaping and coherent control experiments," Opt. Express 19, 26486-26499 (2011)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-19-27-26486
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- T. Brixner and G. Gerber, “Femtosecond polarization pulse shaping,” Opt. Lett.26(8), 557–559 (2001). [CrossRef] [PubMed]
- A. Assion, T. Baumert, M. Bergt, T. Brixner, B. Kiefer, V. Seyfried, M. Strehle, and G. Gerber, “Control of chemical reactions by feedback-optimized phase-shaped femtosecond laser pulses,” Science282(5390), 919–922 (1998). [CrossRef] [PubMed]
- V. I. Prokhorenko, A. M. Nagy, S. A. Waschuk, L. S. Brown, R. R. Birge, and R. J. D. Miller, “Coherent control of retinal isomerization in bacteriorhodopsin,” Science313(5791), 1257–1261 (2006). [CrossRef] [PubMed]
- E. Collini, C. Y. Wong, K. E. Wilk, P. M. G. Curmi, P. Brumer, and G. D. Scholes, “Coherently wired light-harvesting in photosynthetic marine algae at ambient temperature,” Nature463(7281), 644–647 (2010). [CrossRef] [PubMed]
- G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mancal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007). [CrossRef] [PubMed]
- D. J. McCabe, D. R. Austin, A. Tajalli, S. Weber, I. A. Walmsley, and B. Chatel, “Space–time coupling of shaped ultrafast ultraviolet pulses from an acousto-optic programmable dispersive filter,” J. Opt. Soc. Am. B28(1), 58–64 (2011). [CrossRef]
- A. Monmayrant, S. Weber, and B. Chatel, “A newcomer’s guide to ultrashort pulse shaping and characterization,” J. Phys. At. Mol. Opt. Phys.43(10), 103001 (2010). [CrossRef]
- G. S. Engel, T. R. Calhoun, E. L. Read, T.-K. Ahn, T. Mancal, Y.-C. Cheng, R. E. Blankenship, and G. R. Fleming, “Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems,” Nature446(7137), 782–786 (2007). [CrossRef] [PubMed]
- W. Min, S. Lu, S. Chong, R. Roy, G. R. Holtom, and X. S. Xie, “Imaging chromophores with undetectable fluorescence by stimulated emission microscopy,” Nature461(7267), 1105–1109 (2009). [CrossRef] [PubMed]
- J. L. Herek, W. Wohlleben, R. J. Cogdell, D. Zeidler, and M. Motzkus, “Quantum control of energy flow in light harvesting,” Nature417(6888), 533–535 (2002). [CrossRef] [PubMed]
- E. Collini, C. Y. Wong, K. E. Wilk, P. M. G. Curmi, P. Brumer, and G. D. Scholes, “Coherently wired light-harvesting in photosynthetic marine algae at ambient temperature,” Nature463(7281), 644–647 (2010). [CrossRef] [PubMed]
- E. Collini, C. Y. Wong, K. E. Wilk, P. M. G. Curmi, P. Brumer, and G. D. Scholes, “Coherently wired light-harvesting in photosynthetic marine algae at ambient temperature,” Nature463(7281), 644–647 (2010). [CrossRef] [PubMed]
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