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Saturation behaviour of colloidal PbSe quantum dot exciton emission coupled into silicon photonic circuitsCharles A. Foell, Ellen Schelew, Haijun Qiao, Keith A. Abel, Stephen Hughes, Frank C. J. M. van Veggel, and Jeff F. Young »View Author Affiliations
Charles A. Foell,1
Ellen Schelew,1
Haijun Qiao,1,2
Keith A. Abel,3
Stephen Hughes,4
Frank C. J. M. van Veggel,3
and Jeff F. Young1,*
1Department of Physics and Astronomy, University of British Columbia, 6224 Agricultural Rd., Vancouver, B.C., V6T 1Z1, Canada 2Current address: Department of Chemistry, Simon Fraser University, Burnaby, B.C., V5A 1S6, Canada 3Department of Chemistry, University of Victoria, Victoria, B.C., V8W 3V6, Canada 4Department of Physics, Engineering Physics, and Astronomy, Queen’s University, Kingston, ON, K7L 3N6, Canada *Corresponding author: young@physics.ubc.ca |
Optics Express, Vol. 20, Issue 10, pp. 10453-10469 (2012)
http://dx.doi.org/10.1364/OE.20.010453
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Abstract
We report coupling of the excitonic photon emission from photoexcited PbSe colloidal quantum dots (QDs) into an optical circuit that was fabricated in a silicon-on-insulator wafer using a CMOS-compatible process. The coupling between excitons and sub-μm sized silicon channel waveguides was mediated by a photonic crystal microcavity. The intensity of the coupled light saturates rapidly with the optical excitation power. The saturation behaviour was quantitatively studied using an isolated photonic crystal cavity with PbSe QDs site-selectively located at the cavity mode antinode position. Saturation occurs when a few μW of continuous wave HeNe pump power excites the QDs with a Gaussian spot size of 2 μm. By comparing the results with a master equation analysis that rigorously accounts for the complex dielectric environment of the QD excitons, the saturation is attributed to ground state depletion due to a non-radiative exciton decay channel with a trap state lifetime ∼ 3 μs.
© 2012 OSA
OCIS Codes
(230.3120) Optical devices : Integrated optics devices
(230.5590) Optical devices : Quantum-well, -wire and -dot devices
(270.5580) Quantum optics : Quantum electrodynamics
(350.4238) Other areas of optics : Nanophotonics and photonic crystals
ToC Category:
Materials for Integrated Optics
History
Original Manuscript: January 23, 2012
Revised Manuscript: February 24, 2012
Manuscript Accepted: February 27, 2012
Published: April 20, 2012
Virtual Issues
Quantum Dots for Photonic Applications (2012) Optical Materials Express
Citation
Charles A. Foell, Ellen Schelew, Haijun Qiao, Keith A. Abel, Stephen Hughes, Frank C. J. M. van Veggel, and Jeff F. Young, "Saturation behaviour of colloidal PbSe quantum dot exciton emission
coupled into silicon photonic circuits," Opt. Express 20, 10453-10469 (2012)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-20-10-10453
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