Compact phase-stable design for single- and double-quantum two-dimensional electronic spectroscopy
Optics Letters, Vol. 34, Issue 21, pp. 3301-3303 (2009)
http://dx.doi.org/10.1364/OL.34.003301
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Abstract
We report a compact, easy to align, and passively phase-stabilized setup for recording two-dimensional (2D) electronic spectra in three different phase-matching directions in the boxcar geometry. Passive phase stabilization is achieved by a diffractive optical element, the use of refractive optics for introducing pulse delays, and the use of common optics for all pulses. Representative 2D spectra correlating single- and double-quantum coherences in a molecular aggregate are presented.
© 2009 Optical Society of America
OCIS Codes
(300.6290) Spectroscopy : Spectroscopy, four-wave mixing
(300.6300) Spectroscopy : Spectroscopy, Fourier transforms
ToC Category:
Spectroscopy
History
Original Manuscript: July 6, 2009
Revised Manuscript: September 17, 2009
Manuscript Accepted: September 22, 2009
Published: October 23, 2009
Citation
Alexandra Nemeth, Jaroslaw Sperling, Jürgen Hauer, Harald F. Kauffmann, and Franz Milota, "Compact phase-stable design for single- and double-quantum two-dimensional electronic spectroscopy," Opt. Lett. 34, 3301-3303 (2009)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-34-21-3301
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