Recently, we have shown theoretically and experimentally that anomalous dispersion can be employed to enhance the mirror displacement sensitivity of a ring resonator, for applications such as vibrometry, gravitational wave detection and rotation sensing [
1
M. S. Shahriar, G. S. Pati, R. Tripathi, V. Gopal, M. Messall, and K. Salit, “Ultrahigh enhancement in absolute and relative rotation sensing using fast and slow light,” Phys. Rev. A
75(5), 053807 (2007). [CrossRef]
–
4
M. S. Shahriar and M. Salit, “Application of fast-light in gravitational wave detection with interferometers and resonators,” J. Mod. Opt.
55(19), 3133–3147 (2008). [CrossRef]
].This is accomplished by realizing the so-called White Light Cavity (WLC) [
5
A. Wicht, K. Danzmann, M. Fleischhauer, M. Scully, G. Miiller, and R. H. Rinkleff, “White-light cavities, atomic phase coherence, and gravitational wave detectors,” Opt. Commun.
134(1-6), 431–439 (1997). [CrossRef]
–
8
H. Wu and M. Xiao, “White-light cavity with competing linear and nonlinear dispersions,” Phys. Rev. A
77(3), 031801 (2008). [CrossRef]
] which contains a medium with anomalous dispersion [
9
A. Rocco, A. Wicht, R. H. Rinkleff, and K. Danzmann, “Anomalous dispersion of transparent atomic two- and three-level ensembles,” Phys. Rev. A
66(5), 053804 (2002). [CrossRef]
,
10
L. J. Wang, A. Kuzmich, and A. Dogariu, “Gain-assisted superluminal light propagation,” Nature
406(6793), 277–279 (2000). [CrossRef]
[PubMed]
] tuned so that the wavelength becomes independent of frequency. The sensitivity can be defined broadly as
, where
f is the resonance frequency and
L is the length of the cavity. In general,
where
is the sensitivity of the empty cavity, and
SWLC
is that of the WLC. Under ideal conditions, ξ = 1/n
g, where n
g is the group index. For vanishing n
g, the value of ξ diverges. However, higher order non-linearities within the anomalous dispersion profile prevents the divergence, limiting ξ to a finite value that can be as large as 10
7 for realistic condition. This process is called superluminal enhancement since the group velocity of light far exceeds the free space velocity of light.
However, as discussed previously in Refs 1&3, this enhanced sensitivity does not lead to a corresponding improvement in the minimum measurable mirror displacement or rate of rotation, which is proportional to the linewidth of the cavity. This is because the WLC is broadened by a factor that essentially matches the enhancement in sensitivity. In order to circumvent this constraint, it is necessary to make use of an active cavity, as discussed also in Refs 1&3. To see why, consider, for example, a ring laser gyroscope (RLG). In an RLG, the rate of rotation is proportional to the beat frequency between the two counter-propagating modes. If the RLG is now operated in the WLC mode, the rotation sensitivity will scale by ξ, just as described above. However, the quantum-limited frequency noise, which is proportional to the lifetime of a photon in the cavity, would remain unchanged [
1
M. S. Shahriar, G. S. Pati, R. Tripathi, V. Gopal, M. Messall, and K. Salit, “Ultrahigh enhancement in absolute and relative rotation sensing using fast and slow light,” Phys. Rev. A
75(5), 053807 (2007). [CrossRef]
,
3
G. S. Pati, M. Salit, K. Salit, and M. S. Shahriar, “Demonstration of a tunable-bandwidth white-light interferometer using anomalous dispersion in atomic vapor,” Phys. Rev. Lett.
99(13), 133601 (2007). [CrossRef]
[PubMed]
]. Thus, the minimum measurable rotation rate will improve by a factor of ξ. Variation of this model can be used to measure vibrations, gravitational wave as well as other effects with a similarly enhanced sensitivity, by employing a ring laser in a suitable configuration.
