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Optics Letters

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  • Editor: Alan E. Willner
  • Vol. 37, Iss. 24 — Dec. 15, 2012
  • pp: 5058–5060

Purely absorptive fifth-order three-dimensional electronic spectroscopy

Zhengyang Zhang, Kym Lewis Wells, and Howe-Siang Tan  »View Author Affiliations


Optics Letters, Vol. 37, Issue 24, pp. 5058-5060 (2012)
http://dx.doi.org/10.1364/OL.37.005058


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Abstract

We demonstrate a method to measure a purely absorptive fifth-order three-dimensional (3D) electronic spectrum based on a pulse-shaper assisted pump-probe beam geometry setup. The 3D spectra are measured as a function of two independently controlled population times. With phase-cycling and data processing, purely absorptive 3D spectra of chlorophyll a are obtained.

© 2012 Optical Society of America

OCIS Codes
(300.6530) Spectroscopy : Spectroscopy, ultrafast
(320.7150) Ultrafast optics : Ultrafast spectroscopy

ToC Category:
Spectroscopy

History
Original Manuscript: October 1, 2012
Revised Manuscript: October 31, 2012
Manuscript Accepted: November 3, 2012
Published: December 5, 2012

Citation
Zhengyang Zhang, Kym Lewis Wells, and Howe-Siang Tan, "Purely absorptive fifth-order three-dimensional electronic spectroscopy," Opt. Lett. 37, 5058-5060 (2012)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-37-24-5058


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References

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  13. K. L. Wells, Z. Zhang, and J. R. Rouxel, Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371, Singapore, and Laboratoire de Nanotechnologie et d’Instrumentation Optique, Université de Technologie de Troyes-Centre National de la Recherche Scientifique (FRE2671), 12 rue Marie Curie, BP 2060, 10010 Troyes Cedex, France, and H.-S. Tan are preparing a manuscript to be called “Measuring the spectral diffusion of chlorophyll a using two-dimensional electronic spectroscopy.”

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