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Optics Letters

| RAPID, SHORT PUBLICATIONS ON THE LATEST IN OPTICAL DISCOVERIES

  • Editor: Alan E. Willner
  • Vol. 35, Iss. 24 — Dec. 15, 2010
  • pp: 4178–4180

Coherent two-dimensional ultraviolet spectroscopy in fully noncollinear geometry

Ulrike Selig, Carl-Friedrich Schleussner, Michael Foerster, Florian Langhojer, Patrick Nuernberger, and Tobias Brixner  »View Author Affiliations


Optics Letters, Vol. 35, Issue 24, pp. 4178-4180 (2010)
http://dx.doi.org/10.1364/OL.35.004178


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Abstract

We introduce fully noncollinear coherent two-dimensional (2D) spectroscopy in the UV domain with an all-reflective and miniaturized setup design. Phase stability is achieved via pairwise beam manipulation, and the concept can be transferred to all wavelength regimes. Here we present results from an implementation that has been optimized for wavelengths between 250 and 375 nm . Interferometric measurements prove phase stability over several hours. We obtained 2D spectra of the nonpolar UV chromophore p-terphenyl in ethanol, excited with 50 fs pulses at 287 nm .

© 2010 Optical Society of America

OCIS Codes
(300.6290) Spectroscopy : Spectroscopy, four-wave mixing
(300.6300) Spectroscopy : Spectroscopy, Fourier transforms
(300.6540) Spectroscopy : Spectroscopy, ultraviolet
(320.0320) Ultrafast optics : Ultrafast optics
(320.7150) Ultrafast optics : Ultrafast spectroscopy

ToC Category:
Spectroscopy

History
Original Manuscript: July 23, 2010
Revised Manuscript: October 8, 2010
Manuscript Accepted: November 9, 2010
Published: December 13, 2010

Citation
Ulrike Selig, Carl-Friedrich Schleussner, Michael Foerster, Florian Langhojer, Patrick Nuernberger, and Tobias Brixner, "Coherent two-dimensional ultraviolet spectroscopy in fully noncollinear geometry," Opt. Lett. 35, 4178-4180 (2010)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-35-24-4178


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