Thus, in order to make use of the anomalous dispersion to enhance the sensitivity of devices such as a gyroscope, a vibrometer or a gravitational wave detector, it is necessary to develop a ring laser that behaves like a WLC: a superluminal laser. At a first glance, it is far from obvious as to how one might realize such a laser. A simple approach might make use of a gain profile with two adjacent peaks as used for realizing a WLC. The dispersion in the zone between the peaks would be negative, and could be tailored to produce the vanishing value of the group index necessary for superluminal propagation. However, there is an apparent problem with this approach. Under the steady state operating condition, the laser gain profile as a function of frequency is flat, with a constant value matching the round trip loss. For frequencies where the gain is less than loss, the gain profile matches the unsaturated one. The overall profile is therefore non-analytic at the boundaries of these regions. Under such a condition, the Karmers-Kronig (KK) relations [
11
J. S. Toll, “Causality and the dispersion relation: logical foundation,” Phys. Rev.
104(6), 1760–1770 (1956). [CrossRef]
–
13
G. J. Troup and A. Bambini, “The use of the modified Kramers-Kronig relation in the rate equation approach of laser theory,” Phys. Lett.
45A, 393 (1973).
] cannot be used, and it is not obvious what the dispersion profile would be [
14H. Yum, and M. S. Shahriar, “Pump-probe model for the Kramers-Kronig relations in a laser,” to appear in J. Opt. (preprint can be viewed at http://arxiv.org/abs/1003.3686)
]. In this paper, we show how a careful analysis of the behavior of the laser reveals an effective negative dispersion. Specifically, we show that if the gain profile has a dip in the middle, the lasing mode centered at the dip behaves like a WLC, with its frequency becoming highly sensitive to mirror displacement. The enhancement factor can be as high as 1.8 × 10
5, comparable to what is achievable in a passive cavity.
In what follows, we make use of the semi-classical equation of motion for an effectively single mode ring laser [
15M. O. Scully, and W. E. Lamb, Laser Physics, (Westview Press, Boulder, CO, 1974).
]. First, we consider light in a ring laser cavity which contains a dispersive medium. The phase and amplitude of the field are described by a set of self-consistency equations:
where ϕ is the round-trip phase shift, ν is the lasing frequency, and Ω is the resonant frequency of the cavity in the absence of the medium. Ω is given by 2π
mc/
L where
L is the length of the cavity,
c is the vacuum speed of light, and
m is the mode number. χ′ and χ″ are the real and imaginary part of the susceptibility of the medium, respectively.
E is the field amplitude, and
Q is the cavity quality factor. ν
0 is the frequency around which χ″ is symmetric. Ω = ν
0 for a particular length of the cavity:
L = L0
. In our model,
L will be allowed to deviate from
L0
, thereby making Ω differ from ν
0. For simplicity, we assume a situation where lasing is unidirectional, made possible by the presence of an optical diode inside the cavity. Any loss induced by the diode is included in
Q.
For convenience, we define the parameters,
,
. The derivatives
and
characterize the resonant frequency shifts under a perturbation of
L in the empty and filled cavity, respectively. We consider the ratio,
to determine if the amount of the frequency shift is enhanced (
R>1) or diminished (
R<1) by the intracavity medium. To derive
R, we begin with
Eq. (1a). In steady state (
) subtracting ν
0 from both sides, differentiating with respect to
L, and applying
, we get
. By substituting
for
, we get:
In order to determine the value of
R, it is necessary to know how χ′ depends on ν. In case of a passive cavity, this would be determined solely by the response of the medium to a weak probe, and would be related to χ″ by the KK relations. In the case of an active cavity, however, this is no longer true, since χ′ depends indirectly on E, which varies as a function of ν, as determined by a self-consistent solution of
Eq. (1). In the later parts of the paper, we explore this interdependence of χ′ and E in detail in order to establish the behavior of the superluminal laser.
