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Optics Express

Optics Express

  • Editor: Andrew M. Weiner
  • Vol. 22, Iss. 14 — Jul. 14, 2014
  • pp: 16965–16975

100-kHz shot-to-shot broadband data acquisition for high-repetition-rate pump–probe spectroscopy

Florian Kanal, Sabine Keiber, Reiner Eck, and Tobias Brixner  »View Author Affiliations


Optics Express, Vol. 22, Issue 14, pp. 16965-16975 (2014)
http://dx.doi.org/10.1364/OE.22.016965


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Abstract

Shot-to-shot broadband detection is common in ultrafast pump–probe spectroscopy. Taking advantage of the intensity correlation of subsequent laser pulses improves the signal-to-noise ratio. Finite data readout times of CCD chips in the employed spectrometer and the maximum available speed of mechanical pump-beam choppers typically limit this approach to lasers with repetition rates of a few kHz. For high-repetition (≥ 100 kHz) systems, one typically averages over a larger number of laser shots leading to inferior signal-to-noise ratios or longer measurement times. Here we demonstrate broadband shot-to-shot detection in transient absorption spectroscopy with a 100-kHz femtosecond laser system. This is made possible using a home-built high-speed chopper with external laser synchronization and a fast CCD line camera. Shot-to-shot detection can reduce the data acquisition time by two orders of magnitude compared to few-kHz lasers while keeping the same signal-to-noise ratio.

© 2014 Optical Society of America

OCIS Codes
(040.1490) Detectors : Cameras
(040.1520) Detectors : CCD, charge-coupled device
(230.4110) Optical devices : Modulators
(300.6500) Spectroscopy : Spectroscopy, time-resolved
(300.6530) Spectroscopy : Spectroscopy, ultrafast
(320.7100) Ultrafast optics : Ultrafast measurements

ToC Category:
Instrumentation, Measurement, and Metrology

History
Original Manuscript: March 26, 2014
Revised Manuscript: May 9, 2014
Manuscript Accepted: May 19, 2014
Published: July 3, 2014

Virtual Issues
Vol. 9, Iss. 9 Virtual Journal for Biomedical Optics

Citation
Florian Kanal, Sabine Keiber, Reiner Eck, and Tobias Brixner, "100-kHz shot-to-shot broadband data acquisition for high-repetition-rate pump–probe spectroscopy," Opt. Express 22, 16965-16975 (2014)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-22-14-16965


