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Optics Letters

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  • Editor: Alan E. Willner
  • Vol. 35, Iss. 9 — May. 1, 2010
  • pp: 1395–1397

Time-domain spectroscopy of molecular free-induction decay in the infrared

Ian Coddington, William C. Swann, and Nathan R. Newbury  »View Author Affiliations


Optics Letters, Vol. 35, Issue 9, pp. 1395-1397 (2010)
http://dx.doi.org/10.1364/OL.35.001395


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Abstract

Time-domain spectroscopy using dual, coherent frequency combs is used to measure free-induction decay from a molecular gas sample in the near-IR with a time-domain signal-to-noise ratio of 10 6 over a 6 ns window at 55 fs time resolution (corresponding to the 9 THz source bandwidth) and a frequency/timing accuracy set by the frequency combs. The free-induction decay exhibits the expected periodic pulses from the rephasing of the multiply excited rovibrational levels. This demonstration represents the first high-resolution, high-accuracy, broadband measurement of optical free-induction decay, to our knowledge.

© 2010 U.S. Government

OCIS Codes
(120.6200) Instrumentation, measurement, and metrology : Spectrometers and spectroscopic instrumentation
(140.4050) Lasers and laser optics : Mode-locked lasers
(320.7100) Ultrafast optics : Ultrafast measurements

ToC Category:
Ultrafast Optics

History
Original Manuscript: November 23, 2009
Revised Manuscript: February 18, 2010
Manuscript Accepted: March 2, 2010
Published: April 26, 2010

Citation
Ian Coddington, William C. Swann, and Nathan R. Newbury, "Time-domain spectroscopy of molecular free-induction decay in the infrared," Opt. Lett. 35, 1395-1397 (2010)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-35-9-1395


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References

  1. A. Abragam, The Principles of Nuclear Magnetism (Clarendon, 1961).
  2. B. C. Dian, G. G. Brown, K. O. Douglass, and B. H. Pate, Science 320, 924 (2008). [CrossRef] [PubMed]
  3. H. Harde, S. Keiding, and D. Grischkowsky, Phys. Rev. Lett. 66, 1834 (1991). [CrossRef] [PubMed]
  4. A. Bartels, R. Cerna, C. Kistner, A. Thoma, F. Hudert, C. Janke, and T. Dekorsy, Rev. Sci. Instrum. 78, 035107 (2007). [CrossRef] [PubMed]
  5. R. G. Brewer and R. Shoemaker, Phys. Rev. Lett. 27, 631 (1971). [CrossRef]
  6. A. Z. Genack, D. A. Weitz, R. M. Macfarlane, R. M. Shelby, and A. Schenzle, Phys. Rev. Lett. 45, 438 (1980). [CrossRef]
  7. T. Mishina and Y. Masumotot, Phys. Rev. Lett. 71, 2785 (1993). [CrossRef] [PubMed]
  8. N. Tsurumachi, T. Fuji, S. Kawato, T. Hattori, and H. Nakatsuka, Opt. Lett. 19, 1867 (1994). [CrossRef] [PubMed]
  9. I. Coddington, W. C. Swann, and N. R. Newbury, Phys. Rev. Lett. 100, 013902 (2008). [CrossRef] [PubMed]
  10. F. Keilmann, C. Gohle, and R. Holzwarth, Opt. Lett. 29, 1542 (2004). [CrossRef] [PubMed]
  11. A. Schliesser, M. Brehm, F. Keilmann, and D. van der Weide, Opt. Express 13, 9029 (2005). [CrossRef] [PubMed]
  12. T. Yasui, Y. Kabetani, E. Saneyoshi, S. Yokoyama, and T. Araki, Appl. Phys. Lett. 88, 241104 (2006). [CrossRef]
  13. P. Giaccari, J. D. Deschenes, P. Saucier, J. Genest, and P. Tremblay, Opt. Express 16, 4347 (2008). [CrossRef] [PubMed]
  14. B. Bernhardt, A. Ozawa, P. Jacquet, M. Jacquey, Y. Kobayashi, T. Udem, R. Holzwarth, G. Guelachvili, T. W. Hansch, and N. Picque, Nat. Photonics 4, 55 (2009). [CrossRef]
  15. S. Schiller, Opt. Lett. 27, 766 (2002). [CrossRef]
  16. I. Coddington, W. C. Swann, L. Nenadovic, and N. R. Newbury, Nat. Photonics 3, 351 (2009). [CrossRef]
  17. I. Coddington, W. C. Swann, and N. R. Newbury, Opt. Lett. 34, 2153 (2009). [CrossRef] [PubMed]
  18. P. R. Griffiths and J. A. Haseth, Fourier Transform Infrared Spectrometry (Wiley-Interscience, 2007). [CrossRef]
  19. W. C. Swann and S. L. Gilbert, J. Opt. Soc. Am. B 22, 1749 (2005). [CrossRef]
  20. N. R. Newbury, I. Coddington, and W. C. Swann, Opt. Express 18, 7929 (2010). [CrossRef] [PubMed]

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