We can at this point develop additional insight into the behavior of
R by simply assuming that χ′ is antisymmetric around ν = ν
0 (to be validated later). We can then expand χ′ around ν = ν
0, keeping terms up to (Δν)
3 where Δν = ν−ν
0. We get
where
(n = 1 or 3). Since χ′ is assumed to be antisymmetric around ν
0, we have
. Differentiating χ′ with respect to ν, and inserting χ′ and the derivative of χ′ in
Eq. (2), we get:
. Here, we have dropped terms that are small due to the fact that
. Note that if χ′ is assumed to be linear, corresponding to keeping only the first two terms in the expansion of χ′, the enhancement factor simplifies to:
.
To illustrate the physical meaning of this result, we note first that the index can be expressed as . The group index can then be written as , where and . Thus, the enhancement factor in this linear limit is given simply as R≈1/ng. For normal dispersion (ng>1), R becomes less than one. Hence, the resonant frequency shift with respect to the length variation decreases compared to the shift in an empty cavity. For anomalous dispersion (ng<1), the frequency shift is amplified to be equal to 1/ng times the amount of the shift in the empty cavity.
In order to determine the actual value of
R for an active cavity, we need first to establish the explicit dependence of χ′ on the lasing frequency, ν. To this end, we first solve
Eq. (1b) in steady state (
) so that
for
. Since χ″ is a function of
E and ν, the solution to the equation yields the saturated electric field
E in steady state inside the laser cavity as a function of the lasing frequency ν.
Let us consider the case in which the cavity contains a medium with a narrow absorption as well as a medium with a broad gain. This configuration creates a gain profile with a dip in the center. The imaginary part of the susceptibility χ″ can then be written as:
where
, (
k = e or i). We use the subscript “e” for the “envelope” gain profile and “i” for the narrower absorption profile.
Using the modified Kramers-Kronig (MKK) relation [
12
H. C. Bolton and G. J. Troup, “The modification of the Kronig-Kramers relations under saturation conditions,” Philos. Mag.
19(159), 477–485 (1969). [CrossRef]
,
13
G. J. Troup and A. Bambini, “The use of the modified Kramers-Kronig relation in the rate equation approach of laser theory,” Phys. Lett.
45A, 393 (1973).
] for the saturated susceptibility, we can then express the real part of the susceptibility χ′ as:
Here Ω
i (Ω
e) is the Rabi frequency equal to
(
) where
(
) is the dipole moment associated with the absorbing (amplifying) medium. The gain and the absorption linewidths are denoted by Γ
e and Γ
i, respectively. Using the Wigner–Weisskopf model [
16M. O. Scully, and M. S. Zubairy, Quantum Optics , (Cambridge University Press, New York, NY, 1997).
] for spontaneous emission, we can define two parameters:
and
. In terms of these parameters, the Rabi frequencies can then be expressed as
and
. The gain parameters can then be expressed as
and
, where ε
0 is the permittivity of free space, and N
e and N
i represent the density of quantum systems for the absorptive and the amplifying media, respectively.
It is instructive to consider first the case of a conventional gain medium, by setting G
i = 0. From
Eq. (3), χ′ and χ″ are then simply related to each other as
. From
, it then follows that
. The expression for χ′ is linear in ν, and antisymmetric around ν
0. Note that according to
Eq. (1b),
, where Γ
c is the empty cavity linewidth. Therefore, we find from
R in the linear limit that
, where
. Since n
g>1, this implies a reduction in sensitivity when compared to an empty cavity. In a typical laser,
is very small so that this reduction is rather insignificant. The behavior of such a system in the context of the KK relations is discussed in detail in Ref.14, which also addresses the inadequacies of previous studies.
For the case of a conventional laser medium discussed above, it was easy to determine the value of χ′ because of the simple ratio between χ′ and χ″. In particular, this ratio does not depend on the laser intensity. However, for the general case (i.e. G
i≠0), the two terms in χ″ are highly dissimilar. As such, it is no longer possible to find a ratio between χ′ and χ″ that is independent of the laser intensity. Thus, in this case, we need to determine first the manner in which the laser intensity depends on all the parameters, including ν. We define
I≡|
E|
2 so that
and
. By setting
Eq. (3a) equal to −1/
Q, we get
aI
2 +
bI +
c≡0, where
a,
b, and
c are function of various parameters. We keep the solution that is positive over the lasing bandwidth:
. Substituting this solution for
I to evaluate Ω
i
2 and Ω
e
2, in
Eq. (3b) we get an analytic expression for χ′.
