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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 20, Iss. 25 — Dec. 3, 2012
  • pp: 27959–27965

High-order Raman sidebands generated from the near-infrared to ultraviolet region by four-wave Raman mixing of hydrogen using an ultrashort two-color pump beam

Osamu Shitamichi and Totaro Imasaka  »View Author Affiliations


Optics Express, Vol. 20, Issue 25, pp. 27959-27965 (2012)
http://dx.doi.org/10.1364/OE.20.027959


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Abstract

A two-color pump beam consisting of a fundamental beam of a Ti:sapphire laser (35 fs, 802 nm) and a signal beam generated by optical parametric amplification (55 fs, 1203 nm) was utilized to generate multiple Raman sidebands by vibrational four-wave Raman mixing. The second harmonic emission (401 nm) was further employed as a seed beam for enhancing efficiency. Numerous sidebands emitting at 602, 481, 344, 301, 267, 241, 219, 200, and 185 nm were observed by irradiating the beam onto a screen coated with sodium salicylate. The spectral band width of these emission lines was capable of generating 0.9-fs optical pulses by Fourier synthesis.

© 2012 OSA

OCIS Codes
(190.4380) Nonlinear optics : Nonlinear optics, four-wave mixing
(290.5910) Scattering : Scattering, stimulated Raman
(320.7110) Ultrafast optics : Ultrafast nonlinear optics

ToC Category:
Nonlinear Optics

History
Original Manuscript: October 10, 2012
Revised Manuscript: November 13, 2012
Manuscript Accepted: November 16, 2012
Published: November 30, 2012

Citation
Osamu Shitamichi and Totaro Imasaka, "High-order Raman sidebands generated from the near-infrared to ultraviolet region by four-wave Raman mixing of hydrogen using an ultrashort two-color pump beam," Opt. Express 20, 27959-27965 (2012)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-20-25-27959


