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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 20, Iss. 3 — Jan. 30, 2012
  • pp: 3118–3128

Mixed two- and three-photon absorption in bulk rutile (TiO2) around 800 nm

Christopher C. Evans, Jonathan D. B. Bradley, Erwin A. Martí-Panameño, and Eric Mazur  »View Author Affiliations


Optics Express, Vol. 20, Issue 3, pp. 3118-3128 (2012)
http://dx.doi.org/10.1364/OE.20.003118


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Abstract

We observe mixed two- and three-photon absorption in bulk rutile (TiO2) around 800 nm using the open aperture Z-scan technique. We fit the data with an extended model that includes multiphoton absorption, beam quality, and ellipticity. The extracted two- and three-photon absorption coefficients are below 1 mm/GW and 2 mm3/GW2, respectively. We observe negligible two-photon absorption for 813-nm light polarized along the extraordinary axis. We measure the nonlinear index of refraction and obtain two-photon nonlinear figures of merit greater than 1.1 at 774 nm and greater than 12 at 813 nm. Similarly, we obtain three-photon figures of merit that allow operational intensities up to 0.57 GW/mm2. We conclude that rutile is a promising material for all-optical switching applications around 800 nm.

© 2012 OSA

OCIS Codes
(190.4180) Nonlinear optics : Multiphoton processes
(190.4400) Nonlinear optics : Nonlinear optics, materials
(320.2250) Ultrafast optics : Femtosecond phenomena
(320.7130) Ultrafast optics : Ultrafast processes in condensed matter, including semiconductors
(200.6715) Optics in computing : Switching

ToC Category:
Ultrafast Optics

History
Original Manuscript: December 15, 2011
Revised Manuscript: January 20, 2012
Manuscript Accepted: January 20, 2012
Published: January 25, 2012

Citation
Christopher C. Evans, Jonathan D. B. Bradley, Erwin A. Martí-Panameño, and Eric Mazur, "Mixed two- and three-photon absorption in bulk rutile (TiO2) around 800 nm," Opt. Express 20, 3118-3128 (2012)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-20-3-3118


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