Subharmonic resonances in higher-order collision-enhanced wave mixing in a sodium-seeded flame
Optics Letters, Vol. 12, Issue 11, pp. 912-914 (1987)
http://dx.doi.org/10.1364/OL.12.000912
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Abstract
Using four-, six-, and eight-wave-mixing geometries, we observe subharmonic resonances in collision-enhanced spectra in a sodium-seeded hydrogen–air flame. Appearing at high intensity, these resonances occur at ±1/2, ±1/3, ±1/4, and ±1/5 times the frequency of the ground-state hyperfine splitting ωhfs. We argue that these resonances result from higher-order processes, specifically χ(n), where n ≥ 5. In particular, to describe the resonances at ±ωhfs/5, at least χ(13) is required. These high-order collision-enhanced effects are true perturbative nonlinearities and not sequential four-wave mixing processes.
© 1987 Optical Society of America
Citation
Rick Trebino and Larry A. Rahn, "Subharmonic resonances in higher-order collision-enhanced wave mixing in a sodium-seeded flame," Opt. Lett. 12, 912-914 (1987)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-12-11-912
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