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Optics Express

Optics Express

  • Editor: Andrew M. Weiner
  • Vol. 22, Iss. 3 — Feb. 10, 2014
  • pp: 3117–3127

Study on the productivity of silicon nanoparticles by picosecond laser ablation in water: towards gram per hour yield

Romuald Intartaglia, Komal Bagga, and Fernando Brandi  »View Author Affiliations


Optics Express, Vol. 22, Issue 3, pp. 3117-3127 (2014)
http://dx.doi.org/10.1364/OE.22.003117


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Abstract

An investigation on the productivity of silicon nanoparticles by picosecond laser ablation in water is presented. A systematic experimental study is performed as function of the laser wavelength, fluence and ablation time. In case of ablation at 1064 nm silicon nanoparticles with a mean diameter of 40 nm are produced. Instead, ablation at 355 nm results in nanoparticles with a mean diameter of 9 nm for short ablation time while the mean diameter decreases to 3 nm at longer ablation time. An original model based on the in-situ ablation/photo-fragmentation physical process is developed, and it very well explains the experimental productivity findings. The reported phenomenological model has a general validity, and it can be applied to analyze pulsed laser ablation in liquid in order to optimize the process parameters for higher productivity. Finally, an outlook is given towards gram per hour yield of ultra-small silicon nanoparticles.

© 2014 Optical Society of America

OCIS Codes
(350.3390) Other areas of optics : Laser materials processing
(160.4236) Materials : Nanomaterials
(220.4241) Optical design and fabrication : Nanostructure fabrication

ToC Category:
Laser Microfabrication

History
Original Manuscript: December 12, 2013
Revised Manuscript: January 10, 2014
Manuscript Accepted: January 12, 2014
Published: February 3, 2014

Citation
Romuald Intartaglia, Komal Bagga, and Fernando Brandi, "Study on the productivity of silicon nanoparticles by picosecond laser ablation in water: towards gram per hour yield," Opt. Express 22, 3117-3127 (2014)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-22-3-3117


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