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Reflected fourth-harmonic radiation from a centrosymmetric crystal

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Abstract

We present measurements of fourth-harmonic generation in reflection from the interface between two centrosymmetric media Si001SiO2, using femtosecond pulses well below damage threshold. Analyses of signal amplitudes, rotational anisotropy, and sensitivity to surface roughening reveal that the surface dipole fourth-harmonic contribution dominates the bulk quadrupole contribution much more strongly than for second-harmonic generation.

© 1998 Optical Society of America

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