The behavior of χ′ can be understood by plotting it as a function of ν. For illustration, we consider Γ
e = 2π × 10
9s
−1, Γ
i = 2π × 10
7s
−1, ν
0 = 2π × 3.8 × 10
14 s
−1, N
e = 9 × 10
6, and N
i = 1.2645 × 10
11. To fulfill the lasing condition in the spectral range of the absorption dip, we consider the gain peak
and the absorption depth
so as to ensure
at ν = ν
0 where ε is a small fraction. For a given value of G
e, the choice of ε is critical in determining the optimal behavior of χ′. The particular choice of ε = 0.11591 was arrived at via a simple numerical search through the parameter space.
Figure 1
shows χ′ as a function of ν. Note first that far away from ν = ν
0, it agrees asymptotically with the linear value of χ′ for the case of G
i = 0, indicated by the dotted line. The inset figure shows an expanded view of χ′. The steep negative slope of χ′ around around ν = ν
0 is the feature necessary to produce the fast light effect (n
g≈0).
Fig. 1 Real part of the steady-state susceptibility for the combined absorbing and amplifying media (solid line), and the conventional gain medium (dashed line). The inset shows an expanded view of the solid line in the main figure
We can now evaluate the enhancement factor,
R, as expressed in
Eq. (2). We note first that
, where
is evaluated from the solution of the quadratic equation for
I, and
and
are evaluated from
Eq. (3b). Inserting
and
Eq. (3b) in
Eq. (2), we find
R as a function of ν. This is shown in
Fig. 2
for the parameters mentioned above. The insets (a) and (b) show a view expanded horizontally and a view on a linear vertical scale, respectively. The enhancement reaches a peak value of ~1.8 × 10
5 at the center of the gain dip [inset (a)], drops to a minimum (~0.89) and increases to a value close to unity [inset (b)]. These attributes are consistent with the behavior of χ′ shown in
Fig. 1. The peak value of
R corresponds to the steep negative dispersion. As the dispersion turns around and becomes positive, the value of
R drops significantly below unity. Finally, as the dispersion reaches the weak, positive asymptotic value, we recover the behavior expected of a conventional laser, with
R being very close to, but less than unity [inset (b)].
Fig. 2 Sensitivity enhancement associated with
Eq. (2). The inset (a) shows
R in
Eq. (2) in an expanded view (solid line), and its value in the linear limit (dotted line). The inset (b) is an expanded view of
R with a linear vertical scale.
The black lines shown in
Fig. 2 correspond to the exact value of
R given by
Eq. (2). It is also instructive to consider the approximate values of
R, where we assume χ′ to be linear. This is shown by the dotted line in inset (a). Of course, this linear approximation is valid only over a very small range around ν = ν
0. However, it does show clearly that the peak value of
R can be understood simply to be due to the linear, negative dispersion at ν = ν
0.
The enhancement factor R indicates how the lasing frequency ν changes when the length of the cavity, L, is changed. It is also instructive to view graphically the dependence of ν on L explicitly. As discussed earlier, in the empty cavity, we have ν0 = 2πmc/L0
, where ν0 is the resonance frequency (chosen to coincide with the center of the dispersion profile). For concreteness, we have used ν0 = 2π × 3.8 × 1014, corresponding to the D2 transition in Rubidium atoms. We now choose a particular value of the mode number m, so that L is close to one meter. Specifically m = 1282051 yields L0
= 0.99999978 meter.
When the dispersive gain medium is present, the lasing frequency will be ν = ν
0 if
L is kept at
L0
. If
L deviates from
L0
, then ν changes to a different value. Specifically,
, and
from
Eq. (1a) in steady state, so that
. Using the dependence of χ′ on ν as shown in
Fig. 1, we can thus plot L as a function of ν, as shown in
Fig. 3
. Even though
L is plotted on the vertical axis, this plot should be interpreted as showing how ν changes as
L is varied. For ν far away from ν
0, the variation of ν as a function of
L is essentially similar to that of an empty cavity, indicated by the dotted line.
