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Optics Letters

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  • Editor: Alan E. Willner
  • Vol. 37, Iss. 12 — Jun. 15, 2012
  • pp: 2337–2339

Ultrabroadband femtosecond two-dimensional ultraviolet transient absorption

Gerald Auböck, Cristina Consani, Frank van Mourik, and Majed Chergui  »View Author Affiliations


Optics Letters, Vol. 37, Issue 12, pp. 2337-2339 (2012)
http://dx.doi.org/10.1364/OL.37.002337


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Abstract

We present a broadband two-dimensional transient absorption setup for the UV around 300 nm with a time resolution of 150 fs. A narrowband, frequency tunable pump pulse and a broadband probe pulse are generated from the output of a noncollinear optical parametric amplifier operated at 20 kHz repetition rate and combined in a spectrally resolved transient absorption experiment. The high repetition rate and low noise of the setup allow us to acquire high quality two-dimensional data as a function of time delay with an unsurpassed frequency window of 10,000 and 8000cm1 along the probe and pump axis, respectively. The performance of the setup is demonstrated on 2,5-Diphenyloxazol dissolved in cyclohexane.

© 2012 Optical Society of America

OCIS Codes
(300.0300) Spectroscopy : Spectroscopy
(320.0320) Ultrafast optics : Ultrafast optics

ToC Category:
Ultrafast Optics

History
Original Manuscript: March 26, 2012
Manuscript Accepted: March 30, 2012
Published: June 8, 2012

Citation
Gerald Auböck, Cristina Consani, Frank van Mourik, and Majed Chergui, "Ultrabroadband femtosecond two-dimensional ultraviolet transient absorption," Opt. Lett. 37, 2337-2339 (2012)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-37-12-2337


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References

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