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Optics Letters

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  • Editor: Anthony J. Campillo
  • Vol. 31, Iss. 22 — Nov. 15, 2006
  • pp: 3330–3332

Wavelength-tunable ultrashort-pulse output of a photonic-crystal fiber designed to resolve ultrafast molecular dynamics

Anatoly A. Ivanov, Mikhail V. Alfimov, and Aleksei M. Zheltikov  »View Author Affiliations


Optics Letters, Vol. 31, Issue 22, pp. 3330-3332 (2006)
http://dx.doi.org/10.1364/OL.31.003330


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Abstract

Wavelength-tunable 100 fs pulses generated through the soliton self-frequency shift in a photonic-crystal fiber are employed to visualize femtosecond coherence and population relaxation dynamics in molecular aggregates by means of time-resolved sum-frequency generation. This technique reveals an ultrafast dephasing of coherent molecular excitations with a phase relaxation time of about 120 fs and resolves an ultrafast switching of the nonlinear-optical response of molecular aggregates.

© 2006 Optical Society of America

OCIS Codes
(190.4370) Nonlinear optics : Nonlinear optics, fibers
(190.7110) Nonlinear optics : Ultrafast nonlinear optics

ToC Category:
Nonlinear Optics

History
Original Manuscript: April 25, 2006
Revised Manuscript: July 7, 2006
Manuscript Accepted: August 10, 2006
Published: October 26, 2006

Citation
Anatoly A. Ivanov, Mikhail V. Alfimov, and Aleksei M. Zheltikov, "Wavelength-tunable ultrashort-pulse output of a photonic-crystal fiber designed to resolve ultrafast molecular dynamics," Opt. Lett. 31, 3330-3332 (2006)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-31-22-3330


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