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  • Vol. 21, Iss. 18 — Sep. 15, 1996
  • pp: 1448–1450

Self-dispersive sum-frequency generation at interfaces

E. W. M. van der Ham, Q. H. F. Vrehen, and E. R. Eliel  »View Author Affiliations


Optics Letters, Vol. 21, Issue 18, pp. 1448-1450 (1996)
http://dx.doi.org/10.1364/OL.21.001448


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Abstract

We employ the self-dispersive nature of infrared–visible sum-frequency generation at interfaces to record sum-frequency spectra of molecular monolayers with a spectral resolution of a few inverse centimeters, using IR light with a spectral content of approximately 50 cm−1.

© 1996 Optical Society of America

History
Original Manuscript: April 29, 1996
Published: September 15, 1996

Citation
E. W. M. van der Ham, Q. H. F. Vrehen, and E. R. Eliel, "Self-dispersive sum-frequency generation at interfaces," Opt. Lett. 21, 1448-1450 (1996)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-21-18-1448


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References

  1. Y. R. Shen, Nature (London) 337, 519 (1989). [CrossRef]
  2. The angular dispersion for a reflection grating is given by dθdω=−sin θi+sin θrω cos θr, an expression similar to Eq. (1). Here θi and θr are the angles of incidence and diffraction, respectively.
  3. R. J. Bakker, D. A. Jaroszynski, A. F. G. van der Meer, D. Oepts, P. W. van Amersfoort, IEEE J. Quantum Electron. 30, 1635 (1994). [CrossRef]
  4. E. R. Eliel, E. W. M. van der Ham, Q. H. F. Vrehen, M. Barmentlo, G. W. ’t Hooft, J. M. Auerhammer, A. F. G. van der Meer, P. W. van Amersfoort, Appl. Phys. A 60, 113 (1995). [CrossRef]
  5. G. M. H. Knippels, A. F. G. van der Meer, R. F. X. A. M. Mols, P. W. van Amersfoort, R. B. Vrijen, D. J. Maas, L. D. Noordam, Opt. Commun. 118, 546 (1995). [CrossRef]
  6. Note that we assume here that the IVSFG response of gold is spectrally flat over this frequency interval.
  7. P. Guyot-Sionnest, Proc. SPIE 1858, 334 (1993). [CrossRef]
  8. D. Lin-Vien, N. B. Colthup, W. G. Fateley, J. G. Grassell, Infrared and Raman Characteristic Frequencies of Organic Molecules (Academic, Boston, Mass., 1991).

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