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Controlling the Raman response of inhomogeneously distributed multiple vibrational modes with optimally shaped light fields

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Abstract

We demonstrate that Raman-effect-assisted transformations of ultrashort pulses in materials with inhomogeneously distributed multiple vibrational modes can be tailored by optimally ordered pulse sequences and appropriate optical sampling. This suggests attractive strategies for a synthesis of few-cycle pulses, enhanced spectral transformation of light fields, and pulse shaping in silica fibers and other materials with multiple Raman modes.

© 2009 Optical Society of America

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