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Optics Letters

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  • Vol. 7, Iss. 1 — Jan. 1, 1982
  • pp: 25–27

XeI(2π1/22Σ1/2) excimer emission at 1.3 μm

E. Gerck and E. Fill  »View Author Affiliations


Optics Letters, Vol. 7, Issue 1, pp. 25-27 (1982)
http://dx.doi.org/10.1364/OL.7.000025


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Abstract

The collisional enhancing of the magnetic dipole transition I(52P1/2–52P3/2) at 1.3152 μm by Xe is shown to proceed over an exciplex channel: I(52P1/2) + Xe → XeI(2π1/2) → I(52P3/2) + Xe + hν(1.3 μm). The pseudo-first-order rate coefficient for this process is (1.6 ± 0.2) × 10−18 molecule−1 cm3 sec−1. The termolecular rate coefficient for XeI(2π1/2) excimer production is (2 ± 1) × 10−35 molecule−2 cm6 sec−1. The radiative lifetime of the XeI excimer state is of the order of 100 nsec. Similar effects are briefly reported for C2F6, SF6 Kr, Ar, and i-C3F7I.

© 1982 Optical Society of America

History
Original Manuscript: September 25, 1981
Published: January 1, 1982

Citation
E. Gerck and E. Fill, "XeI(2π1/22Σ1/2) excimer emission at 1.3 μm," Opt. Lett. 7, 25-27 (1982)
http://www.opticsinfobase.org/ol/abstract.cfm?URI=ol-7-1-25


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References

  1. L. S. Ershov, V. Yu. Zalesskii, “Collision-induced I(52P1/2–52P3/2) radiative transition,” Sov. J. Quantum Electron. 8, 649 (1978). [CrossRef]
  2. M. Galanti, W. Thieme, K. J. Witte, “Saturation energy density and line profile of the atomic iodine laser transition at high pressure,” IEEE J. Quantum Electron. QE-17, 1817 (1981). [CrossRef]
  3. K. Hohla, K. L. Kompa, in Handbook of Chemical Lasers, R. W. F. Gross, J. F. Bott, eds. (Wiley, New York, 1976).
  4. G. Black, R. L. Sharpless, T. G. Slanger, “Collision-induced emission from O(1S) by He, Ar, N2, H2, Kr, and Xe,” J. Chem. Phys. 63, 4546 (1975). [CrossRef]
  5. G. Black, R. L. Sharpless, T. G. Slanger, “Collision-induced emission from S(1S) by He, Ar, N2, H2, Kr, and Xe,” J. Chem. Phys. 63, 4551 (1975). [CrossRef]
  6. This process was not known to proceed, at least partially, over a radiative channel. The rate should be equal to or less than the total quenching rate by i-C3F7I: S. L. Dobycliin et al., Kvantovaya Elektron. (Moscow) 5, 2461 (1978).
  7. J. J. Ewing, C. A. Brau, “Emission spectrum of XeI* in electron-beam-excited Xe/I2 mixtures,” Phys. Rev. A 12, 129 (1975). [CrossRef]
  8. P. J. Hay, T. H. Dunning, “The covalent and ionic states of the xenon halides,” J. Chem. Phys. 69, 2209 (1978). [CrossRef]
  9. D. Rogovin, P. Avizonis, “Collision-induced gain,” Appl. Phys. Lett. 38, 666 (1981). [CrossRef]

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