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Optics Letters

Optics Letters

| RAPID, SHORT PUBLICATIONS ON THE LATEST IN OPTICAL DISCOVERIES

  • Editor: Alan E. Willner
  • Vol. 37, Iss. 24 — Dec. 15, 2012
  • pp: 5058–5060

Purely absorptive fifth-order three-dimensional electronic spectroscopy

Zhengyang Zhang, Kym Lewis Wells, and Howe-Siang Tan  »View Author Affiliations


Optics Letters, Vol. 37, Issue 24, pp. 5058-5060 (2012)
http://dx.doi.org/10.1364/OL.37.005058


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Abstract

We demonstrate a method to measure a purely absorptive fifth-order three-dimensional (3D) electronic spectrum based on a pulse-shaper assisted pump-probe beam geometry setup. The 3D spectra are measured as a function of two independently controlled population times. With phase-cycling and data processing, purely absorptive 3D spectra of chlorophyll a are obtained.

© 2012 Optical Society of America

OCIS Codes
(300.6530) Spectroscopy : Spectroscopy, ultrafast
(320.7150) Ultrafast optics : Ultrafast spectroscopy

ToC Category:
Spectroscopy

History
Original Manuscript: October 1, 2012
Revised Manuscript: October 31, 2012
Manuscript Accepted: November 3, 2012
Published: December 5, 2012

Citation
Zhengyang Zhang, Kym Lewis Wells, and Howe-Siang Tan, "Purely absorptive fifth-order three-dimensional electronic spectroscopy," Opt. Lett. 37, 5058-5060 (2012)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-37-24-5058

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