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Beaming circularly polarized photons from quantum dots coupled with plasmonic spiral antenna |
Optics Express, Vol. 20, Issue 17, pp. 19297-19304 (2012)
http://dx.doi.org/10.1364/OE.20.019297
Acrobat PDF (2850 KB)
Abstract
Coupling nanoscale emitters via optical antennas enables comprehensive control of photon emission in terms of intensity, directivity and polarization. In this work we report highly directional emission of circularly polarized photons from quantum dots coupled to a spiral optical antenna. The structural chirality of the spiral antenna imprints spin state to the emitted photons. Experimental results reveal that a circular polarization extinction ratio of 10 is obtainable. Furthermore, increasing the number of turns of the spiral gives rise to higher antenna gain and directivity, leading to higher field intensity and narrower angular width of emission pattern in the far field. For a five-turn Archimedes’ spiral antenna, field intensity increase up to 70-fold simultaneously with antenna directivity of 11.7 dB has been measured in the experiment. The highly directional circularly polarized photon emission from such optically coupled spiral antenna may find important applications in single molecule sensing, quantum optics information processing and integrated photonic circuits as a nanoscale spin photon source.
© 2012 OSA
1. Introduction
T. Kosako, Y. Kadoya, and H. F. Hofmann, “Directional control of light by a nano-optical Yagi-Uda Antenna,” Nat. Photonics 4(5), 312–315 (2010). [CrossRef]
P. Mühlschlegel, H. J. Eisler, O. J. Martin, B. Hecht, and D. W. Pohl, “Resonant optical antennas,” Science 308(5728), 1607–1609 (2005). [CrossRef] [PubMed]
H. A. Atwater and A. Polman, “Plasmonics for improved photovoltaic devices,” Nat. Mater. 9(3), 205–213 (2010). [CrossRef] [PubMed]
J. A. Schuller, E. S. Barnard, W. Cai, Y. C. Jun, J. S. White, and M. L. Brongersma, “Plasmonics for extreme light concentration and manipulation,” Nat. Mater. 9(3), 193–204 (2010). [CrossRef] [PubMed]
H. Aouani, O. Mahboub, N. Bonod, E. Devaux, E. Popov, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Bright unidirectional fluorescence emission of molecules in a nanoaperture with plasmonic corrugations,” Nano Lett. 11(2), 637–644 (2011). [CrossRef] [PubMed]
T. Kosako, Y. Kadoya, and H. F. Hofmann, “Directional control of light by a nano-optical Yagi-Uda Antenna,” Nat. Photonics 4(5), 312–315 (2010). [CrossRef]
A. G. Curto, G. Volpe, T. H. Taminiau, M. P. Kreuzer, R. Quidant, and N. F. van Hulst, “Unidirectional emission of a quantum dot coupled to a nanoantenna,” Science 329(5994), 930–933 (2010). [CrossRef] [PubMed]
H. Aouani, O. Mahboub, N. Bonod, E. Devaux, E. Popov, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Bright unidirectional fluorescence emission of molecules in a nanoaperture with plasmonic corrugations,” Nano Lett. 11(2), 637–644 (2011). [CrossRef] [PubMed]
H. Aouani, O. Mahboub, E. Devaux, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Plasmonic antennas for directional sorting of fluorescence emission,” Nano Lett. 11(6), 2400–2406 (2011). [CrossRef] [PubMed]