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References

  1. T. Imasaka, S. Kawasaki, and N. Ishibashi, “Generation of more than 40 laser emission lines from the ultraviolet to the visible regions by two-color stimulated Raman effect,” Appl. Phys. B49(4), 389–392 (1989). [CrossRef]
  2. H. Kawano, Y. Hirakawa, and T. Imasaka, “Generation of more than 40 rotational Raman lines by picosecond and femtosecond Ti:sapphire laser for Fourier synthesis,” Appl. Phys. B65(1), 1–4 (1997). [CrossRef]
  3. S. Yoshikawa and T. Imasaka, “A new approach for the generation of ultrashort optical pulses,” Opt. Commun.96(1-3), 94–98 (1993). [CrossRef]
  4. A. Nazarkin, G. Korn, M. Wittmann, and T. Elsaesser, “Generation of multiple phase-locked Stokes and anti-Stokes components in an impulsively excited Raman medium,” Phys. Rev. Lett.83(13), 2560–2563 (1999). [CrossRef]
  5. M. Wittmann, A. Nazarkin, and G. Korn, “fs-pulse synthesis using phase modulation by impulsively excited molecular vibrations,” Phys. Rev. Lett.84(24), 5508–5511 (2000). [CrossRef] [PubMed]
  6. M. Wittmann, A. Nazarkin, and G. Korn, “Synthesis of periodic femtosecond pulse trains in the ultraviolet by phase-locked Raman sideband generation,” Opt. Lett.26(5), 298–300 (2001). [CrossRef] [PubMed]
  7. N. Zhavoronkov and G. Korn, “Generation of single intense short optical pulses by ultrafast molecular phase modulation,” Phys. Rev. Lett.88, 203901 (2002).
  8. Y. Kida, T. Nagahara, S. Zaitsu, M. Matuse, and T. Imasaka, “Pulse compression based on coherent molecular motion induced by transient stimulated Raman scattering,” Opt. Express14(7), 3083–3092 (2006). [CrossRef] [PubMed]
  9. Y. Kida, S. Zaitsu, and T. Imasaka, “Generation of intense 11-fs ultraviolet pulses using phase modulation by two types of coherent molecular motions,” Opt. Express16(18), 13492–13498 (2008). [CrossRef] [PubMed]
  10. N. Yasaka, Y. Kida, S. Zaitsu, and T. Imasaka, “Generation of high-order rotational Raman sidebands in the deep-ultraviolet region using molecular phase modulation induced by an intensity-modulated optical pulse,” J. App. Phys.108, 056104 (2010).
  11. V. Krylov, A. Rebane, O. Ollikainen, D. Erni, U. Wild, V. Bespalov, and D. Staselko, “Stimulated Raman scattering in hydrogen by frequency-doubled amplified femtosecond Ti:sapphire laser pulses,” Opt. Lett.21(6), 381–383 (1996). [CrossRef] [PubMed]
  12. E. Sali, K. J. Mendham, J. W. G. Tisch, T. Halfmann, and J. P. Marangos, “High-order stimulated Raman scattering in a highly transient regime driven by a pair of ultrashort pulses,” Opt. Lett.29(5), 495–497 (2004). [CrossRef] [PubMed]
  13. E. Sali, P. Kinsler, G. H. C. New, K. J. Mendham, T. Halfmann, J. W. G. Tisch, and J. P. Marangos, “Behavior of high-order stimulated Raman scattering in a highly transient regime,” Phys. Rev. A72(1), 013813 (2005). [CrossRef]
  14. F. C. Turner, A. Trottier, D. Strickland, and L. L. Losev, “Transient multi-frequency Raman generation in SF6,” Opt. Commun.270(2), 419–423 (2007). [CrossRef]
  15. . C. Turner and D. Strickland, “Anti-Stokes enhancement of multifrequency Raman generation in a hollow fiber,” Opt. Lett.33(4), 405 (2008) [CrossRef] [PubMed]
  16. D. D. Yavuz, D. R. Walker, M. Y. Shverdin, G. Y. Yin, and S. E. Harris, “Quasiperiodic Raman technique for ultrashort pulse generation,” Phys. Rev. Lett.91(23), 233602 (2003). [CrossRef] [PubMed]
  17. M. Katsuragawa, K. Yokoyama, T. Onose, and K. Misawa, “Generation of a 10.6-THz ultrahigh-repetition-rate train by synthesizing phase-coherent Raman-sidebands,” Opt. Express13(15), 5628–5634 (2005). [CrossRef] [PubMed]
  18. W.-J. Chen, Z.-M. Hsieh, S. W. Huang, H.-Y. Su, C.-J. Lai, T.-T. Tang, C.-H. Lin, C.-K. Lee, R.-P. Pan, C.-L. Pan, and A. H. Kung, “Sub-single-cycle optical pulse train with constant carrier envelope phase,” Phys. Rev. Lett.100(16), 163906 (2008). [CrossRef] [PubMed]
  19. H.-S. Chan, Z.-M. Hsieh, W.-H. Liang, A. H. Kung, C.-K. Lee, C.-J. Lai, R.-P. Pan, and L.-H. Peng, “Synthesis and measurement of ultrafast waveforms from five discrete optical harmonics,” Science331(6021), 1165–1168 (2011). [CrossRef] [PubMed]
  20. R. Trebino, Frequency-Resolved Optical Gating: The Measurement of Ultrashort Laser Pulses (Kluwer Academic Publishers, 2002).
  21. S.-I. Zaitsu, Y. Miyoshi, F. Kira, S. Yamaguchi, T. Uchimura, and T. Imasaka, “Interferometric characterization of ultrashort deep ultraviolet pulses using a multiphoton ionization mass spectrometer,” Opt. Lett.32(12), 1716–1718 (2007). [CrossRef] [PubMed]
  22. Y. Miyoshi, S. Zaitsu, and T. Imasaka, “In situ third-order interferometric autocorrelation of a femtosecond deep-ultraviolet pulse,” Appl. Phys. B103(4), 789–794 (2011). [CrossRef]
  23. T. Imasaka and T. Imasaka, “Searching for a molecule with a wide frequency domain for non-resonant two-photon ionization to measure the ultrashort optical pulse width,” Opt. Commun.285(16), 3514–3518 (2012). [CrossRef]

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