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Optics Letters

Optics Letters


  • Editor: Anthony J. Campillo
  • Vol. 30, Iss. 23 — Dec. 1, 2005
  • pp: 3222–3224

Broadband coherent anti-Stokes Raman scattering spectroscopy of nitrogen using a picosecond modeless dye laser

Sukesh Roy, Terrence R. Meyer, and James R. Gord  »View Author Affiliations

Optics Letters, Vol. 30, Issue 23, pp. 3222-3224 (2005)

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Broadband picosecond coherent anti-Stokes Raman scattering (CARS) spectroscopy of nitrogen is demonstrated using 145 - ps pump and probe beams and a 115 - ps Stokes beam with a spectral bandwidth of 5 nm . This is, to our knowledge, the first demonstration of broadband CARS using subnanosecond lasers. The short temporal envelope of the laser pulses and the broadband spectral nature of the Stokes beam will enable nonresonant-background-free, single-shot, or time-dependent spectroscopy in high-pressure or hydrocarbon-rich environments. Successful correlation of room-temperature broadband picosecond N 2 CARS with a theoretical spectrum is presented.

© 2005 Optical Society of America

OCIS Codes
(120.1740) Instrumentation, measurement, and metrology : Combustion diagnostics
(140.2050) Lasers and laser optics : Dye lasers
(190.4380) Nonlinear optics : Nonlinear optics, four-wave mixing
(300.6230) Spectroscopy : Spectroscopy, coherent anti-Stokes Raman scattering
(300.6290) Spectroscopy : Spectroscopy, four-wave mixing
(320.5390) Ultrafast optics : Picosecond phenomena

ToC Category:

Sukesh Roy, Terrence R. Meyer, and James R. Gord, "Broadband coherent anti-Stokes Raman scattering spectroscopy of nitrogen using a picosecond modeless dye laser," Opt. Lett. 30, 3222-3224 (2005)

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