T. Ming, L. Zhao, H. Chen, K. C. Woo, J. Wang, and H. Q. Lin, “Experimental evidence of plasmophores: plasmon-directed polarized emission from gold nanorod-fluorophore hybrid nanostructures,” Nano Lett. 11(6), 2296–2303 (2011). [CrossRef] [PubMed]
G. Rui, R. L. Nelson, and Q. Zhan, “Circularly polarized unidirectional emission via a coupled plasmonic spiral antenna,” Opt. Lett. 36(23), 4533–4535 (2011). [CrossRef] [PubMed]
T. Ming, L. Zhao, H. Chen, K. C. Woo, J. Wang, and H. Q. Lin, “Experimental evidence of plasmophores: plasmon-directed polarized emission from gold nanorod-fluorophore hybrid nanostructures,” Nano Lett. 11(6), 2296–2303 (2011). [CrossRef] [PubMed]
2. Methods
2.1 Design of optical spiral antenna and fabrication
2.2 FEM simulation and physical mechanisms
2.3 Experimental setup
Q. Zhan, “Cylindrical vector beams: from mathematical concepts to applications,” Adv. Opt. Photon. 1(1), 1–57 (2009). [CrossRef]
W. Chen and Q. Zhan, “Realization of an evanescent Bessel beam via surface plasmon interference excited by a radially polarized beam,” Opt. Lett. 34(6), 722–724 (2009). [CrossRef] [PubMed]
3. Experimental results and discussion
G. Rui, R. L. Nelson, and Q. Zhan, “Circularly polarized unidirectional emission via a coupled plasmonic spiral antenna,” Opt. Lett. 36(23), 4533–4535 (2011). [CrossRef] [PubMed]
4. Conclusions
R. M. Osgood Jr, N. C. Panoiu, J. I. Dadap, X. Liu, X. Chen, I. Hsieh, E. Dulkeith, W. M. J. Green, and Y. A. Vlasov, “Engineering nonlinearities in nanoscale optical systems: physics and applications in dispersion-engineered silicon nanophotonic wires,” Adv. Opt. Photon. 1(1), 162–235 (2009). [CrossRef]
R. F. Oulton, V. J. Sorger, T. Zentgraf, R. M. Ma, C. Gladden, L. Dai, G. Bartal, and X. Zhang, “Plasmon lasers at deep subwavelength scale,” Nature 461(7264), 629–632 (2009). [CrossRef] [PubMed]
S. Wang, S. Ota, B. Guo, J. Ryu, C. Rhodes, Y. Xiong, S. Kalim, L. Zeng, Y. Chen, M. A. Teitell, and X. Zhang, “Subcellular resolution mapping of endogenous cytokine secretion by nano-plasmonic-resonator sensor array,” Nano Lett. 11(8), 3431–3434 (2011). [CrossRef] [PubMed]
Acknowledgments
References and links
W. L. Stutzman and G. A. Thiele, Antenna theory and design (Wiley, 1998). | |
T. Kosako, Y. Kadoya, and H. F. Hofmann, “Directional control of light by a nano-optical Yagi-Uda Antenna,” Nat. Photonics 4(5), 312–315 (2010). [CrossRef] | |
P. Mühlschlegel, H. J. Eisler, O. J. Martin, B. Hecht, and D. W. Pohl, “Resonant optical antennas,” Science 308(5728), 1607–1609 (2005). [CrossRef] [PubMed] | |
S. Lal, S. Link, and N. J. Halas, “Nano-optics from sensing to waveguiding,” Nat. Photonics 1(11), 641–648 (2007). [CrossRef] | |
E. Cubukcu, E. A. Kort, K. B. Crozier, and F. Capasso, “Plasmonic laser antenna,” Appl. Phys. Lett. 89(9), 093120 (2006). [CrossRef] | |
H. A. Atwater and A. Polman, “Plasmonics for improved photovoltaic devices,” Nat. Mater. 9(3), 205–213 (2010). [CrossRef] [PubMed] | |
J. A. Schuller, E. S. Barnard, W. Cai, Y. C. Jun, J. S. White, and M. L. Brongersma, “Plasmonics for extreme light concentration and manipulation,” Nat. Mater. 9(3), 193–204 (2010). [CrossRef] [PubMed] | |
