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The origin of second harmonic generation hotspots in chiral optical metamaterials [Invited]V. K. Valev, X. Zheng, C.G. Biris, A.V. Silhanek, V. Volskiy, B. De Clercq, O. A. Aktsipetrov, M. Ameloot, N. C. Panoiu, G. A. E. Vandenbosch, and V. V. Moshchalkov »View Author Affiliations
V. K. Valev,1,*
X. Zheng,2
C.G. Biris,3
A.V. Silhanek,4
V. Volskiy,2
B. De Clercq,5
O. A. Aktsipetrov,6
M. Ameloot,5
N. C. Panoiu,3
G. A. E. Vandenbosch,2
and V. V. Moshchalkov4
1Molecular Electronics and Photonics, INPAC, Katholieke Universiteit Leuven, Leuven, Belgium 2ESAT-TELEMIC, K. U. Leuven, B-3001 Leuven, Belgium 3Department of Electronic and Electrical Engineering, University College London, Torrington Place, London WC1E 7JE, United Kingdom 4Superconductivity and Magnetism & Pulsed Fields Group, INPAC, Katholieke Universiteit Leuven, Leuven, Belgium 5University Hasselt and transnational University Limburg, BIOMED, Diepenbeek, Belgium 6Department of Physics, Moscow State University, 11992 Moscow, Russia 7Molecular Electronics and Photonics, INPAC, Katholieke Universiteit Leuven, Leuven, Belgium
*Corresponding author: v.k.valev@fys.kuleuven.be |
Optical Materials Express, Vol. 1, Issue 1, pp. 36-45 (2011)
http://dx.doi.org/10.1364/OME.1.000036
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Abstract
Novel ways to detect the handedness in chiral optical metamaterials by means of the second harmonic generation (SHG) process have recently been proposed. However, the precise origin of the SHG emission has yet to be unambiguously established. In this paper, we present computational simulations of both the electric currents and the electromagnetic fields in chiral planar metamaterials, at the fundamental frequency (FF), and discuss the implications of our results on the characteristics of experimentally measured SHG. In particular, we show that the results of our numerical simulations are in good agreement with the experimental mapping of SHG sources. Thus, the SHG in these metamaterials can be attributed to a strong local enhancement of the electromagnetic fields at the FF, which depends on the particular structure of the patterned metamaterial.
© 2011 OSA
OCIS Codes
(240.4350) Optics at surfaces : Nonlinear optics at surfaces
(160.1585) Materials : Chiral media
(160.3918) Materials : Metamaterials
(180.4315) Microscopy : Nonlinear microscopy
ToC Category:
Chiral Optical Materials
History
Original Manuscript: February 3, 2011
Revised Manuscript: March 14, 2011
Manuscript Accepted: March 14, 2011
Published: April 22, 2011
Virtual Issues
Chiral Optical Materials (2011) Optical Materials Express
Citation
V. K. Valev, X. Zheng, C.G. Biris, A.V. Silhanek, V. Volskiy, B. De Clercq, O. A. Aktsipetrov, M. Ameloot, N. C. Panoiu, G. A. E. Vandenbosch, and V. V. Moshchalkov, "The origin of second harmonic generation hotspots in chiral optical metamaterials [Invited]," Opt. Mater. Express 1, 36-45 (2011)
http://www.opticsinfobase.org/ome/abstract.cfm?URI=ome-1-1-36
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- J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett. 105(7), 077401 (2010). [CrossRef] [PubMed]
- W. Fan, S. Zhang, N. C. Panoiu, A. Abdenour, S. Krishna, R. M. Osgood, K. J. Malloy, and S. R. J. Brueck, “Second harmonic generation from a nanopatterned isotropic nonlinear material,” Nano Lett. 6(5), 1027–1030 (2006). [CrossRef]
- V. V. Pavlov, J. Ferré, P. Meyer, G. Tessier, P. Georges, A. Brun, P. Beauvillain, and V. Mathet, “Linear and non-linear magneto-optical studies of Pt/Co/Pt thin films,” J. Phys. Condens. Matter 13(44), 9867–9878 (2001). [CrossRef]
- J. Butet, J. Duboisset, G. Bachelier, I. Russier-Antoine, E. Benichou, C. Jonin, and P.-F. Brevet, “Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium,” Nano Lett. 10(5), 1717–1721 (2010). [CrossRef] [PubMed]
- J. Butet, G. Bachelier, J. Duboisset, F. Bertorelle, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Three-dimensional mapping of single gold nanoparticles embedded in a homogeneous transparent matrix using optical second-harmonic generation,” Opt. Express 18(21), 22314–22323 (2010). [CrossRef] [PubMed]
- J. Butet, G. Bachelier, I. Russier-Antoine, C. Jonin, E. Benichou, and P.-F. Brevet, “Interference between selected dipoles and octupoles in the optical second-harmonic generation from spherical gold nanoparticles,” Phys. Rev. Lett. 105(7), 077401 (2010). [CrossRef] [PubMed]
- J. D. Byers, H. I. Yee, and J. M. Hicks, “A second harmonic generation analog of optical rotatory dispersion for the study of chiral monolayers,” J. Chem. Phys. 101(7), 6233–6241 (1994). [CrossRef]
- T. Petralli-Mallow, T. M. Wong, J. D. Byers, H. I. Yee, and J. M. Hicks, “Circular dichroism spectroscopy at interfaces: a surface second harmonic generation study,” J. Phys. Chem. 97(7), 1383–1388 (1993). [CrossRef]
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- N. Bloembergen, R. K. Chang, S. Jha, and C. H. Lee, “Optical second-harmonic generation in reflection from media with inversion symmetry,” Phys. Rev. 174(3), 813–822 (1968). [CrossRef]
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ACS Nano
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Appl. Opt.
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Appl. Phys. Lett.
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ChemPhysChem
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Chirality
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IEE Proc., Microw. Antennas Propag.
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IEEE Trans. Antenn. Propag.
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IEEE Trans. Microw. Theory Tech.
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J. Appl. Phys.
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J. Chem. Phys.
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J. Mod. Opt.
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J. Opt. A, Pure Appl. Opt.
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J. Opt. Soc. Am. B
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J. Phys. Chem.
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J. Phys. Condens. Matter
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JETP Lett.
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Nano Lett.
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Opt. Express
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Opt. Lett.
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Phys. Rev.
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Phys. Rev. B
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- F. X. Wang, F. J. Rodríguez, W. M. Albers, R. Ahorinta, J. E. Sipe, and M. Kauranen, “Surface and bulk contributions to the second-order nonlinear optical response of a gold film,” Phys. Rev. B 80(23), 233402 (2009). [CrossRef]
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Phys. Rev. B Condens. Matter
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Phys. Rev. Lett.
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