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Enhancement of high-harmonic generation by laser-induced cluster vibration

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Abstract

Sharp periodic enhancement of high-harmonic generation synchronized to prepulse-induced cluster vibration is observed. Tenfold enhancement of high-harmonic-generation efficiency is achieved by optimal selection of the prepulse–pump delay. This strong correlation between high-harmonic generation and cluster vibration also provides a new tool for studying the vibrational dynamics of nanometer atomic clusters.

© 2007 Optical Society of America

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