J. R. Lakowicz and Y. Fu, “Modification of single molecule fluorescence near metallic nanostructure,” Laser Photon. Rev. 3(1-2), 221–232 (2009). [CrossRef] | |
H. Aouani, O. Mahboub, N. Bonod, E. Devaux, E. Popov, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Bright unidirectional fluorescence emission of molecules in a nanoaperture with plasmonic corrugations,” Nano Lett. 11(2), 637–644 (2011). [CrossRef] [PubMed] | |
A. G. Curto, G. Volpe, T. H. Taminiau, M. P. Kreuzer, R. Quidant, and N. F. van Hulst, “Unidirectional emission of a quantum dot coupled to a nanoantenna,” Science 329(5994), 930–933 (2010). [CrossRef] [PubMed] | |
H. Aouani, O. Mahboub, E. Devaux, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Plasmonic antennas for directional sorting of fluorescence emission,” Nano Lett. 11(6), 2400–2406 (2011). [CrossRef] [PubMed] | |
T. Ming, L. Zhao, H. Chen, K. C. Woo, J. Wang, and H. Q. Lin, “Experimental evidence of plasmophores: plasmon-directed polarized emission from gold nanorod-fluorophore hybrid nanostructures,” Nano Lett. 11(6), 2296–2303 (2011). [CrossRef] [PubMed] | |
G. Rui, R. L. Nelson, and Q. Zhan, “Circularly polarized unidirectional emission via a coupled plasmonic spiral antenna,” Opt. Lett. 36(23), 4533–4535 (2011). [CrossRef] [PubMed] | |
Q. Zhan, “Cylindrical vector beams: from mathematical concepts to applications,” Adv. Opt. Photon. 1(1), 1–57 (2009). [CrossRef] | |
W. Chen and Q. Zhan, “Realization of an evanescent Bessel beam via surface plasmon interference excited by a radially polarized beam,” Opt. Lett. 34(6), 722–724 (2009). [CrossRef] [PubMed] | |
R. M. Osgood Jr, N. C. Panoiu, J. I. Dadap, X. Liu, X. Chen, I. Hsieh, E. Dulkeith, W. M. J. Green, and Y. A. Vlasov, “Engineering nonlinearities in nanoscale optical systems: physics and applications in dispersion-engineered silicon nanophotonic wires,” Adv. Opt. Photon. 1(1), 162–235 (2009). [CrossRef] | |
R. F. Oulton, V. J. Sorger, T. Zentgraf, R. M. Ma, C. Gladden, L. Dai, G. Bartal, and X. Zhang, “Plasmon lasers at deep subwavelength scale,” Nature 461(7264), 629–632 (2009). [CrossRef] [PubMed] | |
S. Wang, S. Ota, B. Guo, J. Ryu, C. Rhodes, Y. Xiong, S. Kalim, L. Zeng, Y. Chen, M. A. Teitell, and X. Zhang, “Subcellular resolution mapping of endogenous cytokine secretion by nano-plasmonic-resonator sensor array,” Nano Lett. 11(8), 3431–3434 (2011). [CrossRef] [PubMed] |
OCIS Codes
(240.6680) Optics at surfaces : Surface plasmons
(260.5430) Physical optics : Polarization
(350.5610) Other areas of optics : Radiation
ToC Category:
Optics at Surfaces
History
Original Manuscript: June 21, 2012
Revised Manuscript: July 26, 2012
Manuscript Accepted: August 3, 2012
Published: August 8, 2012
Citation
Guanghao Rui, Weibin Chen, Don C. Abeysinghe, Robert L. Nelson, and Qiwen Zhan, "Beaming circularly polarized photons from quantum dots coupled with plasmonic spiral antenna," Opt. Express 20, 19297-19304 (2012)
http://www.opticsinfobase.org/oe/abstract.cfm?URI=oe-20-17-19297
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References
- W. L. Stutzman and G. A. Thiele, Antenna theory and design (Wiley, 1998).
