|
Tomographic imaging of asymmetric molecular orbitals with a two-color multicycle laser field |
Optics Letters, Vol. 37, Issue 24, pp. 5208-5210 (2012)
http://dx.doi.org/10.1364/OL.37.005208
Enhanced HTML 
Acrobat PDF (344 KB)
Abstract
We theoretically demonstrate a scheme for tomographic reconstruction of asymmetric molecular orbitals based on high-order harmonic generation with a two-color multicycle laser field. It is shown that by adjusting the relative phase of the two fields, the returning electrons can be forced to recollide from one direction for all the orientations of molecules. Thus, the reconstruction of the asymmetric orbitals can be carried out with multicycle laser field. This releases the stringent requirement of a single-cycle pulse with a stabilized and controllable carrier-envelope phase for the tomographic imaging of asymmetric molecular orbitals.
© 2012 Optical Society of America
OCIS Codes
(190.4160) Nonlinear optics : Multiharmonic generation
(190.7110) Nonlinear optics : Ultrafast nonlinear optics
ToC Category:
Nonlinear Optics
History
Original Manuscript: October 5, 2012
Revised Manuscript: November 7, 2012
Manuscript Accepted: November 15, 2012
Published: December 13, 2012
Citation
Meiyan Qin, Xiaosong Zhu, Qingbin Zhang, and Peixiang Lu, "Tomographic imaging of asymmetric molecular orbitals with a two-color multicycle laser field," Opt. Lett. 37, 5208-5210 (2012)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-37-24-5208
You do not have subscription access to this journal. Citation lists with outbound citation links are available to subscribers only. You may subscribe either as an OSA member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Log in to access OSA Member Subscription
You do not have subscription access to this journal. Cited by links are available to subscribers only. You may subscribe either as an OSA member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Log in to access OSA Member Subscription
You do not have subscription access to this journal. Figure files are available to subscribers only. You may subscribe either as an OSA member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Log in to access OSA Member Subscription
You do not have subscription access to this journal. Article level metrics are available to subscribers only. You may subscribe either as an OSA member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Log in to access OSA Member Subscription
Related Journal Articles 
- Extreme ultraviolet interferometry measurements with high-order harmonics (OL)
- Nanoscale nonlinear optical process: theoretical modeling of second-harmonic generation for both forbidden and allowed light (OL)
- Cascaded highly nondegenerate four-wave-mixing phenomenon in transparent isotropic condensed media (OL)
- Generation of attosecond pulse trains during the reflection of a very intense laser on a solid surface (JOSAB)
- Size dependence of nonlinear Mie scattering in microdroplets illuminated by ultrashort pulses (JOSAB)
Related Conference Papers
- Quantum computation with femtosecond photon echo
- Quantum computation with femtosecond photon echo
- Temporal Confinement of High Order Harmonic Emission by Polarization Gating
- Role of Laser Self-Focusing for High-Order Harmonic Generation in Extended Gas Cells
- High Harmonic Imaging of Conical Intersections
- Gated Large-Bandwidth Soft-X-Ray Continuum Generation on the Leading Edge of the Driver Pulse
« Previous Article | Next Article »
OSA is a member of 