Fig. 3 Illustration of relation between L−L0
and ν−ν0 for |ν−ν0|/2π<80MHz. Dotted line shows the behavior for an empty cavity. The inset shows an expanded view for |ν−ν0|/2π<100kHz.
Around ν = ν
0, a small change in
L corresponds to a very big change in ν as displayed in the inset figure. Specifically, we see that Δ
L≈10
−13 meter produces
f≡Δν/(2π)≈10
5Hz, corresponding to Δ
f/Δ
L~10
18. In contrast, for a bare cavity, Δ
L≈2 × 10
−7 produces Δν/(2π)≈8 × 10
7Hz, corresponding to Δ
f/Δ
L~4 × 10
14. The value of Δ
f/Δ
L for a conventional laser is also very close to this value, as indicated by the convergence of the dotted and solid lines for ν far away from the superluminal region. Thus the enhancement factor,
R, is ~2.5 × 10
3. If we zoom in even more, we will eventually see that as Δ
L→0, we have
R~1.8 × 10
5, as shown in
Fig. 2.
The scheme proposed here for a superluminal laser may be realizable in many different ways. For example, the gain profile can be produced by a diode pumped alkali laser [
17
W. F. Krupke, R. J. Beach, V. K. Kanz, and S. A. Payne, “Resonance transition 795-nm rubidium laser,” Opt. Lett.
28(23), 2336–2338 (2003). [CrossRef]
[PubMed]
]. The dip in the gain profile can be produced by inserting a Raman probe, following the technique shown in Ref.18.
Figure 4
displays the corresponding energy levels, and the experimental configuration to realize a superluminal laser.
Figure 4(a) illustrates the atomic transitions associated with the process for producing a broadband gain profile. The diode pump, applied from the side along the D2 transition, induces population inversion for the D1 transition in the presence of a buffer gas of
4He [
17
W. F. Krupke, R. J. Beach, V. K. Kanz, and S. A. Payne, “Resonance transition 795-nm rubidium laser,” Opt. Lett.
28(23), 2336–2338 (2003). [CrossRef]
[PubMed]
].
Figure 4(b) shows the enegy levels within the D1 transition used for producing the Raman depletion. The lasing beam acts as the Raman pump. The Raman probe is produced by sampling a part of the laser output, and shifting it in frequency with an acousto-optic modulator, operating at the frequency that matches the hyperfine splitting in the ground state [
18
G. S. Pati, M. Salit, K. Salit, and M. S. Shahriar, “Simultaneous slow and fast light effects using probe gain and pump depletion via Raman gain in atomic vapor,” Opt. Express
17(11), 8775–8780 (2009). [CrossRef]
[PubMed]
]. An additional optical pumping beam is applied to produce the population inversion among the metastable hyperfine states necessary for the Raman gain and depletion. Thus, the laser light experiences the Raman dip in the cell B, as illustarted in fig.(c). Efforts are underway in our laboratory to realize such a scheme.
Fig. 4 Energy levels for (a) 795-nm Rb laser to produce broadband gain, (b) Raman depletion to induce narrowband absorption dip. (c) Schematics of the experimental set-up to realize a superluminal laser: PBS, polarizing beam splitter; BS, beam splitter; AOM, acousto-optic modulator. Note that the superluminal laser is the same as the Raman pump. The scheme shown is for 85Rb atoms. The broadband gain is produced by side-pumping with a diode laser array.
To summarize, we have shown that the effective dispersion experienced by a laser frequency is indirectly sensitive to the spectral profile of the unsaturated gain, even though the saturated gain becomes flat, equaling the cavity loss. Specifically, we have shown that a dip in the gain profile when properly tuned, leads to a superluminal group velocity for the lasing mode. The displacement sensitivity of the lasing frequency is enhanced by nearly five orders of magnitude with a wide range of sensing application, including gyroscopy, vibrometry and gravitational wave detection. We also outline an experimental scheme for realizing such a superluminal laser.