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Optics Letters

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  • Editor: Alan E. Willner
  • Vol. 38, Iss. 6 — Mar. 15, 2013
  • pp: 950–952

Stimulated Raman scattering from sulfur-II produced by laser decomposition of liquid carbon disulfide

Wenhui Fang, Zhanlong Li, Dongfei Li, Zuowei Li, Mi Zhou, Zhiwei Men, and Chenglin Sun  »View Author Affiliations


Optics Letters, Vol. 38, Issue 6, pp. 950-952 (2013)
http://dx.doi.org/10.1364/OL.38.000950


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Abstract

Stimulated Raman scattering (SRS) of sulfur-II (S-II) phase was investigated by laser decomposition of liquid carbon disulfide. As a matter of fact, above a threshold of the laser intensity, it is suggested that a strong shock wave is generated in the liquid carbon disulfide, which is decomposed owing to the induced high dynamic pressure and temperature. One bending mode E frequency at 289cm1 and one symmetric stretching mode A1 frequency at 490cm1 of S-II phase were observed. The SRS spectra indicated that S-II structure is formed by laser decomposition, as the strong shock wave generates the stable pressure-temperature range of S-II phase. The dynamic high-pressure and static-electric field generated by laser-induced breakdown results in the softening A1 mode becoming more hardened.

© 2013 Optical Society of America

OCIS Codes
(190.2640) Nonlinear optics : Stimulated scattering, modulation, etc.
(300.6390) Spectroscopy : Spectroscopy, molecular

ToC Category:
Nonlinear Optics

History
Original Manuscript: January 30, 2013
Manuscript Accepted: February 4, 2013
Published: March 13, 2013

Citation
Wenhui Fang, Zhanlong Li, Dongfei Li, Zuowei Li, Mi Zhou, Zhiwei Men, and Chenglin Sun, "Stimulated Raman scattering from sulfur-II produced by laser decomposition of liquid carbon disulfide," Opt. Lett. 38, 950-952 (2013)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-38-6-950


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