2 μm lasers continue to be of interest in medicine based on
absorption by water in the human body [
1H. W. Kang, H. Lee, J. Petersen, J. H. Teichman, and A. J. Welch, Proc. SPIE
6078, 607815 (2006). [CrossRef]
] or by
in remote-sensing applications [
2T. M. Taczak and D. K. Killinger, Appl. Opt.
37, 8460
(1998). [CrossRef]
] and are essential in the detection of wind vortices using lidar
[
3S. M. Hannon and J. A. Thomson, J. Mod. Opt.
41, 2175 (1994). [CrossRef]
]. 2 μm lasers also have the
added benefit of being eye safe [
4G. D. Wilkins, Wright Laboratories Tech. Rep.
WL-TR-96-1017
(1996).
]. The
dual-wavelength operation of the
2 μm laser, if feasible, would allow for the efficient generation of
terahertz waves with multihundred-watt peak
power via a difference-frequency generation
process [
5W. Shi, Y. J. Ding, and P. G. Schunemann, Opt. Commun.
233, 183 (2004). [CrossRef]
].
Laser power scaling with good beam quality can be achieved via
implementation of resonant pump/lase schemes and designing for optimal thermal
management. This may include cryo-cooling, especially where efficiency is the most
critical requirement [
6N. Ter-Gabrielyan, V. Fromzel, T. Lukasiewicz, W. Ryba-Romanowski, and M. Dubinskii, Opt. Lett.
36, 1218 (2011). [CrossRef]
]. While the Ho:YAG
2.1 μm laser meets the criteria of eye safety and emission in an
atmospherically transparent window,
can be a thermally better choice of host for
ions over YAG [
7A. I. Zagumennyi, P. A. Popov, F. Zerouk, Y. D. Zavartsev, S.
A. Kutovoi, and I. A. Shcherbakov, Quantum Electron.
38, 227 (2008). [CrossRef]
], especially for cryo-cooled applications. This was recently demonstrated in
[
8G. A. Newburgh and M. Dubinskii, Proc. SPIE
8039, 803905 (2011). [CrossRef]
], where a
fiber-coupled InGaAsP/InP diode laser
module at
was used to in-band pump a cryo-cooled
single crystal to produce 1.6 W of continuous wave
(CW) output power at 2053 nm. Following this result, a room-temperature laser
version of the
laser was demonstrated with resonant pumping by a much
brighter Tm:YAP laser [
9G. Li, B.-Q. Yao, P.-B. Meng, Y.-L. Ju, and Y.-Z. Wang, Opt. Lett.
36, 2934 (2011). [CrossRef]
]. This laser emitted at
2041, 2053, or 2066 nm but was never shown to emit at multiple wavelengths
simultaneously.
In this Letter, we present the experimental results of a cryo-cooled, resonantly pumped
(at 1966 nm) laser that emits simultaneously at 2053 and
2068 nm with a nearly
quantum-defect-limited optical-to-optical efficiency of . To the best of our knowledge, this is the highest
demonstrated slope efficiency of any -doped laser.
The gain element was cut from a single crystal grown by the
Czochralski method. A section of a boule was selected based on minimal observable stress
birefringence. This section was then cut and polished to form a
laser slab with the -axis orientation perpendicular to the
face. The two faces were antireflection (AR) coated for the
wavelength range 1900 to 2100 nm. The
reflectance at 2050 nm was measured by the vendor to be per surface. The gain element was mounted to the bottom
of a standard liquid-nitrogen-cooled
cryostat using highly thermally conductive
indium cushioning.
The
-axis of the slab was chosen to coincide with the thin
dimension of the gain medium to facilitate cooling as the thermal conductivity of
is at least 50% higher along the
axis versus the
axis (
versus
at 77 K) [
7A. I. Zagumennyi, P. A. Popov, F. Zerouk, Y. D. Zavartsev, S.
A. Kutovoi, and I. A. Shcherbakov, Quantum Electron.
38, 227 (2008). [CrossRef]
].
The simplified optical layout of the experiment is depicted in Fig.
1. The cryostat was set between a pair of cavity
mirrors: a plano–concave (radius of curvature
) dichroic
(
,
) and a
plano–concave (
) output coupler
(reflectivity 71% to 88% at 2050 nm). The two
mirrors were set 125 mm apart and formed a stable cavity. The
cryostat windows were AR coated (1900 to
2100 nm). The transmission loss per cryostat window at 2050 nm was measured to
be
. Transmission losses (2 μm) of the
25 mm long
gain medium were measured to be
per pass. We estimate that the overall round-trip
cavity losses were less than 3%.
Fig. 1. Simplified layout of the experimental laser setup. All the components are
properly listed in the body of the paper.
In order to assess the ultimate laser potential of the gain medium, the laser slab was end-pumped at
1966 nm by a Tm fiber laser collimated and focused by a 20 mm (L1) lens and a
200 mm (L2) lens, respectively. The pump beam at focus had a measured beam quality
factor, , with a radius of . As the laser cavity mode radius
and the
Rayleigh length was 5 mm, we
calculated that the pump beam energy was fully utilized.
