OSA's Digital Library

Optics Letters

Optics Letters


  • Editor: Anthony J. Campillo
  • Vol. 32, Iss. 6 — Mar. 15, 2007
  • pp: 707–709

Chirped-pulse adiabatic control in coherent anti-Stokes Raman scattering for imaging of biological structure and dynamics

Svetlana A. Malinovskaya and Vladimir S. Malinovsky  »View Author Affiliations

Optics Letters, Vol. 32, Issue 6, pp. 707-709 (2007)

View Full Text Article

Enhanced HTML    Acrobat PDF (240 KB)

Browse Journals / Lookup Meetings

Browse by Journal and Year


Lookup Conference Papers

Close Browse Journals / Lookup Meetings

Article Tools



Two novel control methods based on adiabatic passage are proposed to be implemented in coherent anti-Stokes Raman scattering (CARS) microscopy for noninvasive imaging of biological structure and dynamics. The first method provides optimal pulse-area control of the resonant vibrational transitions by using a pair of equally linear-chirped pulses. The second method, named the “roof” method, utilizes the chirp sign variation at the central time and gives robust adiabatic excitation of the resonant vibrational mode. Both methods are robust with respect to suppression of the off-resonant transitions. The methods allow one to achieve chemical sensitivity with high resolution and can be used to obtain CARS spectra of biological molecules with efficiently suppressed background.

© 2007 Optical Society of America

OCIS Codes
(300.6230) Spectroscopy : Spectroscopy, coherent anti-Stokes Raman scattering
(320.5540) Ultrafast optics : Pulse shaping
(320.7120) Ultrafast optics : Ultrafast phenomena

ToC Category:
Ultrafast Optics

Original Manuscript: October 17, 2006
Revised Manuscript: December 20, 2006
Manuscript Accepted: December 29, 2006
Published: February 15, 2007

Virtual Issues
Vol. 2, Iss. 4 Virtual Journal for Biomedical Optics

Svetlana A. Malinovskaya and Vladimir S. Malinovsky, "Chirped-pulse adiabatic control in coherent anti-Stokes Raman scattering for imaging of biological structure and dynamics," Opt. Lett. 32, 707-709 (2007)

Sort:  Author  |  Year  |  Journal  |  Reset  


  1. A. Zumbusch, G. Holtom, and X. S. Xie, Phys. Rev. Lett. 92, 4142 (1999). [CrossRef]
  2. E. O. Potma, W. P. de Boeij, P. J. M. van Haastert, and D. A. Wiersma, Proc. Natl. Acad. Sci. USA 98, 1577 (2001). [CrossRef] [PubMed]
  3. E. O. Potma and X. S. Xie, Opt. Photon. News 15(11), 40 (2004). [CrossRef]
  4. C. L. Evans, E. O. Potma, M. Puorishaag, D. Cote, C. P. Lin, and X. S. Xie, Proc. Natl. Acad. Sci. USA 102, 16807 (2005). [CrossRef] [PubMed]
  5. N. Dudovich, D. Oron, and Y. Silberberg, Nature 418, 512 (2002). [CrossRef] [PubMed]
  6. B. Yellampalle, R. D. Averitt, A. Efimov, and A. J. Taylor, Opt. Express 13, 7672 (2005). [CrossRef] [PubMed]
  7. J. Ogilvie, D. Debarre, X. Solinas, J. Martin, E. Beaurepaire, and M. Joffre, Opt. Express 14, 759 (2006). [CrossRef] [PubMed]
  8. E. Gershgoren, R. A. Bartels, J. T. Fourkas, R. Tobey, M. M. Murnane, and H. C. Kapteyn, Opt. Lett. 28, 361 (2003). [CrossRef] [PubMed]
  9. K. P. Knutsen, J. C. Johnson, A. E. Miller, P. B. Petersen, and R. J. Saykally, Chem. Phys. Lett. 387, 436 (2004). [CrossRef]
  10. S. A. Malinovskaya, Phys. Rev. A 73, 033416 (2006). [CrossRef]
  11. T. Hellerer, A. M. K. Enejder, and A. Zumbusch, Appl. Phys. Lett. 85, 25 (2004). [CrossRef]
  12. G. W. H. Wurpel, J. M. Schins, and M. Müller, Opt. Lett. 27, 1093 (2002). [CrossRef]
  13. E. M. Vartiainen, H. A. Rinia, M. Müller, and M. Bonn, Opt. Express 14, 3622 (2006). [CrossRef] [PubMed]
  14. K. P. Knutsen, B. M. Messer, R. M. Onorato, and R. J. Saykally, J. Phys. Chem. B 110, 5854 (2006). [CrossRef] [PubMed]

Cited By

Alert me when this paper is cited

OSA is able to provide readers links to articles that cite this paper by participating in CrossRef's Cited-By Linking service. CrossRef includes content from more than 3000 publishers and societies. In addition to listing OSA journal articles that cite this paper, citing articles from other participating publishers will also be listed.


Fig. 1 Fig. 2 Fig. 3
Fig. 4

« Previous Article  |  Next Article »

OSA is a member of CrossRef.

CrossCheck Deposited