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Optics Express

Optics Express

  • Editor: Andrew M. Weiner
  • Vol. 22, Iss. 8 — Apr. 21, 2014
  • pp: 8831–8842

Violet-green excitation for NIR luminescence of Yb3+ ions in Bi2O3-B2O3-SiO2-Ga2O3 glasses

Weiwei Li, Jimeng Cheng, Guoying Zhao, Wei Chen, Lili Hu, Malgorzata Guzik, and Georges Boulon  »View Author Affiliations


Optics Express, Vol. 22, Issue 8, pp. 8831-8842 (2014)
http://dx.doi.org/10.1364/OE.22.008831


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Abstract

60Bi2O3-20B2O3-10SiO2-10Ga2O3 glasses doped with 1-9 mol% Yb2O3 were prepared and investigated mainly on their violet-green excitation for the typical NIR emission of Yb3+, generally excited in the NIR. Two violet excitation bands at 365 nm and 405 nm are related to Yb2+ and Bi3+. 465 nm excitation band and 480 nm absorption band in the blue-green are assigned to Bi0 metal nanoparticles/grains. Yb-content-dependence of the excitation and absorption means that Bi0 is the reduced product of Bi3+, but greatly competed by the redox reaction of Yb2+↔Yb3+. It is proved that the violet-green excitations result in the NIR emission of Yb3+. On the energy transfer, the virtual level of Yb3+-Yb3+ as well as Bi0 dimers probably plays an important role. An effective and controllable way is suggested to achieve nano-optical applications by Bi0 metal nanoparticles/grains and Yb3+.

© 2014 Optical Society of America

OCIS Codes
(160.2750) Materials : Glass and other amorphous materials
(160.5690) Materials : Rare-earth-doped materials
(250.5230) Optoelectronics : Photoluminescence
(220.4241) Optical design and fabrication : Nanostructure fabrication

ToC Category:
Materials

History
Original Manuscript: January 24, 2014
Revised Manuscript: March 22, 2014
Manuscript Accepted: March 22, 2014
Published: April 7, 2014

Citation
Weiwei Li, Jimeng Cheng, Guoying Zhao, Wei Chen, Lili Hu, Malgorzata Guzik, and Georges Boulon, "Violet-green excitation for NIR luminescence of Yb3+ ions in Bi2O3-B2O3-SiO2-Ga2O3 glasses," Opt. Express 22, 8831-8842 (2014)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-22-8-8831


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