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Optics Express

Optics Express

  • Editor: C. Martijn de Sterke
  • Vol. 20, Iss. 9 — Apr. 23, 2012
  • pp: 10042–10058

Optical properties of light absorbing carbon aggregates mixed with sulfate: assessment of different model geometries for climate forcing calculations

Michael Kahnert, Timo Nousiainen, Hannakaisa Lindqvist, and Martin Ebert  »View Author Affiliations


Optics Express, Vol. 20, Issue 9, pp. 10042-10058 (2012)
http://dx.doi.org/10.1364/OE.20.010042


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Abstract

Light scattering by light absorbing carbon (LAC) aggregates encapsulated into sulfate shells is computed by use of the discrete dipole method. Computations are performed for a UV, visible, and IR wavelength, different particle sizes, and volume fractions. Reference computations are compared to three classes of simplified model particles that have been proposed for climate modeling purposes. Neither model matches the reference results sufficiently well. Remarkably, more realistic core-shell geometries fall behind homogeneous mixture models. An extended model based on a core-shell-shell geometry is proposed and tested. Good agreement is found for total optical cross sections and the asymmetry parameter.

© 2012 OSA

OCIS Codes
(010.1110) Atmospheric and oceanic optics : Aerosols
(010.1290) Atmospheric and oceanic optics : Atmospheric optics
(010.1310) Atmospheric and oceanic optics : Atmospheric scattering
(290.1350) Scattering : Backscattering
(290.5850) Scattering : Scattering, particles
(290.5825) Scattering : Scattering theory

ToC Category:
Atmospheric and Oceanic Optics

History
Original Manuscript: February 22, 2012
Revised Manuscript: April 12, 2012
Manuscript Accepted: April 12, 2012
Published: April 18, 2012

Citation
Michael Kahnert, Timo Nousiainen, Hannakaisa Lindqvist, and Martin Ebert, "Optical properties of light absorbing carbon aggregates mixed with sulfate: assessment of different model geometries for climate forcing calculations," Opt. Express 20, 10042-10058 (2012)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-20-9-10042


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