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Optics Express

Optics Express

  • Editor: Andrew M. Weiner
  • Vol. 22, Iss. 8 — Apr. 21, 2014
  • pp: 9063–9072

2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line

Julien Réhault, Margherita Maiuri, Cristian Manzoni, Daniele Brida, Jan Helbing, and Giulio Cerullo  »View Author Affiliations

Optics Express, Vol. 22, Issue 8, pp. 9063-9072 (2014)

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We introduce a new scheme for two-dimensional IR spectroscopy in the partially collinear pump-probe geometry. Translating birefringent wedges allow generating phase-locked pump pulses with exceptional phase stability, in a simple and compact setup. A He-Ne tracking scheme permits to scan continuously the acquisition time. For a proof-of-principle demonstration we use lithium niobate, which allows operation up to 5 μm. Exploiting the inherent perpendicular polarizations of the two pump pulses, we also demonstrate signal enhancement and scattering suppression.

© 2014 Optical Society of America

OCIS Codes
(300.6300) Spectroscopy : Spectroscopy, Fourier transforms
(300.6340) Spectroscopy : Spectroscopy, infrared
(300.6530) Spectroscopy : Spectroscopy, ultrafast
(320.7160) Ultrafast optics : Ultrafast technology

ToC Category:

Original Manuscript: February 19, 2014
Revised Manuscript: March 21, 2014
Manuscript Accepted: March 21, 2014
Published: April 7, 2014

Julien Réhault, Margherita Maiuri, Cristian Manzoni, Daniele Brida, Jan Helbing, and Giulio Cerullo, "2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line," Opt. Express 22, 9063-9072 (2014)

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