The
- and
-polarized absorption cross sections are nearly equal at
(
) [
8G. A. Newburgh and M. Dubinskii, Proc. SPIE
8039, 803905 (2011). [CrossRef]
]. This pump
wavelength was chosen to properly utilize the unpolarized pump source. The relatively
low absorption cross section favors more even pump power distribution along the length
of the slab.
Laser experiments were conducted using a range of output coupler reflectivities,
, 81%, and 88%. As shown in Fig.
2, the results demonstrate high incident
pump-to-laser output conversion efficiencies with all used output couplers. The most
notable observation is the nearly quantum-defect-limited slope efficiency (92%)
laser performance with dual-wavelength
operation in a wide range of pump powers using the
output coupler. Proper care was taken to separate the
transmitted pump light from the laser output by introducing a 1° angular deviation
between the pump and laser axis. It was found that under lasing conditions, nearly 99%
of the pump power at 1966 nm was absorbed in the slab.
Fig. 2. Output power versus incident pump-power dependence for the cryo-cooled
laser
resonantly pumped at 1966 nm,
measured with different output coupler reflectivities : a) , (b) , and (c) .
The dual-wavelength laser operation of the cryo-cooled, resonantly pumped
laser was
analyzed using a Yokogawa
AQ6375 optical spectrum analyzer (OSA).
Beginning with the case in Fig.
2(b), the
laser starts lasing at 2053 nm in
polarization at low pump power (2 to 5.5 W),
transitions to a dual-wavelength regime
with 2053 nm (
) and 2068 nm (
polarization) outputs in the pump power range 5.5 to
12 W, and ends with pure 2068 nm emission beyond 12 W. The polarization
of the 2053 and 2068 nm wavelengths was determined by a diffraction grating and a
polymer thin-film polarizer. No discernible
difference in slope efficiency was observed in transition from a mixed
laser output to one of pure 2068 nm emission. We
measured the output beam quality at full power (
) and determined that the beam quality factor,
, was
along both
and
axes. No astigmatism was observed.
In contrast, in the case in Fig.
2(a),
, the laser starts and maintains lasing at 2053 nm
in the full range of available pump power. For the case in Fig.
2(c),
, the laser emits at 2053 nm only at threshold and
quickly transitions to lasing at 2068 nm only.
An OSA trace of the CW dual-wavelength lasing is presented in Fig.
3. The trace was obtained using the outcoupler with
81% reflectivity and OSA resolution of 0.05 nm. The 2053 nm laser line was
found to be significantly spectrally wider than the 2068 nm laser line, usually
versus
(resolution-limited), respectively, for the entire
range of pump power. The OSA trace shown in Fig.
3 is stable in time, but the trace is the result of signal averaging over
the period of time of
. By simultaneous time-resolved power measurement at
each wavelength, we observed that the power at each of the two wavelengths undergoes
rapid fluctuations (on a millisecond time scale) in such a manner that both powers
nearly anticorrelate in time.
Fig. 3. Laser output spectrum of the resonantly pumped, cryo-cooled
laser at the onset of dual-wavelength lasing.
Presented spectral distribution corresponds to output coupler reflectivity of
81% [Fig.
2(b)] and incident pump
power
.
While spectroscopy at this point does not allow us
to predict exactly when the transition of
lasing from 2053 to 2068 nm occurs, we can anticipate this laser behavior. As
observed in our experiments, a strong correlation exists between the gain-medium
temperature and output-coupler transmission value at the point when the output power at
2053 nm equals that at 2068 nm. For equality to hold, the laser gain at
2053 nm (
) must equal the laser gain at 2068 nm
(
):
where
, is the inversion in the gain medium, and
,
[
9G. Li, B.-Q. Yao, P.-B. Meng, Y.-L. Ju, and Y.-Z. Wang, Opt. Lett.
36, 2934 (2011). [CrossRef]
] are the
ground-state absorption cross sections at 2053 and 2068 nm, respectively. The
stimulated emission cross sections at 2053 and 2068 nm are designated by
and
. Under lasing conditions, the net gain of the medium at
2068 nm must also satisfy the following condition:
where
is the length of the gain medium,
is the single-pass passive loss of the laser cavity,
and
is the gain medium ion number density. This allows us
to write the relation,
Equation (
3) leads us to expect that as
decreases, for
wavelength transition occurs for larger values of
, that is, higher gain temperatures associated with
harder optical pumping.
In conclusion, we have demonstrated the CW
dual-wavelength operation of a
cryogenically cooled, resonantly (in-band)
pumped laser with nearly quantum-defect-limited performance.
The gain element, maintained at approximately 80 K and
pumped by a Tm fiber laser at 1966 nm, emitted at the wavelengths of either 2053 or
2068 nm, or both simultaneously, as a function of the
outcoupler transmittance and the incident
pump power. It was observed that the onset of 2068 nm lasing is correlated with the
heating of the gain medium and the outcoupler transmission value. We observed
laser operation at a mixture of 2053 and 2068 nm
with a nearly quantum-defect-limited slope
efficiency of , which is, to the best of our knowledge, the
highest slope efficiency demonstrated for
any -doped laser.