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References

  1. A. H. Zewail, “Femtochemistry: atomic-scale dynamics of the chemical bond,” J. Phys. Chem. A 104, 5660–5694 (2000). [CrossRef]
  2. T. Polack, “Spectroscopie infrarouge impulsionnelle appliquee au transfert de ligands dans les hémoprotéines,” Ph.D. thesis, École Polytechnique, Paris (2003).
  3. T. Polack, J. P. Ogilvie, S. Franzen, M. H. Vos, M. Joffre, J.-L. Martin, and A. Alexandrou, “CO vibration as a probe of ligand dissociation and transfer in myoglobin,” Phys. Rev. Lett. 93, 018102 (2004). [CrossRef] [PubMed]
  4. G. Auböck, C. Consani, R. Monni, A. Cannizzo, F. v. Mourik, and M. Chergui, “Femtosecond pump/supercontinuum-probe setup with 20 kHz repetition rate,” Rev. Sci. Instrum. 83, 093105 (2012). [CrossRef] [PubMed]
  5. P. Tournois, “Acousto-optic programmable dispersive filter for adaptive compensation of group delay time dispersion in laser systems,” Opt. Commun. 140, 245–249 (1997). [CrossRef]
  6. J. Buback, M. Kullmann, F. Langhojer, P. Nuernberger, R. Schmidt, F. Würthner, and T. Brixner, “Ultrafast bidirectional photoswitching of a spiropyran,” J. Am. Chem. Soc. 132, 16510–16519 (2010). [CrossRef] [PubMed]
  7. U. Megerle, I. Pugliesi, C. Schriever, C. Sailer, and E. Riedle, “Sub-50 fs broadband absorption spectroscopy with tunable excitation: Putting the analysis of ultrafast molecular dynamics on solid ground,” Appl. Phys. B 96, 215–231 (2009). [CrossRef]
  8. S. D. McClure, D. B. Turner, P. C. Arpin, T. Mirkovic, and G. D. Scholes, “Coherent oscillations in the PC577 cryptophyte antenna occur in the excited electronic state,” J. Phys. Chem. B 118, 1296–1308 (2014). [CrossRef] [PubMed]
  9. J. Piel, E. Riedle, L. Gundlach, R. Ernstorfer, and R. Eichberger, “Sub-20 fs visible pulses with 750 nJ energy from a 100 kHz noncollinear optical parametric amplifier,” Opt. Lett. 31, 1289–1291 (2006). [CrossRef] [PubMed]
  10. A. Yabushita, Y.-H. Lee, and T. Kobayashi, “Development of a multiplex fast-scan system for ultrafast time-resolved spectroscopy,” Rev. Sci. Instrum. 81, 063110 (2010). [CrossRef] [PubMed]
  11. M. J. Feldstein, P. Vöhringer, and N. F. Scherer, “Rapid-scan pump-probe spectroscopy with high time and wavenumber resolution: optical-Kerr-effect measurements of neat liquids,” J. Opt. Soc. Am. B 12, 1500–1510 (1995). [CrossRef]
  12. K. F. Lee, A. Bonvalet, P. Nuernberger, and M. Joffre, “Unobtrusive interferometer tracking by path length oscillation for multidimensional spectroscopy,” Opt. Express 17, 12379–12384 (2009). [CrossRef] [PubMed]
  13. Y. H. Meyer, M. Pittman, and P. Plaza, “Transient absorption of symmetrical carbocyanines,” J. Photochem. Photobiol. A 114, 1–21 (1998). [CrossRef]
  14. D. Wang, H. Jiang, H. Yang, C. Liu, Q. Gong, J. Xiang, and G. Xu, “Investigation on photoexcited dynamics of IR-140 dye in ethanol by femtosecond supercontinuum-probing technique,” J. Opt. A: Pure Appl. Opt. 4, 155–159 (2002). [CrossRef]
  15. D. Wang, H. Jiang, S. Wu, H. Yang, Q. Gong, J. Xiang, and G. Xu, “An investigation of solvent effects on the optical properties of dye IR-140 using the pump supercontinuum-probing technique,” J. Opt. A: Pure Appl. Opt. 5, 515–519 (2003). [CrossRef]
  16. M. Bradler, P. Baum, and E. Riedle, “Femtosecond continuum generation in bulk laser host materials with sub-μJ pump pulses,” Appl. Phys. B 97, 561–574 (2009). [CrossRef]
  17. I. H. M. van Stokkum, D. S. Larsen, and R. van Grondelle, “Global and target analysis of time-resolved spectra,” Biochim. Biophys. Acta, Bioenerg. 1657, 82–104 (2004). [CrossRef]
  18. J. J. Snellenburg, S. P. Laptenok, R. Seger, K. M. Mullen, and I. H. M. van Stokkum, “Glotaran: a Java-based Graphical User Interface for the R-package TIMP,” J. Stat. Softw. 49, 1–22 (2012).
  19. K. M. Mullen and I. H. M. van Stokkum, “TIMP: an R package for modeling multi-way spectroscopic measurements,” J. Stat. Softw. 18, 1–46 (2007).
  20. C. Schriever, S. Lochbrunner, E. Riedle, and D. J. Nesbitt, “Ultrasensitive ultraviolet-visible 20 fs absorption spectroscopy of low vapor pressure molecules in the gas phase,” Rev. Sci. Instrum. 79, 013107 (2008). [CrossRef]
  21. D. Polli, L. Lüer, and G. Cerullo, “High-time-resolution pump-probe system with broadband detection for the study of time-domain vibrational dynamics,” Rev. Sci. Instrum. 78, 103108 (2007). [CrossRef] [PubMed]
  22. D. Linde, “Characterization of the noise in continuously operating mode-locked lasers,” Appl. Phys. B 39, 201–217 (1986). [CrossRef]

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