High-spectral-resolution coherent anti-Stokes Raman scattering with interferometrically detected broadband chirped pulses
Optics Letters, Vol. 31, Issue 10, pp. 1543-1545 (2006)
http://dx.doi.org/10.1364/OL.31.001543
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Abstract
To achieve high-spectral-resolution multiplex coherent anti-Stokes Raman scattering (CARS), one typically uses a narrowband pump pulse and a broadband Stokes pulse. This is to ensure a correspondence between anti-Stokes and vibrational frequencies. We obtain high-resolution CARS spectra of isopropanol, using a broadband chirped pump pulse and a broadband Stokes pulse, by detecting the anti-Stokes pulse with spectral interferometry. With the temporally resolved anti-Stokes signal, we can remove the chirp of the anti-Stokes pulse and restore high spectral resolution while also rejecting nonresonant scattering.
© 2006 Optical Society of America
OCIS Codes
(190.7110) Nonlinear optics : Ultrafast nonlinear optics
(300.6450) Spectroscopy : Spectroscopy, Raman
ToC Category:
Spectroscopy
History
Original Manuscript: January 9, 2006
Revised Manuscript: February 17, 2006
Manuscript Accepted: February 22, 2006
Citation
Gareth W. Jones, Daniel L. Marks, Claudio Vinegoni, and Stephen A. Boppart, "High-spectral-resolution coherent anti-Stokes Raman scattering with interferometrically detected broadband chirped pulses," Opt. Lett. 31, 1543-1545 (2006)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-31-10-1543
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