- T. Kosako, Y. Kadoya, and H. F. Hofmann, “Directional control of light by a nano-optical Yagi-Uda Antenna,” Nat. Photonics4(5), 312–315 (2010). [CrossRef]
- P. Mühlschlegel, H. J. Eisler, O. J. Martin, B. Hecht, and D. W. Pohl, “Resonant optical antennas,” Science308(5728), 1607–1609 (2005). [CrossRef] [PubMed]
- S. Lal, S. Link, and N. J. Halas, “Nano-optics from sensing to waveguiding,” Nat. Photonics1(11), 641–648 (2007). [CrossRef]
- E. Cubukcu, E. A. Kort, K. B. Crozier, and F. Capasso, “Plasmonic laser antenna,” Appl. Phys. Lett.89(9), 093120 (2006). [CrossRef]
- H. A. Atwater and A. Polman, “Plasmonics for improved photovoltaic devices,” Nat. Mater.9(3), 205–213 (2010). [CrossRef] [PubMed]
- J. A. Schuller, E. S. Barnard, W. Cai, Y. C. Jun, J. S. White, and M. L. Brongersma, “Plasmonics for extreme light concentration and manipulation,” Nat. Mater.9(3), 193–204 (2010). [CrossRef] [PubMed]
- J. R. Lakowicz and Y. Fu, “Modification of single molecule fluorescence near metallic nanostructure,” Laser Photon. Rev.3(1-2), 221–232 (2009). [CrossRef]
- H. Aouani, O. Mahboub, N. Bonod, E. Devaux, E. Popov, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Bright unidirectional fluorescence emission of molecules in a nanoaperture with plasmonic corrugations,” Nano Lett.11(2), 637–644 (2011). [CrossRef] [PubMed]
- A. G. Curto, G. Volpe, T. H. Taminiau, M. P. Kreuzer, R. Quidant, and N. F. van Hulst, “Unidirectional emission of a quantum dot coupled to a nanoantenna,” Science329(5994), 930–933 (2010). [CrossRef] [PubMed]
- H. Aouani, O. Mahboub, E. Devaux, H. Rigneault, T. W. Ebbesen, and J. Wenger, “Plasmonic antennas for directional sorting of fluorescence emission,” Nano Lett.11(6), 2400–2406 (2011). [CrossRef] [PubMed]
- T. Ming, L. Zhao, H. Chen, K. C. Woo, J. Wang, and H. Q. Lin, “Experimental evidence of plasmophores: plasmon-directed polarized emission from gold nanorod-fluorophore hybrid nanostructures,” Nano Lett.11(6), 2296–2303 (2011). [CrossRef] [PubMed]
- G. Rui, R. L. Nelson, and Q. Zhan, “Circularly polarized unidirectional emission via a coupled plasmonic spiral antenna,” Opt. Lett.36(23), 4533–4535 (2011). [CrossRef] [PubMed]
- Q. Zhan, “Cylindrical vector beams: from mathematical concepts to applications,” Adv. Opt. Photon.1(1), 1–57 (2009). [CrossRef]
- W. Chen and Q. Zhan, “Realization of an evanescent Bessel beam via surface plasmon interference excited by a radially polarized beam,” Opt. Lett.34(6), 722–724 (2009). [CrossRef] [PubMed]
- R. M. Osgood, N. C. Panoiu, J. I. Dadap, X. Liu, X. Chen, I. Hsieh, E. Dulkeith, W. M. J. Green, and Y. A. Vlasov, “Engineering nonlinearities in nanoscale optical systems: physics and applications in dispersion-engineered silicon nanophotonic wires,” Adv. Opt. Photon.1(1), 162–235 (2009). [CrossRef]
- R. F. Oulton, V. J. Sorger, T. Zentgraf, R. M. Ma, C. Gladden, L. Dai, G. Bartal, and X. Zhang, “Plasmon lasers at deep subwavelength scale,” Nature461(7264), 629–632 (2009). [CrossRef] [PubMed]
- S. Wang, S. Ota, B. Guo, J. Ryu, C. Rhodes, Y. Xiong, S. Kalim, L. Zeng, Y. Chen, M. A. Teitell, and X. Zhang, “Subcellular resolution mapping of endogenous cytokine secretion by nano-plasmonic-resonator sensor array,” Nano Lett.11(8), 3431–3434 (2011). [CrossRef] [PubMed]
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