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Optics Letters

| RAPID, SHORT PUBLICATIONS ON THE LATEST IN OPTICAL DISCOVERIES

  • Editor: Anthony J Campillo
  • Vol. 32, Iss. 1 — Jan. 1, 2007
  • pp: 59–61

Modulated conjugation as a means for attaining a record high intrinsic hyperpolarizability

Javier Pérez-Moreno, Yuxia Zhao, Koen Clays, and Mark G. Kuzyk  »View Author Affiliations


Optics Letters, Vol. 32, Issue 1, pp. 59-61 (2007)
http://dx.doi.org/10.1364/OL.32.000059


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Abstract

We report on a series of chromophores that have been synthesized with a modulated conjugation path between donor and acceptor. Hyper-Rayleigh scattering measurements of the best molecule show an enhanced intrinsic hyperpolarizability that breaches the apparent limit of all previously studied molecules.

© 2006 Optical Society of America

OCIS Codes
(020.0020) Atomic and molecular physics : Atomic and molecular physics
(020.4900) Atomic and molecular physics : Oscillator strengths
(190.0190) Nonlinear optics : Nonlinear optics

ToC Category:
Nonlinear Optics

History
Original Manuscript: August 14, 2006
Revised Manuscript: October 9, 2006
Manuscript Accepted: October 10, 2006
Published: December 13, 2006

Citation
Javier Pérez-Moreno, Yuxia Zhao, Koen Clays, and Mark G. Kuzyk, "Modulated conjugation as a means for attaining a record high intrinsic hyperpolarizability," Opt. Lett. 32, 59-61 (2007)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-32-1-59


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References

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  2. M. G. Kuzyk, Phys. Rev. Lett. 85, 1218 (2000). [CrossRef] [PubMed]
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  9. Y. Shen, L. Qiu, J. Hao, Y. Zhao, J. Pérez-Moreno, M. G. Kuzyk, and K. Clays, 'Complex hybrid conjugation as a means for improving the intrinsic hyperpolarizability,' manuscript in preparation.
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