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Sub-Doppler tunable far-infrared spectroscopy

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Abstract

The first experimental observations to our knowledge of sub-Doppler linewidths in a cell made using tunable far-infrared radiation are reported. A double-resonance scheme has been used, combining CO2-laser infrared radiation with tunable far-infrared radiation to observe a sub-Doppler line shape in an excited vibrational state of CH3OH.

© 1987 Optical Society of America

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