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Optics Letters

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  • Editor: Alan E. Willner
  • Vol. 34, Iss. 16 — Aug. 15, 2009
  • pp: 2471–2473

Ultrafast third-order nonlinear optical properties of Zn Pc ( O Bu ) 6 ( NCS ) DMSO solution

DeGui Kong, WuBiao Duan, XueRu Zhang, ChunYing He, Qing Chang, YuXiao Wang, YaChen Gao, and YingLin Song  »View Author Affiliations


Optics Letters, Vol. 34, Issue 16, pp. 2471-2473 (2009)
http://dx.doi.org/10.1364/OL.34.002471


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Abstract

The ultrafast third-order nonlinear optical properties of Zn Pc ( O Bu ) 6 ( NCS ) /dimethyl sulfoxide solution are investigated by optical Kerr effect (OKE) and pump–probe techniques with femtosecond pulses. Using C S 2 as the reference, the third-order susceptibility of the sample solution is obtained as about 1.40 × 10 14 esu at a concentration of 3.00 × 10 5 M . The second hyperpolarizability for the sample solution is deduced to be as large as 2.35 × 10 31 esu . The dynamic characteristics of the nonlinear optical response and the origins of the OKE signal can be attributed to excited singlet state populations.

© 2009 Optical Society of America

OCIS Codes
(190.0190) Nonlinear optics : Nonlinear optics
(190.3270) Nonlinear optics : Kerr effect
(320.2250) Ultrafast optics : Femtosecond phenomena

ToC Category:
Nonlinear Optics

History
Original Manuscript: April 13, 2009
Manuscript Accepted: June 22, 2009
Published: August 11, 2009

Citation
DeGui Kong, WuBiao Duan, XueRu Zhang, ChunYing He, Qing Chang, YuXiao Wang, YaChen Gao, and YingLin Song, "Ultrafast third-order nonlinear optical properties of ZnPc(OBu)6(NCS)/DMSO solution," Opt. Lett. 34, 2471-2473 (2009)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-34-16-2471


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